1,089 research outputs found
Bimagnon studies in cuprates with Resonant Inelastic X-ray Scattering at the O K edge. II - The doping effect in La2-xSrxCuO4
We present RIXS data at O K edge from La2-xSrxCuO4 vs. doping between x=0.10
and x=0.22 with attention to the magnetic excitations in the Mid-Infrared
region. The sampling done by RIXS is the same as in the undoped cuprates
provided the excitation is at the first pre-peak induced by doping. Note that
this excitation energy is about 1.5 eV lower than that needed to see bimagnons
in the parent compound. This approach allows the study of the upper region of
the bimagnon continuum around 450 meV within about one third of the Brilluoin
Zone around \Gamma. The results show the presence of damped bimagnons and of
higher even order spin excitations with almost constant spectral weight at all
the dopings explored here. The implications on high Tc studies are briefly
addressed
Inelastic X-ray scattering from valence electrons near absorption edges of FeTe and TiSe
We study resonant inelastic x-ray scattering (RIXS) peaks corresponding to
low energy particle-hole excited states of metallic FeTe and semi-metallic
TiSe for photon incident energy tuned near the absorption edge of
Fe and Ti respectively. We show that the cross section amplitudes are well
described within a renormalization group theory where the effect of the core
electrons is captured by effective dielectric functions expressed in terms of
the the atomic scattering parameters of Fe and Ti. This method can be
used to extract the dynamical structure factor from experimental RIXS spectra
in metallic systems.Comment: 6 pages, 4 figure
Exchange Splitting and Charge Carrier Spin Polarization in EuO
High quality thin films of the ferromagnetic semiconductor EuO have been
prepared and were studied using a new form of spin-resolved spectroscopy. We
observed large changes in the electronic structure across the Curie and
metal-insulator transition temperature. We found that these are caused by the
exchange splitting of the conduction band in the ferromagnetic state, which is
as large as 0.6 eV. We also present strong evidence that the bottom of the
conduction band consists mainly of majority spins. This implies that doped
charge carriers in EuO are practically fully spin polarized.Comment: 4 pages, 5 figure
High-energy magnetic excitations in overdoped LaSrCuO studied by neutron and resonant inelastic X-ray scattering
We have performed neutron inelastic scattering and resonant inelastic X-ray
scattering (RIXS) at the Cu- edge to study high-energy magnetic
excitations at energy transfers of more than 100 meV for overdoped
LaSrCuO with ( K) and
(non-superconducting) using identical single crystal samples for the two
techniques. From constant-energy slices of neutron scattering cross-sections,
we have identified magnetic excitations up to ~250 meV for . Although
the width in the momentum direction is large, the peak positions along the (pi,
pi) direction agree with the dispersion relation of the spin-wave in the
non-doped LaCuO (LCO), which is consistent with the previous RIXS
results of cuprate superconductors. Using RIXS at the Cu- edge, we have
measured the dispersion relations of the so-called paramagnon mode along both
(pi, pi) and (pi, 0) directions. Although in both directions the neutron and
RIXS data connect with each other and the paramagnon along (pi, 0) agrees well
with the LCO spin-wave dispersion, the paramagnon in the (pi, pi) direction
probed by RIXS appears to be less dispersive and the excitation energy is lower
than the spin-wave of LCO near (pi/2, pi/2). Thus, our results indicate
consistency between neutron inelastic scattering and RIXS, and elucidate the
entire magnetic excitation in the (pi, pi) direction by the complementary use
of two probes. The polarization dependence of the RIXS profiles indicates that
appreciable charge excitations exist in the same energy range of magnetic
excitations, reflecting the itinerant character of the overdoped sample. A
possible anisotropy in the charge excitation intensity might explain the
apparent differences in the paramagnon dispersion in the (pi, pi) direction as
detected by the X-ray scattering.Comment: 7 pages, 7 figure
Combining immunotherapy and anticancer agents: the right path to achieve cancer cure?
This article summarizes the immune mediated effect of chemotherapies, the biological and clinical features of new immunotherapies like checkpoint blockers and the rational to use these treatment in combinatio
Surface-induced crystallization in supercooled tetrahedral liquids
Freezing is a fundamental physical phenomenon that has been studied over many
decades; yet the role played by surfaces in determining nucleation has remained
elusive. Here we report direct computational evidence of surface induced
nucleation in supercooled systems with a negative slope of their melting line
(dP/dT < 0). This unexpected result is related to the density decrease
occurring upon crystallization, and to surface tension facilitating the initial
nucleus formation. Our findings support the hypothesis of surface induced
crystallization of ice in the atmosphere, and provide insight, at the atomistic
level, into nucleation mechanisms of widely used semiconductors.Comment: 5 pages, 4 figure
Evidence of orbital reconstruction at interfaces in La0.67Sr0.33MnO3 films
Electronic properties of transition metal oxides at interfaces are influenced
by strain, electric polarization and oxygen diffusion. Linear dichroism (LD)
x-ray absorption, diffraction, transport and magnetization on thin
La0.7Sr0.3MnO3 films, allow identification of a peculiar universal interface
effect. We report the LD signature of preferential 3d-eg(3z2-r2) occupation at
the interface, suppressing the double exchange mechanism. This surface orbital
reconstruction is opposite of that favored by residual strain and independent
of dipolar fields, chemical nature of the substrate and capping.Comment: 13 pages, 5 figure
High-resolution resonant inelastic soft X-ray scattering as a probe of the crystal electrical field in lanthanides demonstrated for the case of CeRh2Si2
The magnetic properties of rare earth compounds are usually well captured by
assuming a fully localized f shell and only considering the Hund's rule ground
state multiplet split by a crystal electrical field (CEF). Currently, the
standard technique for probing CEF excitations in lanthanides is inelastic
neutron scattering. Here we show that with the recent leap in energy
resolution, resonant inelastic soft X-ray scattering has become a serious
alternative for looking at CEF excitations with some distinct advantages
compared to INS. As an example we study the CEF scheme in CeRh2Si2, a system
that has been intensely studied for more than two decades now but for which no
consensus has been reached yet as to its CEF scheme. We used two new features
that have only become available very recently in RIXS, high energy resolution
of about 30 meV as well as polarization analysis in the scattered beam, to find
a unique CEF description for CeRh2Si2. The result agrees well with previous INS
and magnetic susceptibility measurements. Due to its strong resonant character,
RIXS is applicable to very small samples, presents very high cross sections for
all lanthanides, and further benefits from the very weak coupling to phonon
excitation. The rapid progress in energy resolution of RIXS spectrometers is
making this technique increasingly attractive for the investigation of the CEF
scheme in lanthanides
Evolution of magnetic phases and orbital occupation in (SrMnO3)n/(LaMnO3)2n superlattices
The magnetic and electronic modifications induced at the interfaces in
(SrMnO)/(LaMnO) superlattices have been investigated
by linear and circular magnetic dichroism in the Mn L x-ray absorption
spectra. Together with theoretical calculations, our data demonstrate that the
charge redistribution across interfaces favors in-plane ferromagnetic (FM)
order and orbital occupation, in agreement with the
average strain. Far from interfaces, inside LaMnO, electron localization
and local strain favor antiferromagnetism (AFM) and
orbital occupation. For the high density of interfacial planes ultimately
leads to dominant FM order forcing the residual AFM phase to be in-plane too,
while for the FM layers are separated by AFM regions having
out-of-plane spin orientation.Comment: accepted for publication as a Rapid Communication in Physical Review
Multiple double-exchange mechanism by Mn-doping in manganite compounds
Double-exchange mechanisms in REAEMnO manganites (where
RE is a trivalent rare-earth ion and AE is a divalent alkali-earth ion) relies
on the strong exchange interaction between two Mn and Mn ions
through interfiling oxygen 2p states. Nevertheless, the role of RE and AE ions
has ever been considered "silent" with respect to the DE conducting mechanisms.
Here we show that a new path for DE-mechanism is indeed possible by partially
replacing the RE-AE elements by Mn-ions, in La-deficient
LaMnO thin films. X-ray absorption spectroscopy demonstrated
the relevant presence of Mn ions, which is unambiguously proved to be
substituted at La-site by Resonant Inelastic X-ray Scattering. Mn is
proved to be directly correlated to the enhanced magneto-transport properties
because of an additional hopping mechanism trough interfiling Mn-ions,
theoretically confirmed by calculations within the effective single band model.
The very idea to use Mn both as a doping element and an ions
electronically involved in the conduction mechanism, has never been foreseen,
revealing a new phenomena in transport properties of manganites. More
important, such a strategy might be also pursed in other strongly correlated
materials.Comment: 6 pages, 5 figure
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