541 research outputs found
Fission modes of mercury isotopes
Background: Recent experiments on beta-delayed fission in the mercury-lead
region and the discovery of asym- metric fission in 180 Hg [1] have stimulated
theoretical interest in the mechanism of fission in heavy nuclei. Purpose: We
study fission modes and fusion valleys in 180 Hg and 198 Hg to reveal the role
of shell effects in pre-scission region and explain the experimentally observed
fragment mass asymmetry and its variation with A. Methods: We use the
self-consistent nuclear density functional theory employing Skyrme and Gogny
energy density functionals. Results: The potential energy surfaces in
multi-dimensional space of collective coordinates, including elongation,
triaxiality, reflection-asymmetry, and necking, are calculated for 180 Hg and
198 Hg. The asymmetric fission valleys - well separated from fusion valleys
associated with nearly spherical fragments - are found in in both cases. The
density distributions at scission configurations are studied and related to the
experimentally observed mass splits. Conclusions: The energy density
functionals SkM\ast and D1S give a very consistent description of the fission
process in 180 Hg and 198 Hg. We predict a transition from asymmetric fission
in 180 Hg towards more symmetric distribution of fission fragments in 198 Hg.
For 180 Hg, both models yield 100 Ru/80 Kr as the most probable split. For 198
Hg, the most likely split is 108 Ru/90 Kr in HFB-D1S and 110 Ru/88 Kr in
HFB-SkM\ast.Comment: 6 pages, 5 figures, to be published in Physical Review
The contrasting fission potential-energy structure of actinides and mercury isotopes
Fission-fragment mass distributions are asymmetric in fission of typical
actinide nuclei for nucleon number in the range
and proton number in the range . For somewhat
lighter systems it has been observed that fission mass distributions are
usually symmetric. However, a recent experiment showed that fission of
Hg following electron capture on Tl is asymmetric. We calculate
potential-energy surfaces for a typical actinide nucleus and for 12 even
isotopes in the range Hg--Hg, to investigate the similarities
and differences of actinide compared to mercury potential surfaces and to what
extent fission-fragment properties, in particular shell structure, relate to
the structure of the static potential-energy surfaces. Potential-energy
surfaces are calculated in the macroscopic-microscopic approach as functions of
fiveshape coordinates for more than five million shapes. The structure of the
surfaces are investigated by use of an immersion technique. We determine
properties of minima, saddle points, valleys, and ridges between valleys in the
5D shape-coordinate space. Along the mercury isotope chain the barrier heights
and the ridge heights and persistence with elongation vary significantly and
show no obvious connection to possible fragment shell structure, in contrast to
the actinide region, where there is a deep asymmetric valley extending from the
saddle point to scission. The mechanism of asymmetric fission must be very
different in the lighter proton-rich mercury isotopes compared to the actinide
region and is apparently unrelated to fragment shell structure. Isotopes
lighter than Hg have the saddle point blocked from a deep symmetric
valley by a significant ridge. The ridge vanishes for the heavier Hg isotopes,
for which we would expect a qualitatively different asymmetry of the fragments.Comment: 8 pages, 9 figure
Mass distributions for induced fission of different Hg isotopes
With the improved scission-point model the mass distributions are calculated
for induced fission of different Hg isotopes with the masses 180-196. The
drastic change in the shape of the mass distribution from asymmetric to
symmetric is revealed with increasing mass number of the fissioning Hg isotope,
and the reactions are proposed to verify this prediction experimentally. The
asymmetric mass distribution of fission fragments observed in the recent
experiment on the fission of 180Hg is explained. The calculated mass
distribution and mean total kinetic energy of fission fragments are in a good
agreement with the available experimental data
Sharp change over from compound nuclear fission to shape dependent quasi fission
Fission fragment mass distribution has been measured from the decay of
Bk nucleus populating via two entrance channels with slight difference
in mass asymmetries but belonging on either side of the Businaro Gallone mass
asymmetry parameter. Both the target nuclei were deformed. Near the Coulomb
barrier, at similar excitation energies the width of the fission fragment mass
distribution was found to be drastically different for the N +
Th reaction compared to the B + U reaction. The entrance
channel mass asymmetry was found to affect the fusion process sharply.Comment: 4 pages,6 figure
Non-Markovian large amplitude motion and nuclear fission
The general problem of dissipation in macroscopic large-amplitude collective
motion and its relation to energy diffusion of intrinsic degrees of freedom of
a nucleus is studied. By applying the cranking approach to the nuclear many
body system, a set of coupled dynamical equations for the collective classical
variables and the quantum mechanical occupancies of the intrinsic nuclear
states is derived. Different dynamical regimes of the intrinsic nuclear motion
and its consequences on time properties of collective dissipation are
discussed. The approach is applied to the descant of the nucleus from the
fission barrier.Comment: 9 pages and 3 figure
Investigation of the quasifission process by theoretical analysis of experimental data of fissionlike reaction products
The fusion excitation function is the important quantity in planning
experiments for the synthesis of superheavy elements. Its values seem to be
determined by the experimental study of the hindrance to complete fusion by the
observation of mass, angular and energy distributions of the fissionlike
fragments. There is ambiguity in establishment of the reaction mechanism
leading to the observed binary fissionlike fragments. The fissionlike fragments
can be produced in the quasifission, fast fission, and fusion-fission processes
which have overlapping in the mass (angular, kinetic energy) distributions of
fragments. The branching ratio between quasifission and complete fusion
strongly depends on the characteristics of the entrance channel. In this paper
we consider a wide set of reactions (with different mass asymmetry and mass
symmetry parameters) with the aim to explain the role played by many quantities
on the reaction mechanisms. We also present the results of study of the
Ca+Bk reaction used to synthesize superheavy nuclei with Z = 117
by the determination of the evaporation residue cross sections and the
effective fission barriers of excited nuclei formed along the
de-excitation cascade of the compound nucleus.Comment: 21 pages, 15 figures, 2 table
Sub-barrier capture with quantum diffusion approach: actinide-based reactions
With the quantum diffusion approach the behavior of capture cross sections
and mean-square angular momenta of captured systems are revealed in the
reactions with deformed nuclei at subbarrier energies. The calculated results
are in a good agreement with existing experimental data. With decreasing
bombarding energy under the barrier the external turning point of the
nucleusnucleus potential leaves the region of short-range nuclear interaction
and action of friction. Because of this change of the regime of interaction, an
unexpected enhancement of the capture cross section is expected at bombarding
energies far below the Coulomb barrier. This effect is shown its worth in the
dependence of mean-square angular momentum of captured system on the bombarding
energy. From the comparison of calculated and experimental capture cross
sections, the importance of quasifission near the entrance channel is shown for
the actinide-based reactions leading to superheavy nuclei.Comment: 11 pages, 16 figures, Regular Articl
Angular anisotropy of the fusion-fission and quasifission fragments
The anisotropy in the angular distribution of the fusion-fission and
quasifission fragments for the O+U, F+Pb and
S+Pb reactions is studied by analyzing the angular momentum
distributions of the dinuclear system and compound nucleus which are formed
after capture and complete fusion, respectively. The orientation angles of
axial symmetry axes of colliding nuclei to the beam direction are taken into
account for the calculation of the variance of the projection of the total spin
onto the fission axis. It is shown that the deviation of the experimental
angular anisotropy from the statistical model picture is connected with the
contribution of the quasifission fragments which is dominant in the
S+Pb reaction. Enhancement of anisotropy at low energies in the
O+U reaction is connected with quasifission of the dinuclear
system having low temperature and effective moment of inertia.Comment: 17 pages 8 figures. Submitted to Euro. Phys. Jour.
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