54 research outputs found
Electronic Raman scattering in Tl2Ba2CuO6+x: symmetry of the order parameter, oxygen doping effects, and normal state scattering
Single crystals of the optimally doped, moderately and strongly overdoped
high temperature superconductor Tl2Ba2CuO6+x (Tl-2201) with Tc=80, 56 and 30K,
respectively, have been investigated by polarized Raman scattering. By taking
the peak position of the B_1g component of electronic Raman scattering as
2Delta_0 we found that the reduced gap value (2Delta_0/k_BT_c) strongly
decreases with increasing doping. The behavior of the low frequency scattering
for the B_1g and B_2g scattering components is similar for optimally doped and
overdoped crystals and can be described by a w^3 - and w -law, respectively,
which is consistent with a d-wave symmetry of the order parameter. In contrast
to the optimally doped Tl-2201 in both, moderately and strongly overdoped
Tl-2201, the relative (compared to the B_1g) intensity of the A_1g scattering
component is suppressed. We suggest that the van Hove singularity is
responsible for the observed changes of Raman intensity and reduced gap value
with doping. Electronic Raman scattering in the normal state is discussed in
the context of the scattering from impurities and compared to the existing
infrared data. The scattering rate evaluated from the Raman measurements is
smaller for the overdoped samples, compared to the moderately overdoped
samples.Comment: 7 pages, 7 figure
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SPIN POLARIZED PHOTOELECTRON SPECTROSCOPY AS A PROBE OF MAGNETIC SYSTEMS.
Spin-polarized photoelectron spectroscopy has developed into a versatile tool for the study of surface and thin film magnetism. In this chapter, we examine the methodology of the technique and its recent application to a number of different problems. We first examine the photoemission process itself followed by a detailed review of spin-polarization measurement techniques and the related experimental requirements. We review studies of spin polarized surface states, interface states and quantum well states followed by studies of the technologically important oxide systems including half-metallic transition metal oxides, ferromagnet/oxide interfaces and the antiferromagnetic cuprates that exhibit high Tc Superconductivity. We also discuss the application of high-resolution photoemission with spin resolving capabilities to the study of spin dependent self energy effects
Perpendicular exchange bias in antiferromagnetic-ferromagnetic nanostructures
This article may be downloaded for personal use only. Any other use requires prior permission of the author and the American Institute of Physics.Exchange bias effects have been induced along the perpendicular-to-film direction in nanostructures prepared by electron beamlithography, consisting of a ferromagnetic [Pt/Co] multilayer exchange coupled to an antiferromagnet (FeMn). As a general trend, the exchange bias field and the blocking temperature decrease, whereas the coercivity increases, as the size of the nanostructures is reduced
Inhomogeneity of the intrinsic magnetic field in superconducting YBa2Cu3OX compounds as revealed by rare-earth EPR-probe
X-band electron paramagnetic resonance on doped Er3+ and Yb3+ ions in
Y0.99(Yb,Er)0.01Ba2Cu3OX compounds with different oxygen contents in the wide
temperature range (4-120)K have been made. In the superconducting species, the
strong dependencies of the linewidth and resonance line position from the sweep
direction of the applied magnetic field are revealed at the temperatures
significantly below TC. The possible origins of the observed hysteresis are
analyzed. Applicability of the presented EPR approach to extract information
about the dynamics of the flux-line lattice and critical state parameters
(critical current density, magnetic penetration depth, and characteristic
spatial scale of the inhomogeneity) is discussedComment: 17 pages, 5 Figures. Renewed versio
Complex ferromagnetic state and magnetocaloric effect in single crystalline Nd_{0.7}Sr_{0.3}MnO_{3}
The magnetocaloric effect in single crystalline Nd_{0.7}Sr_{0.3}MnO_{3} is
investigated by measuring the field-induced adiabatic change in temperature
which reveals a single negative peak around 130 K well below the Curie
temperature (T_C=203 K). In order to understand this unusual magnetocaloric
effect, we invoke the reported {55}^Mn spin-echo nuclear magnetic resonance,
electron magnetic resonance and polarized Raman scattering measurements on
Nd_{0.7}Sr_{0.3}MnO_{3}. We show that this effect is a manifestation of a
competition between the double exchange mechanism and correlations arising from
coupled spin and lattice degrees of freedom which results in a complex
ferromagnetic state. The critical behavior of Nd_{0.7}Sr_{0.3}MnO_{3} near
Curie temperature is investigated to study the influence of the coupled degrees
of freedom. We find a complicated behavior at low fields in which the order of
the transition could not be fixed and a second-order-like behavior at high
fields.Comment: Accepted for publication in Phys. Rev.
Influence of Co spin-state on optical properties of LaCoO and HoCoO
Optical properties of the isoelectronic compounds LaCoO and HoCoO has
been experimentally and theoretically investigated. We've measured the real
and imaginary parts of the dielectric
function, reflectance and optical conductivity at room temperature.
The shift of the most pronounced spectral features to the high energy region on
0.3 eV associated with larger distortions due to the smaller rare earth ionic
radii in HoCoO in comparison with LaCoO was observed. Also there was
found an enhancement of absorption intensity in the range 1.3-2.3 eV in all
kinds of spectra in HoCoO, which can be attributed basing on the results of
LDA+U calculations to the different spin-states of Co ion in these
compounds. The shift of the onset of the absorption from less than 0.1 eV in
LaCoO to 0.7 eV in HoCoO and an absorption intensity enhancement in a
narrow spectral range 1.2-2.6 eV in HoCoO are clearly seen from the
calculated convolution of partial densities of states obtained in the LDA+U
approach. Such changes are assumed to be induced by the different Co
spin-state in these compounds at room temperature.Comment: 10 pages, 3 figure
Phonon Raman scattering in LaMn₁₋xCoxO₃ (x = 0, 0.2, 0.3, 0.4, and 1.0)
The Raman-active phonons in perovskite-like LaMn₁–xCoxO₃ (x = 0, 0.2, 0.3, 0.4, and 1.0) were studied by measuring Raman spectra at temperatures of 295 and 5 K. The changes in the spectra with Co doping are correlated with the decrease of orthorhombic distortions. Surprisingly more phonon lines than allowed for the rhombohedral LaCoO₃ structure were observed
Composite fluoropolymer piezoelectric membranes for reconstructive recovery surgery
In the present study, we performed the results of studies on the formation of composite fluoropolymer piezoelectric membranes based on a copolymer of vinylidene fluoride with tetrafluoroethylene (VDF-TeFE) and polyethylpyrrolidone (PEP) by the electrospinning method. Using scanning electron microscopy, the effect of the PEP content on the structure of the formed membranes was studied. The biocompatibility of the obtained membranes was studied by fluorescence microscopy on a model of human skin fibroblasts. The studied samples with a PEP content of 0, 5, and 15% have good adhesive characteristics, preserve the viability and potential of cells to divide, and therefore are most suitable for further use in regenerative medicine
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