629 research outputs found
Core excitations across the neutron shell gap in ÂČâ°â·Tl
The single closed-neutron-shell, one proton-hole nucleus 207Tl was populated in deep-inelastic collisions of a 208Pb beam with a 208Pb target. The yrast and near-yrast level scheme has been established up to high excitation energy, comprising an octupol
Large scale shell model calculations for odd-odd Mn isotopes
Large scale shell model calculations have been carried out for odd-odd
Mn isotopes in two different model spaces. First set of calculations
have been carried out in full shell valence space with two recently
derived shell interactions namely GXPF1A and KB3G treating Ca
as core. The second set of calculations have been performed in
valence space with the interaction treating Ca as core and
imposing a truncation by allowing up to a total of six particle excitations
from the 0f orbital to the upper orbitals for protons and
from the upper orbitals to the 0g orbital for neutron. For
low-lying states in Mn, the KB3G and GXPF1A both predicts good results
and for Mn, KB3G is much better than GXPF1A. For negative parity and
high-spin positive parity states in both isotopes interaction is
required. Experimental data on Mn is sparse and therefore it is not
possible to make any definite conclusions. More experimental data on negative
parity states is needed to ascertain the importance of 0g and higher
orbitals in neutron rich Mn isotopes.Comment: 5 pages, 4 figures, Submitted to Eur. Phys. J.
Highly deformed Ca configurations in Si + C
The possible occurrence of highly deformed configurations in the Ca
di-nuclear system formed in the Si + C reaction is investigated
by analyzing the spectra of emitted light charged particles. Both inclusive and
exclusive measurements of the heavy fragments (A 10) and their
associated light charged particles (protons and particles) have been
made at the IReS Strasbourg {\sc VIVITRON} Tandem facility at bombarding
energies of Si) = 112 MeV and 180 MeV by using the {\sc ICARE}
charged particle multidetector array. The energy spectra, velocity
distributions, and both in-plane and out-of-plane angular correlations of light
charged particles are compared to statistical-model calculations using a
consistent set of parameters with spin-dependent level densities. The analysis
suggests the onset of large nuclear deformation in Ca at high spin.Comment: 33 pages, 11 figure
Quantitative hopanoid analysis enables robust pattern detection and comparison between laboratories
Hopanoids are steroid-like lipids from the isoprenoid family that are produced primarily by bacteria. Hopanes, molecular fossils of hopanoids, offer the potential to provide insight into environmental transitions on the early Earth, if their sources and biological functions can be constrained. Semiquantitative methods for mass spectrometric analysis of hopanoids from cultures and environmental samples have been developed in the last two decades. However, the structural diversity of hopanoids, and possible variability in their ionization efficiencies on different instruments, have thus far precluded robust quantification and hindered comparison of results between laboratories. These ionization inconsistencies give rise to the need to calibrate individual instruments with purified hopanoids to reliably quantify hopanoids. Here, we present new approaches to obtain both purified and synthetic quantification standards. We optimized 2-methylhopanoid production in Rhodopseudomonas palustris TIE-1 and purified 2Me-diplopterol, 2Me-bacteriohopanetetrol (2Me-BHT), and their unmethylated species (diplopterol and BHT). We found that 2-methylation decreases the signal intensity of diplopterol between 2 and 34% depending on the instrument used to detect it, but decreases the BHT signal less than 5%. In addition, 2Me-diplopterol produces 10Ă higher ion counts than equivalent quantities of 2Me-BHT. Similar deviations were also observed using a flame ionization detector for signal quantification in GC. In LC-MS, however, 2Me-BHT produces 11Ă higher ion counts than 2Me-diplopterol but only 1.2Ă higher ion counts than the sterol standard pregnane acetate. To further improve quantification, we synthesized tetradeuterated (D_4) diplopterol, a precursor for a variety of hopanoids. LC-MS analysis on a mixture of (D4)-diplopterol and phospholipids showed that under the influence of co-eluted phospholipids, the D_4-diplopterol internal standard quantifies diplopterol more accurately than external diplopterol standards. These new quantitative approaches permit meaningful comparisons between studies, allowing more accurate hopanoid pattern detection in both laboratory and environmental samples
Cross-shell excitation in two-proton knockout: Structure of Ca
The two-proton knockout reaction Be(Ti,Ca) has
been studied at 72 MeV/nucleon. Besides the strong feeding of the Ca
ground state, the only other sizeable cross section proceeds to a 3 level
at 3.9 MeV. There is no measurable direct yield to the first excited 2
state at 2.6 MeV. The results illustrate the potential of such direct reactions
for exploring cross-shell proton excitations in neutron-rich nuclei and
confirms the doubly-magic nature of Ca
Octupole transitions in the 208Pb region
The 208Pb region is characterised by the existence of collective octupole states.
Here we populated such states in 208Pb + 208Pb deep-inelastic reactions. Îł-ray angular
distribution measurements were used to infer the octupole character of several E3 transitions.
The octupole character of the 2318 keV 17â â 14+ in 208Pb, 2485 keV 19/2
â â 13/2
+ in
207Pb, 2419 keV 15/2
â â 9/2
+ in 209Pb and 2465 keV 17/2
+ â 11/2
â in 207Tl transitions was
demonstrated for the first time. In addition, shell model calculations were performed using two
different sets of two-body matrix elements. Their predictions were compared with emphasis on
collective octupole states.This work is supported by the Science and Technology Facilities Council
(STFC), UK, US Department of Energy, Office of Nuclear Physics, under Contract No. DEAC02-06CH11357
and DE-FG02-94ER40834, NSF grant PHY-1404442
Extended Hauser-Feshbach Method for Statistical Binary-Decay of Light-Mass Systems
An Extended Hauser-Feshbach Method (EHFM) is developed for light heavy-ion
fusion reactions in order to provide a detailed analysis of all the possible
decay channels by including explicitly the fusion-fission phase-space in the
description of the cascade chain. The mass-asymmetric fission component is
considered as a complex-fragment binary-decay which can be treated in the same
way as the light-particle evaporation from the compound nucleus in
statistical-model calculations. The method of the phase-space integrations for
the binary-decay is an extension of the usual Hauser-Feshbach formalism to be
applied to the mass-symmetric fission part. The EHFM calculations include
ground-state binding energies and discrete levels in the low excitation-energy
regions which are essential for an accurate evaluation of the phase-space
integrations of the complex-fragment emission (fission). In the present
calculations, EHFM is applied to the first-chance binary-decay by assuming that
the second-chance fission decay is negligible. In a similar manner to the
description of the fusion-evaporation process, the usual cascade calculation of
light-particle emission from the highly excited complex fragments is applied.
This complete calculation is then defined as EHFM+CASCADE. Calculated
quantities such as charge-, mass- and kinetic-energy distributions are compared
with inclusive and/or exclusive data for the S+Mg and
Cl+C reactions which have been selected as typical examples.
Finally, the missing charge distributions extracted from exclusive measurements
are also successfully compared with the EHFM+CASCADE predictions.Comment: 34 pages, 6 Figures available upon request, Phys. Rev. C (to be
published
Contrasting properties of particle-particle and hole-hole excitations in 206Tl and 210Bi nuclei
A complete-spectroscopy investigation of low-lying, low-spin states in the one-proton-hole and one-neutron-hole nucleus 206Tl has been performed by using thermal neutron capture and \u3b3-coincidence technique with the FIPPS Ge array at ILL Grenoble. The new experimental results, together with data for the one-proton-particle and one-neutron-particle nucleus 210Bi (taken from a previous study done at ILL in the EXILL campaign), allowed for an extensive comparison with predictions of shell-model calculations performed with realistic interactions. No phenomenological adjustments were introduced in the calculations. In 210Bi, state energies, transition multipolarities and decay branchings agree well with theory for the three well separated multiplets of states which dominate the low-lying excitations. On the contrary, in 206Tl significant discrepancies are observed: in the same energy region, six multiplets were identified, with a significant mixing among them being predicted, as a consequence of the smaller energy separation between the active orbitals. The discrepancies in 206Tl are attributed to the larger uncertainties in the determination of the off-diagonal matrix elements of the realistic shell-model interaction with respect to the calculated diagonal matrix elements, the only ones playing a major role in the case of 210Bi. The work points to the need of more advanced approaches in the construction of the realistic interactions
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