Magnetic Properties of the RAuBi2 (R = Ce, Pr, Nd, Gd, Sm) Series of Intermetallic Compounds

AbstractIn this work we report the physical properties of the series of intermetallic compounds RAuBi2 (R = Ce, Pr, Nd, Gd, Sm) studied by means of x-ray powder diffraction, magnetic susceptibility, heat capacity and electrical resistivity measurements. These compounds were grown using the metallic Bi self-flux technique and they crystallize in a tetragonal ZrCuSi2 (P4/nmm) structure. Our RAuBi2 single crystals show an antiferromagnetic ordering TN ≥ 2.3K for all measured compounds. The values of TN show a dramatic breakdown of the De Gennes factor along this series

Evolution From Insulator (x=0.003) To Metal (x=1) Of The Eu 2+ Local Environment In Ca 1-xeu Xb 6

The local environment of Eu2+ (4 f7, S=72) in Ca1-x Eux B6 (0.003≤x≤1.00) is studied by means of electron spin resonance (ESR). For x≲0.07 the resonances have Lorentzian line shape, indicating an insulating environment for the Eu2+ ions. For x≳0.07, the lines broaden and become Dysonian in shape, suggesting a change to metallic environment for the Eu2+ ions, anticipating the semimetallic character of EuB6. The broadening is attributed to a spin-flip scattering relaxation process due to the exchange interaction between conduction and Eu2+ 4f electrons. High field ESR measurements for x≳0.30 reveal narrower and anisotropic linewidths, which are attributed to magnetic polarons and Fermi surface effects, respectively. © 2005 American Institute of Physics.9710Young, D.P., (1999) Nature (London), 397, p. 412Zhitomirsky, M.E., (1999) Nature (London), 402, p. 251Tromp, H.J., (2000) Phys. Rev. Lett., 87, p. 016401Massidda, S., Continenza, A., De Pascale, T.M., Monnier, R., (1997) Z. Phys. B: Condens. Matter, 102, p. 83Urbano, R.R., (2002) Phys. Rev. B, 65, p. 180407Bennett, M.C., (2004) Phys. Rev. B, 69, p. 132407Urbano, R.R., Pagliuso, P.G., Rettori, C., Oseroff, S.B., Sarrao, J.L., Schlottmann, P., Fisk, Z., (2004) Phys. Rev. B, 70, p. 140401Pake, G.E., Purcell, E.M., (1948) Phys. Rev., 74, p. 1184Bloembergen, N., (1952) J. Appl. Phys., 23, p. 1383Feher, G., Kip, A.F., (1955) Phys. Rev., 98, p. 337Dyson, F.J., (1955) Phys. Rev., 98, p. 349Sperlich, G., Jansen, K., (1974) Solid State Commun., 15, p. 1105Essam, J.W., (1972) Phase Transitions and Critical Phenomena, 2, p. 197. , Academic, LondonSchlottmann, P., Hellberg, C.S., (1996) J. Appl. Phys., 79, p. 6414Fisk, Z., (1979) J. Appl. Phys., 50, p. 1911Goodrich, R.G., Harrison, N., Vuillemin, J.J., Tekul, A., Hall, D.W., Fisk, Z., Young, D., Sarrao, J., (1998) Phys. Rev. B, 58, p. 14896Rhyee, J.-S., Cho, B.K., Ri, H.-C., (2003) Phys. Rev. B, 67, p. 125102Wigger, G.A., Beeli, C., Felder, E., Ott, H.R., Bianchi, A.D., Fisk, Z., (2004) Phys. Rev. Lett., 93, p. 14720

Quantum Critical Kondo Quasiparticles Probed By Esr In β-ybalb 4

Electron spin resonance (ESR) can probe conduction electrons (CE) and local moment (LM) spin systems in different materials. A CE spin resonance (CESR) is observed in metallic systems based on light elements or with enhanced Pauli susceptibility. LM ESR can be seen in compounds with paramagnetic ions and localized d or f electrons. Here we report a remarkable and unprecedented ESR signal in the heavy-fermion superconductor β-YbAlB4 which behaves as a CESR at high temperatures and acquires characteristics of the Yb3 LM ESR at low temperature. This dual behavior strikes as an in situ unique observation of the Kondo quasiparticles in a quantum critical regime. The proximity to a quantum critical point may favor the appearance of this dual character of the ESR signal in β-YbAlB4. © 2011 American Physical Society.1072Tien, C., Yu, J., Duh, H., (1993) Jpn. J. Appl. Phys., 32, p. 2658. , JAPNDE 0021-4922 10.1143/JJAP.32.2658Sichelschmidt, J., (2003) Phys. Rev. Lett., 91, p. 156401. , PRLTAO 0031-9007 10.1103/PhysRevLett.91.156401Sichelschmidt, J., (2007) J. Phys. Condens. Matter, 19, p. 016211. , JCOMEL 0953-8984 10.1088/0953-8984/19/1/016211Krellner, C., Forster, T., Jeevan, H., Geibel, C., Sichelschmidt, J., Relevance of ferromagnetic correlations for the electron spin resonance in kondo lattice systems (2008) Physical Review Letters, 100 (6), p. 066401. , http://oai.aps.org/oai?verb=GetRecord&Identifier=oai:aps.org: PhysRevLett.100.066401&metadataPrefix=oai_apsmeta_2, DOI 10.1103/PhysRevLett.100.066401Abrahams, E., Wolfle, P., (2008) Phys. Rev. B, 78, p. 104423. , PRBMDO 1098-0121 10.1103/PhysRevB.78.104423Schlottmann, P., (2009) Phys. Rev. B, 79, p. 045104. , PRBMDO 1098-0121 10.1103/PhysRevB.79.045104Macaluso, R.T., Nakatsuji, S., Kuga, K., Thomas, E.L., Machida, Y., Maeno, Y., Fisk, Z., Chan, J.Y., Crystal structure and physical properties of polymorphs of LnAlB 4 (Ln = Yb, Lu) (2007) Chemistry of Materials, 19 (8), pp. 1918-1922. , DOI 10.1021/cm062244+Nakatsuji, S., (2008) Nature Phys., 4, p. 603. , NPAHAX 1745-2473 10.1038/nphys1002Duque, J.G.S., (2009) Phys. Rev. B, 79, p. 035122. , PRBMDO 1098-0121 10.1103/PhysRevB.79.035122Trovarelli, O., (2000) Phys. Rev. Lett., 85, p. 626. , PRLTAO 0031-9007 10.1103/PhysRevLett.85.626Gegenwart, P., (2002) Phys. Rev. Lett., 89, p. 056402. , PRLTAO 0031-9007 10.1103/PhysRevLett.89.056402Dyson, F.J., (1955) Phys. Rev., 98, p. 349. , PHRVAO 0031-899X 10.1103/PhysRev.98.349Tao, L.J., (1971) Phys. Rev. B, 4, p. 5. , PRBMDO 0556-2805 10.1103/PhysRevB.4.5Abragam, A., Bleaney, B., (1970) EPR of Transitions Ions, , Clarendon, OxfordSattler, J.P., Nemarich, J., (1970) Phys. Rev. B, 1, p. 4249. , PRBMDO 0556-2805 10.1103/PhysRevB.1.4249Rettori, C., (1981) Physica (Amsterdam), 107, p. 359. , PHYBE3 0378-4363 10.1016/0378-4363(81)90485-XHuber, D.L., (2004) Phys. Rev. B, 70, p. 125417. , PRBMDO 1098-0121 10.1103/PhysRevB.70.125417Oseroff, S.B., (1977) Phys. Rev. B, 15, p. 1283. , PRBMDO 0556-2805 10.1103/PhysRevB.15.1283Continetino, M., (2005) Braz. J. Phys., 35, p. 197. , BJPHE6 0103-9733 10.1590/S0103-97332005000100018Coleman, P., Pepin, C., Si, Q., Ramazashvili, R., How do Fermi liquids get heavy and die? (2001) Journal of Physics Condensed Matter, 13 (35), pp. R723-R738. , DOI 10.1088/0953-8984/13/35/202, PII S095389840124853XMonod, P., (1978) J. Phys. (Paris), 39, pp. 6-1472. , JOPQAG 0302-0738 10.1051/jphyscol:19786589Rettori, C., (1997) Phys. Rev. B, 55, p. 1016. , PRBMDO 0163-1829 10.1103/PhysRevB.55.1016Pagliuso, P.G., (1997) Phys. Rev. B, 56, p. 8933. , PRBMDO 0163-1829 10.1103/PhysRevB.56.8933Urbano, R.R., (2002) Phys. Rev. Lett., 89, p. 087602. , PRLTAO 0031-9007 10.1103/PhysRevLett.89.087602Likodimos, V., Koutandos, S., Pissas, M., Papavassiliou, G., Prassides, K., Conduction electron spin resonance in Mg1-xAl xB2 (2003) Europhysics Letters, 61 (1), pp. 116-121. , DOI 10.1209/epl/i2003-00257-1Sercheli, M.S., Kopelevich, Y., Ricardo Da Silva, R., Torres, J.H.S., Rettori, C., Evidence for internal field in graphite: A conduction electron spin-resonance study (2002) Solid State Communications, 121 (9-10), pp. 579-583. , DOI 10.1016/S0038-1098(01)00465-3, PII S0038109801004653Walmsley, L., Rettori, C., C-Axis resistivity in graphite-AlCl3 as found by CESR measurements (1990) Synthetic Metals, 36 (2), pp. 235-239. , DOI 10.1016/0379-6779(90)90056-QPfluger, P., (1983) Synth. Met., 8, p. 15. , SYMEDZ 0379-6779 10.1016/0379-6779(83)90004-8Nevidomskyy, A.H., Coleman, P., (2009) Phys. Rev. Lett., 102, p. 077202. , PRLTAO 0031-9007 10.1103/PhysRevLett.102.077202Si, Q., Rabello, S., Ingersent, K., Smith, J.L., Locally critical quantum phase transitions in strongly correlated metals (2001) Nature, 413 (6858), pp. 804-808. , DOI 10.1038/3510150

Pseudogap Formation in the Symmetric Anderson Lattice Model

We present self-consistent calculations for the self-energy and magnetic susceptibility of the 2D and 3D symmetric Anderson lattice Hamiltonian, in the fluctuation exchange approximation. At high temperatures, strong f-electron scattering leads to broad quasiparticle spectral functions, a reduced quasiparticle band gap, and a metallic density of states. As the temperature is lowered, the spectral functions narrow and a pseudogap forms at the characteristic temperature $T_x$ at which the width of the quasiparticle spectral function at the gap edge is comparable to the renormalized activation energy. For $T << T_x$, the pseudogap is approximately equal to the hybridization gap in the bare band structure. The opening of the pseudogap is clearly apparent in both the spin susceptibility and the compressibility.Comment: RevTeX - 14 pages and 7 figures (available on request), NRL-JA-6690-94-002

Noncubic Symmetry In Ca 1-xeu Xb 6 (0.15≲x≤1.00): An Electron-spin-resonance Study

The Eu2+ (4 f7, S=72) g value in Ca1-x Eux B6 (0.15≲x≤1.00) was measured by means of electron spin resonance at two frequencies (fields), 9.4 (≈3.4 kOe) and 34.4 GHz (≈12.1 kOe). The g value was found to be anisotropic and magnetic-field dependent. The amplitude of the anisotropy increases at low temperatures. The observed angular and temperature dependences of the g value suggest tetragonal symmetry caused, presumably, by a distortion along a direction perpendicular to the largest crystal face, the [001] direction. Due to the platelet shape of the samples, part of the anisotropy of the g value can also be attributed to demagnetization effects. The g values decrease at higher fields, which is interpreted in terms of a two-band model involving an exchange interaction between the localized Eu2+ 4 f7 electrons with conduction Eu2+ 5d -like electrons and B 2p -like holes. © 2006 American Institute of Physics.998Etourneau, J., Hagenmuller, P., (1985) Philos. Mag. B, 52, p. 589Young, D.P., (1999) Nature (London), 397, p. 412Zhitomirsky, M.E., Rice, T.M., Anisimov, V.I., (1999) Nature (London), 402, p. 251Degiorgi, L., Felder, E., Ott, H.R., Sarrao, J.L., Fisk, Z., (1997) Phys. Rev. Lett., 79, p. 5134Massidda, S., Continenza, A., De Pascale, T.M., Monnier, R., (1997) Z. Phys. B: Condens. Matter, 102, p. 83Süllow, S., (1998) Phys. Rev. B, 57, p. 5860Booth, C.H., Sarrao, J.L., Hundley, M.F., Cornelius, A.L., Kwei, G.H., Bianchi, A., Fisk, Z., Lawrence, J.M., (2001) Phys. Rev. B, 63, p. 224302Paschen, S., Pushim, D., Schlatter, M., Vonlanthen, P., Ott, H.R., Young, D.P., Fisk, Z., (2000) Phys. Rev. B, 61, p. 4174Wigger, G.A., Walti, Ch., Ott, H.R., Bianchi, A.D., Fisk, Z., (2002) Phys. Rev. B, 66, p. 212410Wigger, G.A., Beeli, C., Felder, E., Ott, H.R., Bianchi, A.D., Fisk, Z., (2004) Phys. Rev. Lett., 93, p. 147203Uimin, G., (1997) Phys. Rev. B, 55, p. 8267Sturm, H., Elschner, B., Hock, K.-H., (1985) Phys. Rev. Lett., 54, p. 1291Altshuler, T.S., Bresler, M.S., (1999) J. Exp. Theor. Phys., 88, p. 1019Süllow, S., Prasad, I., Aronson, M.C., Bogdanovich, S., Sarrao, J.L., Fisk, Z., (2000) Phys. Rev. B, 62, p. 11626Urbano, R.R., Pagliuso, P.G., Rettori, C., Oseroff, S.B., Sarrao, J.L., Schlottmann, P., Fisk, Z., (2004) Phys. Rev. B, 70, p. 140401Urbano, R.R., (2005) Phys. Rev. B, 71, p. 184422Feher, G., Kip, A.F., (1955) Phys. Rev., 98, p. 337. , 0031-899X 10.1103/PhysRev.98.337Dyson, F.J., (1955) Phys. Rev., 98, p. 349. , 0031-899X 10.1103/PhysRev.98.349Pake, G.E., Purcell, E.M., (1948) Phys. Rev., 74, p. 1184Abragam, A., Bleaney, B., (1970) EPR of Transition Ions, , Clarendon, OxfordKunii, S., Uemura, T., Chiba, Y., Kasuya, T., Date, M., (1985) J. Magn. Magn. Mater., 52, p. 271. , 0304-8853 10.1016/0304-8853(85)90277-XKunii, S., (2000) J. Phys. Soc. Jpn., 69, p. 3789Bisch, P.M., Troper, A., Gomes, A.A., (1976) Phys. Rev. B, 13, p. 3902. , 0556-2805 10.1103/PhysRevB.13.3902Troper, A., De Menezes, O.L.T., Lederer, P., Gomes, A.A., (1978) Phys. Rev. B, 18, p. 3709. , 0556-2805 10.1103/PhysRevB.18.3709Barberis, G.E., Davidov, D., Donoso, J.P., Rettori, C., Suassuna, J.F., Dokter, H.D., (1979) Phys. Rev. B, 19, p. 5495. , 0163-1829 10.1103/PhysRevB.19.5495Pagliuso, P.G., Rettori, C., Sarrao, J.L., Cornelius, A., Hundley, M.F., Fisk, Z., Oseroff, S.B., (1999) Phys. Rev. B, 60, p. 13515Calderón, M.J., Wegener, L.G.L., Littlewood, P.B., (2004) Phys. Rev. B, 70, p. 092404Davidov, D., Maki, K., Orbach, R., Rettori, C., Chock, E.P., (1973) Solid State Commun., 12, p. 62

Probing The Electronic Structure Of Pure And Doped Cem In5 (m=co,rh,ir) Crystals With Nuclear Quadrupolar Resonance

We report calculations of the electric-field gradients (EFGs) in pure and doped CeM In5 (M=Co, Rh, and Ir) compounds and compare with experiment. The degree to which the Ce4f electron is localized is treated within various models: the local-density approximation, generalized gradient approximation (GGA), GGA+U, and 4f -core approaches. We find that there is a correlation between the observed EFG and whether the 4f electron participates in the band formation or not. We also find that the EFG evolves linearly with Sn doping in CeRhIn5, suggesting the electronic structure is modified by doping. In contrast, the observed EFG in CeCoIn5 doped with Cd changes little with doping. These results indicate that nuclear quadrupolar resonance is a sensitive probe of electronic structure. © 2008 The American Physical Society.7724Slichter, C.P., (1990) Principles of Magnetic Resonance, , 3rd ed. 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Esr Of Gd3+ In The Kondo-lattice Compound Ybagcu4 And Its Reference Compounds Ragcu4 (r=y,lu)

Low-temperature (T&lt;30 K) electron-spin-resonance (ESR) experiments of Gd3+ diluted in the Kondo-lattice compound YbAgCu4 and its reference compounds YAgCu4 and LuAgCu4 are interpreted in terms of an enhanced density of states at the Fermi level for the Yb-based compound. The results of susceptibility and ESR (Korringa rate and g-shift) measurements show negligible electron-electron exchange enhancement for all the studied compounds. The exchange interaction between the Gd3+ local moment and the conduction electrons (c-e) is c-e wave vector dependent in all three compounds.561489338937Falicov, L.M., Hanke, W., Maple, M.B., (1981) Valence Fluctuation in Solids, , North-Holland, AmsterdamWachter, P., Boppart, H., (1982) Valence Instabilities, , North-Holland, AmsterdamMuller-Hartmann, E., Roden, B., Wohlleben, D., (1984) Valence Fluctuation, , North-Holland, AmsterdamBarberis, G.E., Foglio, M.E., Crow, J.E., Schlottmann, P., (1991) Valence Fluctuations, , North-Holland, AmsterdamKojima, K., Nakai, Y., Sizuki, T., Asano, H., Izumi, F., Fujita, T., Hihara, T., (1990) J. Phys. Soc. Jpn., 59, p. 792Rossel, C., Yang, K.N., Maple, M.B., Fisk, Z., Zirngiebl, E., Thompson, J.D., (1987) Phys. Rev. B, 35, p. 1914Fisk, Z., Maple, M.B., (1992) J. Alloys Compd., 183, p. 303Pillmayr, N., Bauer, E., Yoshimura, K., (1992) J. Magn. Magn. Mater., 104-107, p. 639Rajan, V.T., (1983) Phys. Rev. Lett., 51, p. 308Coqblin, B., Schrieffer, J.R., (1963) Phys. Rev., 185, p. 847Rettori, C., Oseroff, S.B., Rao, D., Pagliuso, P.G., Barberis, G.E., Sarrao, J., Fisk, Z., Hundley, M., (1997) Phys. Rev. B, 55, p. 1016Sarrao, J.L., Benton, C.L., Fisk, Z., Lawrence, J.M., Mandrus, D., Thompson, J.D., (1996) Physica B, 223-224, p. 366Sarrao, J.L., Immer, C.D., Benton, C.L., Fisk, Z., Lawrence, J.M., Mandrus, M., Thompson, J.D., (1996) Phys. Rev. B, 54, p. 12207Bachmann, R., DiSalvo, F.J., Geballe, T.H., Greene, R.L., Howard, R.E., King, C.N., Kivisch, H.C., Zubek, R.B., (1972) Rev. Sci. Instrum., 43, p. 205Feher, G., Kip, A.F., (1955) Phys. Rev., 98, p. 337Dyson, F.J., (1955) Phys. Rev., 98, p. 349Pake, G.E., Purcell, E.M., (1948) Phys. Rev., 74, p. 1184Yosida, K., (1957) Phys. Rev., 106, p. 893Korringa, J., (1950) Physica, 16, p. 601. , AmsterdamMoriya, T., (1963) J. Phys. Soc. Jpn., 18, p. 516Narath, A., (1967) Phys. Rev., 163, p. 232Davidov, D., Maki, K., Orbach, R., Rettori, C., Chock, E.P., (1973) Solid State Commun., 12, p. 621Davidov, D., Orbach, R., Rettori, C., Shaltiel, D., Tao, L.J., Ricks, B., (1971) Phys. Lett., 35 A, p. 339Rettori, C., Kim, H.M., Chock, E.P., Davidov, D., (1974) Phys. Rev. B, 10, p. 1826Narath, A., Weaver, H.T., (1968) Phys. Rev., 175, p. 373Shaw, R.W., Warren, W.W., (1971) Phys. Rev. B, 3, p. 1562Davidov, D., Chelkowski, A., Rettori, C., Orbach, R., Maple, M.B., (1973) Phys. Rev. B, 7, p. 1029Barberis, G.E., Davidov, D., Donoso, J.P., Rettori, C., Suassuna, J.F., Dokter, H.D., (1979) Phys. Rev. B, 19, p. 5495Abragam, A., Bleaney, B., (1970) EPR of Transition Ions, , Clarendon, OxfordSchlottmann, P., (1985) Theory of Heavy Fermion and Valence Fluctuation, p. 68. , edited by T. Kasuya and T. Saso Springer-Verlag. BerlinTsujii, N., He, J., Yoshimura, K., Kosuge, K., Michor, H., Kreiner, K., Hilscher, G., (1997) Phys. Rev. B, 55, p. 1032Watson, R.E., Freeman, A.J., Koide, S., (1969) Phys. Rev. B, 186, p. 625Continentino, M.A., (1993) Phys. Rev. B, 47, p. 11587Barberis, G.E., Davidov, D., Rettori, C., Donoso, J.P., Torriani, I., Gandra, F.C.G., (1980) Phys. Rev. Lett., 45, p. 1966Schaeffer, H., Elschner, B., (1983) Z. Phys. B, 53, p. 109Gandra, F.G., Schultz, S., Oseroff, S.B., Fisk, Z., Smith, J.L., (1985) Phys. Rev. Lett., 55, p. 2719Gandra, F.G., Pontes, M.J., Schultz, S., Oseroff, S.B., (1987) Solid State Commun., 64, p. 85

Esr Study Of The Eu2+ G -value In The Metallic Phase Of Cubic Hexaboride Ca1-x Eux B6 (0.15 X≤1.00)

The angular, magnetic field, and temperature dependence of the Eu2+ (4 f7, S=7/2) g -value in Ca1-x Eux B6 (0.15 x≤1.00) is measured by means of electron spin resonance at two microwave frequencies, 9.4 and 34.4 GHz. The g -value is found to be anisotropic and magnetic-field-dependent. The reduction with field of the positive g -shift is interpreted in terms of the exchange interaction between the localized Eu2+ 4 f7 electrons with the conduction Eu2+ 5d -like electrons and B 2p -like holes. The angular, temperature, and x dependence of the anisotropy of the g -value can be attributed to demagnetization effects due to the platelet-like shape of the samples. High-resolution synchrotron x-ray diffraction experiments show the absence of distortions larger than δa/a∼ 10-4. 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Magnetic structure of CeRhIn_5 as a function of pressure and temperature

We report magnetic neutron-diffraction and electrical resistivity studies on single crystals of the heavy-fermion antiferromagnet CeRhIn$_{5}$ at pressures up to 2.3 GPa. These experiments show that the staggered moment of Ce and the incommensurate magnetic structure change weakly with applied pressure up to 1.63 GPa, where resistivity, specific heat and NQR measurements confirm the presence of bulk superconductivity. This work places new constraints on an interpretation of the relationship between antiferromagnetism and unconventional superconductivity in CeRhIn$_{5}$.Comment: 6 pages, 6 figures, submitted to Phys. Rev.

Quantum Oscillations In Eufe2 As2 Single Crystals

Quantum oscillation measurements provide relevant information about the Fermi surface (FS) properties of strongly correlated metals. Here, we report on the Shubnikov-de Haas effect via high-field resistivity measurements of EuFe2As2 (Eu122) and BaFe2As2 (Ba122) single crystals. Although both pnictide compounds are isovalent with similar effective masses and density of states, at the Fermi level, our results reveal subtle changes in their fermiology. Remarkably, although the spin-density-wave (SDW) ordering temperature is higher in the Eu-rich end, Eu122 displays a much more isotropic and three-dimensional-like FS when compared with Ba122, in agreement with band structure calculations. Our experimental results suggest an anisotropic contribution of the Fe 3d orbitals to the FS in Ba122. We speculate that this orbital differentiation may be responsible for the suppression of the SDW phase in the FeAs-based compounds.9019Kamihara, Y., Watanabe, T., Hirano, M., Hosono, H., (2008) J. Am. 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