77 research outputs found
Fingerprinting the magnetic behavior of antiferromagnetic nanostructures using remanent magnetization curves
Antiferromagnetic (AF) nanostructures from Co3O4, CoO and Cr2O3 were prepared
by the nanocasting method and were characterized magnetometrically. The field
and temperature dependent magnetization data suggests that the nanostructures
consist of a core-shell structure. The core behaves as a regular
antiferromagnet and the shell as a two-dimensional diluted antiferromagnet in a
field (2d DAFF) as previously shown on Co3O4 nanowires [Benitez et al., Phys.
Rev. Lett. 101, 097206 (2008)]. Here we present a more general picture on three
different material systems, i.e. Co3O4, CoO and Cr2O3. In particular we
consider the thermoremanent (TRM) and the isothermoremanent (IRM) magnetization
curves as "fingerprints" in order to identify the irreversible magnetization
contribution originating from the shells. The TRM/IRM fingerprints are compared
to those of superparamagnetic systems, superspin glasses and 3d DAFFs. We
demonstrate that TRM/IRM vs. H plots are generally useful fingerprints to
identify irreversible magnetization contributions encountered in particular in
nanomagnets.Comment: submitted to PR
A Novel Dielectric Anomaly in Cuprates and Nickelates: Signature of an Electronic Glassy State
The low-frequency dielectric response of hole-doped insulators
La_{2}Cu_{1-x}Li_{x}O_{4} and La_{2-x}Sr_{x}NiO_{4} shows a large dielectric
constant \epsilon ^{'} at high temperature and a step-like drop by a factor of
100 at a material-dependent low temperature T_{f}. T_{f} increases with
frequency and the dielectric response shows universal scaling in a Cole-Cole
plot, suggesting that a charge glass state is realized both in the cuprates and
in the nickelates.Comment: 5 pages, 4 figure
Spinless impurities in high Tc cuprates: Kondo-like behavior
We compare the effects of in-plane non magnetic Li and Zn
impurities on the normal state of high-T cuprates. Y NMR shows that the
extra hole introduced by Li is not localized in its vicinity. The Tc depression
and induced moments on near neighbour Cu sites of Zn or Li are found identical.
These universal effects of spinless impurities establish the major influence of
the spin perturbation with respect to the charge defect. The susceptibility of
the induced moment measured by Li NMR displays a 1/(T+Theta) behavior. Theta
increases with doping up to about 200 K in the overdoped regime. We attribute
this to a "Kondo like" effect.Comment: To appear in Phys.Rev.Lett. (22 nov. 99) Minor modifications compared
to previous version. 8 pages (4 pages for text + 4 figures
Spin Glass Behavior in RuSr2Gd1.5Ce0.5Cu2O10
The dynamics of the magnetic properties of polycrystalline
RuSr2Gd1.5Ce0.5Cu2O10 (Ru-1222) have been studied by ac susceptibility and dc
magnetization measurements, including relaxation and ageing studies. Ru-1222 is
a reported magneto-superconductor with Ru spins magnetic ordering at
temperatures near 100 K and superconductivity in Cu-O2 planes below Tc ~ 40 K.
The exact nature of Ru spins magnetic ordering is still debated and no
conclusion has been reached yet. In this work, a frequency-dependent cusp was
observed in ac susceptibility vs. T measurements, which is interpreted as a
spin glass transition. The change in the cusp position with frequency follows
the Vogel-Fulcher law, which is commonly accepted to describe a spin glass with
magnetically interacting clusters. Such interpretation is supported by
themoremanaent magnetization (TRM) measurements at T = 60 K. TRM relaxations
are well described by a stretched exponential relation, and present significant
ageing effects.Comment: 4 pages, 6 figures, submitted to Phys. Rev.
Mean-field theory of temperature cycling experiments in spin-glasses
We study analytically the effect of temperature cyclings in mean-field
spin-glasses. In accordance with real experiments, we obtain a strong
reinitialization of the dynamics on decreasing the temperature combined with
memory effects when the original high temperature is restored. The same
calculation applied to mean-field models of structural glasses shows no such
reinitialization, again in accordance with experiments. In this context, we
derive some relations between experimentally accessible quantities and propose
new experimental protocols. Finally, we briefly discuss the effect of field
cyclings during isothermal aging.Comment: Some misprints corrected, references updated, final version to apper
in PR
Freezing and large time scales induced by geometrical frustration
We investigate the properties of an effective Hamiltonian with competing
interactions involving spin and chirality variables, relevant for the
description of the {\it trimerized} version of the spin-1/2 {\it kagome}
antiferromagnet. Using classical Monte Carlo simulations, we show that
remarkable behaviors develop at very low temperatures. Through an {\it order by
disorder} mechanism, the low-energy states are characterized by a dynamical
freezing of the chiralities, which decouples the lattice into ``dimers'' and
``triangles'' of antiferromagnetically coupled spins. Under the presence of an
external magnetic field, the particular topology of the chiralities induces a
very slow spin dynamics, reminiscent of what happens in ordinary spin glasses.Comment: 12 pages, 13 figure
Phase Separation and the Low-Field Bulk Magnetic Properties of Pr0.7Ca0.3MnO3
We present a detailed magnetic study of the perovskite manganite
Pr0.7Ca0.3MnO3 at low temperatures including magnetization and a.c.
susceptibility measurements. The data appear to exclude a conventional spin
glass phase at low fields, suggesting instead the presence of correlated
ferromagnetic clusters embedded in a charge-ordered matrix. We examine the
growth of the ferromagnetic clusters with increasing magnetic field as they
expand to occupy almost the entire sample at H ~ 0.5 T. Since this is well
below the field required to induce a metallic state, our results point to the
existence of a field-induced ferromagnetic insulating state in this material.Comment: 15 pages with figures, submitted to Physical Review
Real spin glasses relax slowly in the shade of hierarchical trees
The Parisi solution of the mean-field spin glass has been widely accepted and
celebrated. Its marginal stability in 3d and its complexity however raised the
question of its relevance to real spin glasses. This paper gives a short
overview of the important experimental results which could be understood within
the mean-field solution. The existence of a true phase transition and the
particular behaviour of the susceptibility below the freezing temperature,
predicted by the theory, are clearly confirmed by the experimental results. The
behaviour of the complex order parameter and of the Fluctuation Dissipation
ratio are in good agreement with results of spontaneous noise measurements. The
very particular ultrametric symmetry, the key feature of the theory, provided
us with a simple description of the rejuvenation and memory effects observed in
experiment. Finally, going a step beyond mean-field, the paper shortly
discusses new analyses in terms of correlated domains characterized by their
length scales, as well as new experiments on superspin glasses which compare
well with recent theoretical simulations.Comment: To appear in the proceedings of "Wandering with Curiosity in Complex
Landscapes", a scientific conference in honour of Giorgio Parisi for his 60th
birthday, Roma, September 8-10 2008 (submitted for the special issue of the
Journal of Statistical Physics, 2009
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