Density Functional Theory studies of cluster states in nuclei

The framework of nuclear energy density functionals is applied to a study of the formation and evolution of cluster states in nuclei. The relativistic functional DD-ME2 is used in triaxial and reflection-asymmetric relativistic Hartree-Bogoliubov calculations of relatively light $N = Z$ and neutron-rich nuclei. The role of deformation and degeneracy of single-nucleon states in the formation of clusters is analysed, and interesting cluster structures are predicted in excited configurations of Be, C, O, Ne, Mg, Si, S, Ar and Ca $N = Z$ nuclei. Cluster phenomena in neutron-rich nuclei are discussed, and it is shown that in neutron-rich Be and C nuclei cluster states occur as a result of molecular bonding of $\alpha$-particles by the excess neutrons, and also that proton covalent bonding can occur in $^{10}$C

Covariant energy density functionals with and without tensor couplings at the Hartree-Bogoliubov level

Background: The study of additional terms in functionals is relevant to better describe nuclear structure phenomenology. Among these terms, the tensor one is known to impact nuclear structure properties, especially in neutron-rich nuclei. However, its effect has not been studied on the whole nuclear chart yet. Purpose: The impact of terms corresponding to the tensor at the Hartree level, is studied for infinite nuclear matter as well as deformed nuclei, by developing new density-dependent functionals including these terms. In particular, we study in details the improvement such a term can bring to the description of specific nuclear observables. Methods: The framework of covariant energy density functional is used at the Hartree-Bogoliubov level. The free parameters of covariant functionals are optimized by combining Markov-Chain-Monte-Carlo and simplex algorithms. Results: An improvement of the RMS binding energies, spin-orbit splittings and gaps is obtained over the nuclear chart, including axially deformed ones, when including tensors terms. Small modifications of the potential energy surface and densities are also found. In infinite matter, the Dirac mass is shifted to a larger value, in better agreement with experiments. Conclusions: Taking into account additional terms corresponding to the tensor terms in the vector-isoscalar channel at the Hartree level, improves the description of nuclear properties, both in nuclei and in nuclear matter

Alpha-particle formation and clustering in nuclei

The nucleonic localization function has been used for a decade to study the formation of alpha-particles in nuclei, by providing a measure of having nucleons of a given spin in a single place. However, differences in interpretation remain, compared to the nucleonic density of the nucleus. In order to better understand the respective role of the nucleonic localization function and the densities in the alpha-particle formation in cluster states or in alpha-decay mechanism, both an analytic approximation and microscopic calculations, using energy density functionals, are undertaken. The nucleonic localization function is shown to measure the anti-centrifugal effect, and is not sensitive to the level of compactness of the alpha-particle itself. It probes the purity of the spatial overlap of four nucleons in the four possible (spin, isospin) states. The density provides, in addition, information on the compactness of an alpha-particle cluster.Comment: 8 pages, 5 figure

Relativistic Hartree-Fock-Bogoliubov model for deformed nuclei

The relativistic Hartree-Fock-Bogoliubov model for axially deformed nuclei (RHFBz) is introduced. The model is based on an effective Lagrangian with density-dependent meson-nucleon couplings in the particle-hole channel, and the central part of the Gogny force is used in the pairing channel. The RHFBz quasiparticle equations are solved by expansion in the basis of a deformed harmonic oscillator. Illustrative RHFBz calculations are performed for carbon, neon, and magnesium isotopes. The effect of explicitly including the pion field is investigated for binding energies, deformation parameters, and charge radii and has an impact on the nuclei’s shape

Rooting the EDF method into the ab initio framework. PGCM-PT formalism based on MR-IMSRG pre-processed Hamiltonians

Recently, ab initio techniques have been successfully connected to the traditional valence-space shell model. In doing so, they can either explicitly provide ab initio shell-model effective Hamiltonians or constrain the construction of empirical ones. In the present work, the possibility to follow a similar path for the nuclear energy density functional (EDF) method is analyzed. For this connection to be actualized, two theoretical techniques are instrumental: the recently proposed ab initio PGCM-PT many-body formalism and the MR-IMSRG pre-processing of the nuclear Hamiltonian. Based on both formal arguments and numerical results, possible new lines of research are briefly discussed, namely to compute ab initio EDF effective Hamiltonians at low computational cost, to constrain empirical ones or to produce them directly via an effective field theory that remains to be invented.Comment: 20 pages, 7 figure

Localization and clustering in the nuclear Fermi liquid

Using the framework of nuclear energy density functionals we examine the conditions for single-nucleon localization and formation of cluster structures in finite nuclei. We propose to characterize localization by the ratio of the dispersion of single-nucleon wave functions to the average inter-nucleon distance. This parameter generally increases with mass and describes the gradual transition from a hybrid phase in light nuclei, characterized by the spatial localization of individual nucleon states that leads to the formation of cluster structures, toward the Fermi liquid phase in heavier nuclei. Values of the localization parameter that correspond to a crystal phase cannot occur in finite nuclei. Typical length and energy scales in nuclei allow the formation of liquid drops, clusters, and halo structures.Comment: 6 pages, 3 figure

Microscopic description of α\alpha, 2α2\alpha, and cluster decays of 216,218^{216,218}Rn and 220−224^{220-224}Ra

Alpha and cluster decays are analyzed for heavy nuclei located above $^{208}$Pb on the chart of nuclides: $^{216,218}$Rn and $^{220-224}$Ra, that are also candidates for observing the $2 \alpha$ decay mode. A microscopic theoretical approach based on relativistic Energy Density Functionals (EDF), is used to compute axially-symmetric deformation energy surfaces as functions of quadrupole, octupole and hexadecupole collective coordinates. Dynamical least-action paths for specific decay modes are calculated on the corresponding potential energy surfaces. The effective collective inertia is determined using the perturbative cranking approximation, and zero-point and rotational energy corrections are included in the model. The predicted half-lives for $\alpha$-decay are within one order of magnitude of the experimental values. In the case of single $\alpha$ emission, the nuclei considered in the present study exhibit least-action paths that differ significantly up to the scission point. The differences in alpha-decay lifetimes are not only driven by Q values, but also by variances of the least-action paths prior to scission. In contrast, the $2 \alpha$ decay mode presents very similar paths from equilibrium to scission, and the differences in lifetimes are mainly driven by the corresponding Q values. The predicted $^{14}$C cluster decay half-lives are within three orders of magnitudes of the empirical values, and point to a much more complex pattern compared to the alpha-decay mode.Comment: 9 pages, 13 figure

Direct mass measurements of 19B, 22C, 29F, 31Ne, 34Na and other light exotic nuclei

We report on direct time-of-flight based mass measurements of 16 light neutron-rich nuclei. These include the first determination of the masses of the Borromean drip-line nuclei $^{19}$B, $^{22}$C and $^{29}$F as well as that of $^{34}$Na. In addition, the most precise determinations to date for $^{23}$N and $^{31}$Ne are reported. Coupled with recent interaction cross-section measurements, the present results support the occurrence of a two-neutron halo in $^{22}$C, with a dominant $\nu2s_{1/2}^2$ configuration, and a single-neutron halo in $^{31}$Ne with the valence neutron occupying predominantly the 2$p_{3/2}$ orbital. Despite a very low two-neutron separation energy the development of a halo in $^{19}$B is hindered by the 1$d_{5/2}^2$ character of the valence neutrons.Comment: 5 page