Molecular alignment from circular dichroic photoelectron angular distributions in (n+1) resonance enhanced multiphoton ionization

The theory for determination of molecular alignment from circular dichroism in photoelectron angular distributions is generalized to treat the case in which the excitation polarization direction and the laboratory z axis do not coincide. A new method of data analysis is presented here. Alignment created by surface scattering or photofragmentation should be obtainable by these procedures. For studies of orientation with elliptically polarized excitation, differential cross sections at a given collection angle are found to be, to a good approximation, independent of excited-state alignment. Orientation can thus be obtained from differential cross sections by the methods developed by Kummel, Sitz, and Zare [J. Chem. Phys. 88, 6707 (1988)]

Extraction of alignment parameters from circular dichroic photoelectron angular distribution (CDAD) measurements

In a previous paper, we showed that circular dichroism in photoelectron angular distributions (CDAD) can be used to probe alignment in gas phase atoms and linear molecules. Often this alignment is parametrized through the moments of alignment A(2), A(4), etc., which are commonly extracted from fluorescence polarization measurements. In this paper we show how these can be simply extracted from CDAD spectra. This technique can be used in principle to extract the moments to any order

Optimization of Multi-Frequency Magnonic Waveguides with Enhanced Group Velocities by Exchange Coupled Ferrimagnet/Ferromagnet Bilayers

We report broadband spectroscopy and numerical analysis by which we explore propagating spin waves in a magnetic bilayer consisting of a 23 nm thick permalloy film deposited on 130 nm thick $Y_{3}Fe_{5}O_{12}$. In the bilayer, we observe a characteristic mode that exhibits a considerably larger group velocity at small in-plane magnetic field than both the magnetostatic and perpendicular standing spin waves. Using the finite element method, we confirm the observations by simulating the mode profiles and dispersion relations. They illustrate the hybridization of spin wave modes due to exchange coupling at the interface. The high-speed propagating mode found in the bilayer can be utilized to configure multi-frequency spin wave channels enhancing the performance of spin wave based logic devices

Experimental proof of the reciprocal relation between spin Peltier and spin Seebeck effects in a bulk YIG/Pt bilayer

We verify for the first time the reciprocal relation between the spin Peltier and spin Seebeck effects in a bulk YIG/Pt bilayer. Both experiments are performed on the same YIG/Pt device by a setup able to accurately determine heat currents and to separate the spin Peltier heat from the Joule heat background. The sample-specific value for the characteristics of both effects measured on the present YIG/Pt bilayer is (6.2 \pm 0.4)\times 10^{-3} \,\, \mbox{KA^{-1}}. In the paper we also discuss the relation of both effects with the intrinsic and extrinsic parameters of YIG and Pt and we envisage possible strategies to optimize spin Peltier refrigeration.Comment: 11 pages, 3 figure

(1+ 1) CDAD: A new technique for studying photofragment alignment

We report a new technique for measuring photofragment alignment in the gas phase by observing circular dichroism in photoelectron angular distributions (CDAD). This technique is well suited for determining the gas phase alignment of linear molecules. The experiment involves excitation of the photofragment with linearly polarized light followed by photoionization with left or right circularly polarized light. The difference between the photoelectron angular distributions for these two cases is the CDAD spectrum. By measuring CDAD through two different excitation branches, one can obtain the ground state photofragment alignment A(2)0 using a simple analytical formula independent of the photoionization dynamics