Observation of inversion, hysteresis, and collapse of spin in optically trapped polariton condensates

The spin and intensity of optically trapped polariton condensates are studied under steady-state elliptically-polarised nonresonant pumping. Three distinct effects are observed: (1) spin inversion where condensation occurs in the opposite handedness from the pump, (2) spin/intensity hysteresis as the pump power is scanned, and (3) a sharp ‘spin collapse’ transition in the condensate spin as a function of the pump ellipticity. We show these effects are strongly dependent on trap size and sample position and are linked to small counterintuitive energy differences between the condensate spin components. Our results, which fail to be fully described within the commonly used nonlinear equations for polariton condensates, show that a more accurate microscopic picture is needed to unify these phenomena in a two-dimensional condensate theory

Spontaneous spin bifurcations and ferromagnetic phase transitions in a spinor exciton-polariton condensate

We observe a spontaneous parity breaking bifurcation to a ferromagnetic state in a spatially trapped exciton-polariton condensate. At a critical bifurcation density under nonresonant excitation, the whole condensate spontaneously magnetizes and randomly adopts one of two elliptically polarized (up to 95% circularly-polarized) states with opposite handedness of polarization. The magnetized condensate remains stable for many seconds at 5 K, but at higher temperatures it can flip from one magnetic orientation to another. We optically address these states and demonstrate the inversion of the magnetic state by resonantly injecting 100-fold weaker pulses of opposite spin. Theoretically, these phenomena can be well described as spontaneous symmetry breaking of the spin degree of freedom induced by different loss rates of the linear polarizations.This work was supported by Grants EPSRC No. EP/G060649/1, EU No. CLERMONT4 235114, EU No. INDEX 289968, Spanish MEC (MAT2008-01555), Greek GSRT ARISTEIA Apollo program and Fundación La Caixa, and Mexican CONACYT No. 251808. FP acknowledges financial support through an EPSRC doctoral prize fellowship at the University of Cambridge and a Schrödinger fellowship at the University of Oxford.This is the final version of the article. It first appeared from the American Physical Society via http://dx.doi.org/10.1103/PhysRevX.5.03100

Interrogating Nanojunctions Using Ultraconfined Acoustoplasmonic Coupling

Single nanoparticles are shown to develop a localized acoustic resonance, the bouncing mode, when placed on a substrate. If both substrate and nanoparticle are noble metals, plasmonic coupling of the nanoparticle to its image charges in the film induces tight light confinement in the nanogap. This yields ultrastrong “acoustoplasmonic” coupling with a figure of merit 7 orders of magnitude higher than conventional acousto-optic modulators. The plasmons thus act as a local vibrational probe of the contact geometry. A simple analytical mechanical model is found to describe the bouncing mode in terms of the nanoscale structure, allowing transient pump-probe spectroscopy to directly measure the contact area for individual nanoparticles.This work is supported by UK EPSRC grants EP/G060649/1, EP/L027151/1 and ERC grant LINASS 320503, as well as the Winton Programme for the Physics of Sustainability (FB, YdV-IR, JM), the Dr Manmohan Singh Scholarship from St John’s College (RC)

Synchronization crossover of polariton condensates in weakly disordered lattices

We demonstrate that the synchronization of a lattice of solid-state condensates when intersite tunneling is switched on depends strongly on the weak local disorder. This finding is vital for implementation of condensate arrays as computation devices. The condensates here are nonlinear bosonic fluids of exciton-polaritons trapped in a weakly disordered Bose-Hubbard potential, where the nearest-neighboring tunneling rate (Josephson coupling) can be dynamically tuned. The system can thus be tuned from a localized to a delocalized fluid as the number density or the Josephson coupling between nearest neighbors increases. The localized fluid is observed as a lattice of unsynchronized condensates emitting at different energies set by the disorder potential. In the delocalized phase, the condensates synchronize and long-range order appears, evidenced by narrowing of momentum and energy distributions, new diffraction peaks in momentum space, and spatial coherence between condensates. Our paper identifies similarities and differences of this nonequilibrium crossover to the traditional Bose-glass to superfluid transition in atomic condensates

Spin Order and Phase Transitions in Chains of Polariton Condensates

We demonstrate that multiply coupled spinor polariton condensates can be optically tuned through a sequence of spin-ordered phases by changing the coupling strength between nearest neighbors. For closed four-condensate chains these phases span from ferromagnetic (FM) to antiferromagnetic (AFM), separated by an unexpected crossover phase. This crossover phase is composed of alternating FM-AFM bonds. For larger eight-condensate chains, we show the critical role of spatial inhomogeneities and demonstrate a scheme to overcome them and prepare any desired spin state. Our observations thus demonstrate a fully controllable nonequilibrium spin lattice.We acknowledge Grants No. EPSRC EP/L027151/1, No. EU INDEX 289968, No. ERC “POLAFLOW” Starting Grant, ERC LINASS 320503, Spanish MEC (MAT2008- 01555), Mexican CONACYT 251808, Leverhulme Trust Grant No. VP1-2013-011 and Fundación La Caixa. H. S. and I. S. acknowledge support by the Research Fund of the University of Iceland, The Icelandic Research Fund, Grant No. 163082-051. T. L. was supported by the MOE AcRF Tier 1 Grant No. 2016-T1-001-084. P. S. acknowledges financial support from the Stavros Niarchos Foundation, “ARCHERS” project

Strain-assisted optomechanical coupling of polariton condensate spin to a micromechanical resonator

We report spin and intensity coupling of an exciton-polariton condensate to the mechanical vibrations of a circular membrane microcavity. We optically drive the microcavity resonator at the lowest mechanical resonance frequency while creating an optically-trapped spin-polarized polariton condensate in different locations on the microcavity, and observe spin and intensity oscillations of the condensate at the vibration frequency of the resonator. Spin oscillations are induced by vibrational strain driving, whilst the modulation of the optical trap due to the displacement of the membrane causes intensity oscillations in the condensate emission. Our results demonstrate spin-phonon coupling in a macroscopically coherent condensate

Spontaneous spin bifurcations and ferromagnetic phase transitions in a spinor exciton-polariton condensate

We observe a spontaneous parity breaking bifurcation to a ferromagnetic state in a spatially trapped exciton-polariton condensate. At a critical bifurcation density under nonresonant excitation, the whole condensate spontaneously magnetizes and randomly adopts one of two elliptically polarized (up to 95% circularly polarized) states with opposite handedness of polarization. The magnetized condensate remains stable for many seconds at 5 K, but at higher temperatures, it can flip from one magnetic orientation to another. We optically address these states and demonstrate the inversion of the magnetic state by resonantly injecting 100- fold weaker pulses of opposite spin. Theoretically, these phenomena can be well described as spontaneous symmetry breaking of the spin degree of freedom induced by different loss rates of the linear polarizations.Publisher PDFPeer reviewe

Stochastic spin flips in polariton condensates: Nonlinear tuning from GHz to sub-Hz

The stability of spin of macroscopic quantum states to intrinsic noise is studied for non-resonantly-pumped optically-trapped polariton condensates. We demonstrate flipping between the two spin-polarised states with >104 slow-down of the flip rate by tuning the optical pump power. Individual spin flips faster than 50 ps are time resolved using single-shot streak camera imaging. We reproduce our results within a mean-field model accounting for cross-spin scattering between excitons and polaritons, yielding a ratio of cross- to co-spin scattering of ∼0.6, in contrast with previous literature suggestions. © 2018 The Author(s). Published by IOP Publishing Ltd on behalf of Deutsche Physikalische Gesellschaf