Fast Single-Charge Sensing with an rf Quantum Point Contact

We report high-bandwidth charge sensing measurements using a GaAs quantum point contact embedded in a radio frequency impedance matching circuit (rf-QPC). With the rf-QPC biased near pinch-off where it is most sensitive to charge, we demonstrate a conductance sensitivity of 5x10^(-6) e^(2)/h Hz^(-1/2) with a bandwidth of 8 MHz. Single-shot readout of a proximal few-electron double quantum dot is investigated in a mode where the rf-QPC back-action is rapidly switched.Comment: related papers available at http://marcuslab.harvard.ed

Subtleties of witnessing quantum coherence in non-isolated systems

Identifying non-classicality unambiguously and inexpensively is a long-standing open challenge in physics. The No-Signalling-In-Time protocol was developed as an experimental test for macroscopic realism, and serves as a witness of quantum coherence in isolated quantum systems by comparing the quantum state to its completely dephased counterpart. We show that it provides a lower bound on a certain resource-theoretic coherence monotone. We go on to generalise the protocol to the case where the system of interest is coupled to an environment. Depending on the manner of the generalisation, the resulting witness either reports on system coherence alone, or on a disjunction of system coherence with either (i) the existence of non-classical system-environment correlations or (ii) non-negligible dynamics in the environment. These are distinct failure modes of the Born approximation in non-isolated systems.Comment: 16pp, 2 figs, 5 thms. v2: typos corrected, references added and small change to title to reflect that of published versio

Cotunneling Spectroscopy in Few-Electron Quantum Dots

Few-electron quantum dots are investigated in the regime of strong tunneling to the leads. Inelastic cotunneling is used to measure the two-electron singlet-triplet splitting above and below a magnetic field driven singlet-triplet transition. Evidence for a non-equilibrium two-electron singlet-triplet Kondo effect is presented. Cotunneling allows orbital correlations and parameters characterizing entanglement of the two-electron singlet ground state to be extracted from dc transport.Comment: related papers available at http://marcuslab.harvard.ed

Rapid Single-Shot Measurement of a Singlet-Triplet Qubit

We report repeated single-shot measurements of the two-electron spin state in a GaAs double quantum dot. The readout scheme allows measurement with fidelity above 90% with a 7 microsecond cycle time. Hyperfine-induced precession between singlet and triplet states of the two-electron system are directly observed, as nuclear Overhauser fields are quasi-static on the time scale of the measurement cycle. Repeated measurements on millisecond to second time scales reveal evolution of the nuclear environment.Comment: supplemental material at http://marcuslab.harvard.edu/papers/single_shot_sup.pd

Acute tryptophan depletion attenuates conscious appraisal of social emotional signals in healthy female volunteers

Rationale: Acute tryptophan depletion (ATD) decreases levels of central serotonin. ATD thus enables the cognitive effects of serotonin to be studied, with implications for the understanding of psychiatric conditions, including depression. Objective: To determine the role of serotonin in conscious (explicit) and unconscious/incidental processing of emotional information. Materials and methods: A randomized, double-blind, cross-over design was used with 15 healthy female participants. Subjective mood was recorded at baseline and after 4 h, when participants performed an explicit emotional face processing task, and a task eliciting unconscious processing of emotionally aversive and neutral images presented subliminally using backward masking. Results: ATD was associated with a robust reduction in plasma tryptophan at 4 h but had no effect on mood or autonomic physiology. ATD was associated with significantly lower attractiveness ratings for happy faces and attenuation of intensity/arousal ratings of angry faces. ATD also reduced overall reaction times on the unconscious perception task, but there was no interaction with emotional content of masked stimuli. ATD did not affect breakthrough perception (accuracy in identification) of masked images. Conclusions: ATD attenuates the attractiveness of positive faces and the negative intensity of threatening faces, suggesting that serotonin contributes specifically to the appraisal of the social salience of both positive and negative salient social emotional cues. We found no evidence that serotonin affects unconscious processing of negative emotional stimuli. These novel findings implicate serotonin in conscious aspects of active social and behavioural engagement and extend knowledge regarding the effects of ATD on emotional perception

In-vivo magnetic resonance imaging of hyperpolarized silicon particles

Silicon-based micro and nanoparticles have gained popularity in a wide range of biomedical applications due to their biocompatibility and biodegradability in-vivo, as well as a flexible surface chemistry, which allows drug loading, functionalization and targeting. Here we report direct in-vivo imaging of hyperpolarized 29Si nuclei in silicon microparticles by MRI. Natural physical properties of silicon provide surface electronic states for dynamic nuclear polarization (DNP), extremely long depolarization times, insensitivity to the in-vivo environment or particle tumbling, and surfaces favorable for functionalization. Potential applications to gastrointestinal, intravascular, and tumor perfusion imaging at sub-picomolar concentrations are presented. These results demonstrate a new background-free imaging modality applicable to a range of inexpensive, readily available, and biocompatible Si particles.Comment: Supplemental Material include

Wide-angle perfect absorber/thermal emitter in the THz regime

We show that a perfect absorber/thermal emitter exhibiting an absorption peak of 99.9% can be achieved in metallic nanostructures that can be easily fabricated. The very high absorption is maintained for large angles with a minimal shift in the center frequency and can be tuned throughout the visible and near-infrared regime by scaling the nanostructure dimensions. The stability of the spectral features at high temperatures is tested by simulations using a range of material parameters.Comment: Submitted to Phys. Rev. Let

Latched Detection of Excited States in an Isolated Double Quantum Dot

Pulsed electrostatic gating combined with capacitive charge sensing is used to perform excited state spectroscopy of an electrically isolated double-quantum-dot system. The tunneling rate of a single charge moving between the two dots is affected by the alignment of quantized energy levels; measured tunneling probabilities thereby reveal spectral features. Two pulse sequences are investigated, one of which, termed latched detection, allows measurement of a single tunneling event without repetition. Both provide excited-state spectroscopy without electrical contact to the double-dot system.Comment: related papers available at http://marcuslab.harvard.ed