3,950 research outputs found
The Quasi-1D S=1/2 Antiferromagnet Cs2CuCl4 in a Magnetic Field
Magnetic excitations of the quasi-1D S=1/2 Heisenberg antiferromagnet (HAF)
Cs2CuCl4 have been measured as a function of magnetic field using neutron
scattering. For T<0.62 K and B=0 T the weak inter-chain coupling produces 3D
incommensurate ordering. Fields greater than Bc =1.66 T, but less than the
field (~8 T) required to fully align the spins, are observed to decouple the
chains, and the system enters a disordered intermediate-field phase (IFP). The
IFP excitations are in agreement with the predictions of Muller et al. for the
1D S=1/2 HAF, and Talstra and Haldane for the related 1/r^2 chain (the
Haldane-Shastry model). This behaviour is inconsistent with linear spin-wave
theory.Comment: 10 pages, 4 encapsulated postscript figures, LaTeX, to be published
in PRL, e-mail comments to [email protected]
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Group 13 Decamethylmetallocenium Cations
Salts containing the decamethylmetallocenium cations, [( C5Me5) M-2](+) ( or Cp*M-2(+)) of the group 13 "metals" B, Al and Ga have been prepared using a variety of synthetic routes. Precursor molecules of the type Cp*2MX ( X = Cl, Br, Me) exhibit structural features that vary significantly depending on the size and electronegativity of the central atom. While salt metathesis, halide abstraction and methanide abstraction methods represent viable routes for the preparation of salts of Cp*B-2(+) and Cp*Al-2(+), acidolysis of a Cp* group from Cp*Ga-3 is the most reliable method for the synthesis of the analogous gallium cation. Gallocenium cations are less stable than either of the lighter congeneric cations since they prove to be susceptible to decomposition reactions involving the "back-transfer" of ligands from the counter anion. Density functional theory (DFT) calculations revealed that, whereas Cp*Ga-2(+) is predicted to adopt a molecular structure more similar to that of Cp*B-2(+), the electronic structure of the gallium cation bears a greater resemblance to that of Cp*Al-2(+).Chemistr
Optical Conductivity in a Two-Band Superconductor: Pb
We demonstrate the effect of bandstructure on the superconducting properties
of Pb by calculating the strong-coupling features in the optical conductivity,
, due to the electron-phonon interaction. The importance of
momentum dependence in the calculation of the properties of superconductors has
previously been raised for MgB. Pb resembles MgB in that it is a two
band superconductor in which the bands' contributions to the Fermi surface have
very different topologies. We calculate by calculating a
memory function which has been recently used to analyze of
BiSrCaCuO. In our calculations the two components of
the Fermi surface are described by parameterizations of de Haas--van Alphen
data. We use a phonon spectrum which is a fit to neutron scattering data. By
including the momentum dependence of the Fermi surface good agreement is found
with the experimentally determined strong-coupling features which can be
described by a broad peak at around 4.5 meV and a narrower higher peak around 8
meV of equal height. The calculated features are found to be dominated by
scattering between states within the third band. By contrast scattering between
states in the second band leads to strong-coupling features in which the height
of the high energy peak is reduced by compared to that of the low
energy peak. This result is similar to that in the conventional isotropic
(momentum independent) treatment of superconductivity. Our results show that it
is important to use realistic models of the bandstructure and phonons, and to
avoid using momentum averaged quantities, in calculations in order to get
quantitatively accurate results
FUSE Spectra of the Black Hole Binary LMC X-3
Far-ultraviolet spectra of LMC X-3 were taken covering photometric phases
0.47 to 0.74 in the 1.7-day orbital period of the black-hole binary (phase zero
being superior conjunction of the X-ray source). The continuum is faint and
flat, but appears to vary significantly during the observations. Concurrent
RXTE/ASM observations show the system was in its most luminous X-ray state
during the FUSE observations. The FUV spectrum contains strong terrestrial
airglow emission lines, while the only stellar lines clearly present are
emissions from the O VI resonance doublet. Their flux does not change
significantly during the FUSE observations. These lines are modelled as two
asymmetrical profiles, including the local ISM absorptions due to C II and
possibly O VI. Velocity variations of O VI emission are consistent with the
orbital velocity of the black hole and provide a new constraint on its mass.Comment: 12 pages including 1 table, 4 diagrams To appear in A
AGN in the XMM-Newton first-light image as probes for the interstellar medium in the LMC
The XMM-Newton first-light image revealed X-ray point sources which show
heavily absorbed power-law spectra. The spectral indices and the probable
identification of a radio counterpart for the brightest source suggest AGN
shining through the interstellar gas of the Large Magellanic Cloud (LMC). The
column densities derived from the X-ray spectra in combination with HI
measurements will allow to draw conclusions on HI to H_2 ratios in the LMC and
compare these with values found for the galactic plane.Comment: 4 pages, LaTex, 4 figures, Accepted for publication in A&A Letter
Isotopic Production Cross Sections in Proton-Nucleus Collisions at 200 MeV
Intermediate mass fragments (IMF) from the interaction of Al,
Co and Au with 200 MeV protons were measured in an angular range
from 20 degree to 120 degree in the laboratory system. The fragments, ranging
from isotopes of helium up to isotopes of carbon, were isotopically resolved.
Double differential cross sections, energy differential cross sections and
total cross sections were extracted.Comment: accepted by Phys. Rev.
Steady Hall Magnetohydrodynamics Near a X-type Magnetic Neutral Line
Hall magnetohydrodynamics (MHD) properties near a two-dimensional (2D) X-type
magnetic neutral line in the steady state are considered via heuristic and
rigorous developments. Upon considering the steady-state as the asymptotic
limit of the corresponding \textit{time-dependent} problem and using a rigorous
development, Hall effects are shown to be able to sustain the hyperbolicity of
the magnetic field (and hence a more open X-point configuration) near the
neutral line in the steady state. The heuristic development misses this subtle
connection of the steady state with the corresponding \textit{time-dependent}
problem and predicts only an elongated current-sheet configuration (as in
resistive MHD). However, the heuristic development turns out to be useful in
providing insight into the lack of dependence of the reconnection rate on the
mechanism breaking the frozen-in condition of the magnetic field lines. The
latter result can be understood in terms of the ability of the ions and
electrons to transport equal amounts of magnetic flux per unit time out of the
reconnection region.Comment: 1-10 page
On stability of the three-dimensional fixed point in a model with three coupling constants from the expansion: Three-loop results
The structure of the renormalization-group flows in a model with three
quartic coupling constants is studied within the -expansion method up
to three-loop order. Twofold degeneracy of the eigenvalue exponents for the
three-dimensionally stable fixed point is observed and the possibility for
powers in to appear in the series is investigated.
Reliability and effectiveness of the -expansion method for the given
model is discussed.Comment: 14 pages, LaTeX, no figures. To be published in Phys. Rev. B, V.57
(1998
Two and Three Dimensional Incommensurate Modulation in Optimally-Doped BiSrCaCuO
X-ray scattering measurements on optimally-doped single crystal samples of
the high temperature superconductor BiSrCaCuO reveal
the presence of three distinct incommensurate charge modulations, each
involving a roughly fivefold increase in the unit cell dimension along the {\bf
b}-direction. The strongest scattering comes from the well known (H, K
0.21, L) modulation and its harmonics. However, we also observe broad
diffraction which peak up at the L values complementary to those which
characterize the known modulated structure. These diffraction features
correspond to correlation lengths of roughly a unit cell dimension,
20 in the {\bf c} direction, and of 185
parallel to the incommensurate wavevector. We interpret these features as
arising from three dimensional incommensurate domains and the interfaces
between them, respectively. In addition we investigate the recently discovered
incommensuate modulations which peak up at (1/2, K 0.21, L) and related
wavevectors. Here we explicitly study the L-dependence of this scattering and
see that these charge modulations are two dimensional in nature with weak
correlations on the scale of a bilayer thickness, and that they correspond to
short range, isotropic correlation lengths within the basal plane. We relate
these new incommensurate modulations to the electronic nanostructure observed
in BiSrCaCuO using STM topography.Comment: 8 pages, 8 figure
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