Simulated XUV Photoelectron Spectra of THz-pumped Liquid Water

Highly intense, sub-picosecond terahertz (THz) pulses can be used to induce ultrafast temperature jumps (T-jumps) in liquid water. A supercritical state of gas-like water with liquid density is established, and the accompanying structural changes are expected to give rise to time-dependent chemical shifts. We investigate the possibility of using extreme ultraviolet (XUV) photoelectron spectroscopy as a probe for ultrafast dynamics induced by sub-picosecond THz pulses of varying intensities and frequencies. To this end, we use ab initio methods to calculate photoionization cross sections and photoelectron energies of (H2O)$_{20}$ clusters embedded in an aqueous environment represented by point charges. The cluster geometries are sampled from ab initio molecular dynamics simulations modeling the THz-water interactions. We find that the peaks in the valence photoelectron spectrum are shifted by up to 0.4 eV after the pump pulse, and that they are broadened with respect to unheated water. The shifts can be connected to structural changes caused by the heating, but due to saturation effects they are not sensitive enough to serve as a thermometer for T-jumped water

Limitations to THz generation by optical rectification using tilted pulse fronts

Terahertz (THz) generation by optical rectification (OR) using tilted-pulse-fronts is studied. One-dimensional (1-D) and 2-D spatial models, which simultaneously account for (i) the nonlinear coupled interaction of the THz and optical radiation, (ii) angular and material dispersion, (iii) absorption, iv) self-phase modulation and (v) stimulated Raman scattering are presented. We numerically show that the large experimentally observed cascaded frequency down-shift and spectral broadening (cascading effects) of the optical pump pulse is a direct consequence of THz generation. In the presence of this large spectral broadening, the phase mismatch due to angular dispersion is greatly enhanced. Consequently, this cascading effect in conjunction with angular dispersion is shown to be the strongest limitation to THz generation in lithium niobate for pumping at 1 micron. It is seen that the exclusion of these cascading effects in modeling OR, leads to a significant overestimation of the optical-to-THz conversion efficiency. The simulation results are supported by experiments

Direct laser acceleration of electrons in free-space

Compact laser-driven accelerators are versatile and powerful tools of unarguable relevance on societal grounds for the diverse purposes of science, health, security, and technology because they bring enormous practicality to state-of-the-art achievements of conventional radio-frequency accelerators. Current benchmarking laser-based technologies rely on a medium to assist the light-matter interaction, which impose material limitations or strongly inhomogeneous fields. The advent of few cycle ultra-intense radially polarized lasers has materialized an extensively studied novel accelerator that adopts the simplest form of laser acceleration and is unique in requiring no medium to achieve strong longitudinal energy transfer directly from laser to particle. Here we present the first observation of direct longitudinal laser acceleration of non-relativistic electrons that undergo highly-directional multi-GeV/m accelerating gradients. This demonstration opens a new frontier for direct laser-driven particle acceleration capable of creating well collimated and relativistic attosecond electron bunches and x-ray pulses

Long-term Hybrid Stabilization of the Carrier-Envelope Phase

Controlling the carrier envelope phase (CEP) in mode-locked lasers over practically long timescales is crucial for real-world applications in ultrafast optics and precision metrology. We present a hybrid solution that combines a feed-forward technique to stabilize the phase offset in fast timescales and a feedback technique that addresses slowly varying sources of interference and locking bandwidth limitations associated with gain media with long upper-state lifetimes. We experimentally realize the hybrid stabilization system in an Er:Yb:glass mode-locked laser and demonstrate 75 hours of stabilization with integrated phase noise of 14 mrad (1 Hz to 3 MHz), corresponding to around 11 as of carrier to envelope jitter. Additionally, we examine the impact of environmental factors, such as humidity and pressure, on the long-term stability and performance of the system.Comment: 11 pages, 6 figures, 1 table; to be published in Optics Express; revisions include adjustment of some citations, additions to section 2, and added information in table

Design, Optimization, and Blackbox Optimization of Laser Systems

Chirped pulse amplification (CPA) and subsequent nonlinear optical (NLO) systems constitute the backbone of myriad advancements in semiconductor and additive manufacturing, communication networks, biology and medicine, defense and national security, and a host of other sectors over the past decades. Accurately and efficiently modeling CPA and NLO-based laser systems is challenging because of the multitude of coupled linear and nonlinear processes and high variability in simulation frameworks. The lack of fully-integrated models severely hampers further advances in tailoring existing or materializing new CPA+NLO systems. Such tools are the key to enabling emerging optimization and inverse design approaches reliant on data-driven machine learning methods. Here, we present a modular start-to-end software model encompassing an array of amplifier designs and nonlinear optics techniques. The simulator renders time- and frequency-resolved electromagnetic fields alongside essential physical characteristics of energy, fluence, and spectral distribution. To demonstrate its robustness and real-world applicability -- specifically, reverse engineering, system optimization, and inverse design -- we present a case study on the LCLS-II photo-injector laser, representative of a high-power and spectro-temporally non-trivial CPA+NLO system

Laser-Induced Linear Electron Acceleration in Free Space

Linear acceleration in free space is a topic that has been studied for over 20 years, and its ability to eventually produce high-quality, high energy multi-particle bunches has remained a subject of great interest. Arguments can certainly be made that such an ability is very doubtful. Nevertheless, we chose to develop an accurate and truly predictive theoretical formalism to explore this remote possibility in a computational experiment. The formalism includes exact treatment of Maxwell's equations, exact relativistic treatment of the interaction among the multiple individual particles, and exact treatment of the interaction at near and far field. Several surprising results emerged. For example, we find that 30 keV electrons (2.5% energy spread) can be accelerated to 7.7 MeV (2.5% spread) and to 205 MeV (0.25% spread) using 25 mJ and 2.5 J lasers respectively. These findings should hopefully guide and help develop compact, high-quality, ultra-relativistic electron sources, avoiding conventional limits imposed by material breakdown or structural constraints.Comment: Supplementary Information starts on pg 1

Primeras luces de un espectroscopio impreso en 3D

La espectroscopía aplicada a la astronomía es una de las técnicas más potentes que tenemos para poder estudiar la naturaleza física de los astros. Esta técnica nos ha permitido, entre otras cosas, poder determinar la composición química de las fotosferas estelares, la detección de exoplanetas y es la técnica que nos ha permitido poder medir la expansión del universo. Al tratarse de una técnica tan potente los miembros del Grupo Universitario de Astronomía decidimos iniciarnos en esta técnica