2,910 research outputs found
Magnetic ordering in GdNi2B2C revisited by resonant x-ray scattering: evidence for the double-q model
Recent theoretical efforts aimed at understanding the nature of
antiferromagnetic ordering in GdNi2B2C predicted double-q ordering. Here we
employ resonant elastic x-ray scattering to test this theory against the
formerly proposed, single-q ordering scenario. Our study reveals a satellite
reflection associated with a mixed-order component propagation wave vector,
viz., (q_a,2q_b,0) with q_b = q_a approx= 0.55 reciprocal lattice units, the
presence of which is incompatible with single-q ordering but is expected from
the double-q model. A (3q_a,0,0) wave vector (i.e., third-order) satellite is
also observed, again in line with the double-q model. The temperature
dependencies of these along with that of a first-order satellite are compared
with calculations based on the double-q model and reasonable qualitative
agreement is found. By examining the azimuthal dependence of first-order
satellite scattering, we show the magnetic order to be, as predicted,
elliptically polarized at base temperature and find the temperature dependence
of the "out of a-b plane" moment component to be in fairly good agreement with
calculation. Our results provide qualitative support for the double-q model and
thus in turn corroborate the explanation for the "magnetoelastic paradox"
offered by this model.Comment: 8 pages, 5 figures. Submitted to Phys. Rev.
Drastic annealing effects in transport properties of single crystals of the YbNi2B2C heavy fermion system
We report temperature dependent resistivity, specific heat, magnetic
susceptibility and thermoelectric power measurements made on the heavy fermion
system YbNi2B2C, for both as grown and annealed single crystals. Our results
demonstrate a significant variation in the temperature dependent electrical
resistivity and thermoelectric power between as grown crystals and crystals
that have undergone optimal (150 hour, 950 C) annealing, whereas the
thermodynamic properties: (c_p(T) and chi(T)) remain almost unchanged. We
interpret these results in terms of redistributions of local Kondo temperatures
associated with ligandal disorder for a small (~ 1%) fraction of the Yb sites.Comment: 5 pages, 4 figures, submitted to PR
Magnetic and superconducting phase diagrams in ErNi2B2C
We present measurements of the superconducting upper critical field Hc2(T)
and the magnetic phase diagram of the superconductor ErNi2B2C made with a
scanning tunneling microscope (STM). The magnetic field was applied in the
basal plane of the tetragonal crystal structure. We have found large gapless
regions in the superconducting phase diagram of ErNi2B2C, extending between
different magnetic transitions. A close correlation between magnetic
transitions and Hc2(T) is found, showing that superconductivity is strongly
linked to magnetism.Comment: 5 pages, 4 figure
Intrinsic pinning on structural domains in underdoped single crystals of Ba(FeCo)As
Critical current density was studied in single crystals of
Ba(FeCo)As for the values of spanning the entire doping
phase diagram. A noticeable enhancement was found for slightly underdoped
crystals with the peak at . Using a combination of polarized-light
imaging, x-ray diffraction and magnetic measurements we associate this behavior
with the intrinsic pinning on structural domains in the orthorhombic phase.
Domain walls extend throughout the sample thickness in the direction of
vortices and act as extended pinning centers. With the increasing domain
structure becomes more intertwined and fine due to a decrease of the
orthorhombic distortion. This results in the energy landscape with maze-like
spatial modulations favorable for pinning. This finding shows that iron-based
pnictide superconductors, characterized by high values of the transition
temperature, high upper critical fields, and low anisotropy may intrinsically
have relatively high critical current densities.Comment: estimation of Jc correcte
Direct observation of Fe spin reorientation in single crystalline YbFe6Ge6
We have grown single crystals of YbFe6Ge6 and LuFe6Ge6 and characterized
their anisotropic behaviour through low field magnetic susceptibility,
field-dependent magnetization, resistivity and heat capacity measurements. The
Yb+3 valency is confirmed by LIII XANES measurements. YbFe6Ge6 crystals exhibit
a field-dependent, sudden reorientation of the Fe spins at about 63 K, a unique
effect in the RFe6Ge6 family (R = rare earths) where the Fe ions order
anti-ferromagnetically with Neel temperatures above 450 K and the R ions'
magnetism appears to behave independently. The possible origins of this unusual
behaviour of the ordered Fe moments in this compound are discussed.Comment: 12 pages, 8 figures, accepted in J. Phys.: Cond. Matte
Ferromagnetism or slow paramagnetic relaxation in Fe-doped LiN?
We report on isothermal magnetization, M\"ossbauer spectroscopy, and
magnetostriction as well as temperature-dependent alternating-current (ac)
susceptibility, specific heat, and thermal expansion of single crystalline and
polycrstalline Li(LiFe)N with and .
Magnetic hysteresis emerges at temperatures below K with
coercivity fields of up to T at K and magnetic
anisotropy energies of K (meV). The ac susceptibility is strongly
frequency dependent (--Hz) and reveals an effective energy
barrier for spin reversal of K. The relaxation times
follow Arrhenius behavior for K. For K, however, the
relaxation times of s are only weakly
temperature-dependent indicating the relevance of a quantum tunneling process
instead of thermal excitations. The magnetic entropy amounts to more than
J molK which significantly exceeds ln2, the
value expected for the entropy of a ground state doublet. Thermal expansion and
magnetostriction indicate a weak magneto-elastic coupling in accordance with
slow relaxation of the magnetization. The classification of
Li(LiFe)N as ferromagnet is stressed and contrasted with highly
anisotropic and slowly relaxing paramagnetic behavior.Comment: 12 pages, 10 figure
Anisotropy Reversal of the Upper Critical Field at Low Temperatures and Spin-Locked Superconductivity in K2Cr3As3
We report the first measurements of the anisotropic upper critical field
for KCrAs single crystals up to 60 T and K. Our results show that the upper critical field parallel to the Cr
chains, , exhibits a paramagnetically-limited behavior,
whereas the shape of the curve (perpendicular to the Cr
chains) has no evidence of paramagnetic effects. As a result, the curves
and cross at K, so that
the anisotropy parameter
increases from near to at 0.6 K. This behavior of is inconsistent with triplet
superconductivity but suggests a form of singlet superconductivity with the
electron spins locked onto the direction of Cr chains
Ingredients for the electronic nematic phase in FeSe revealed by its anisotropic optical response
The origin of the anisotropy in physical quantities related to a symmetry-broken (nematic) electronic state is still very much debated in high-temperature superconductors. FeSe at ambient pressure undergoes a structural, tetragonal-to-orthorhombic phase transition at Ts≃90 K without any magnetic ordering on further cooling, which leads to an ideal electronic nematicity. Our unprecedented optical results provide evidence that the low-energy excitation spectrum in the nematic phase is shaped by an important interplay of the anisotropic Drude weight and scattering rate. In the zero-frequency limit though, the temperature dependence of the anisotropic scattering rate plays the dominant role and, combined with the nematic order parameter as evinced from the high energy optical response, accounts for the anisotropic dc resistivity. This favors the scattering by anisotropic spin fluctuations as the prominent candidate in governing the properties of the nematic phase
Structural optimization of framed structures using generalized optimality criteria
The application of a generalized optimality criteria to framed structures is presented. The optimality conditions, Lagrangian multipliers, resizing algorithm, and scaling procedures are all represented as a function of the objective and constraint functions along with their respective gradients. The optimization of two plane frames under multiple loading conditions subject to stress, displacement, generalized stiffness, and side constraints is presented. These results are compared to those found by optimizing the frames using a nonlinear mathematical programming technique
Imaging Orbital-selective Quasiparticles in the Hund's Metal State of FeSe
Strong electronic correlations, emerging from the parent Mott insulator
phase, are key to copper-based high temperature superconductivity (HTS). By
contrast, the parent phase of iron-based HTS is never a correlated insulator.
But this distinction may be deceptive because Fe has five active d-orbitals
while Cu has only one. In theory, such orbital multiplicity can generate a
Hund's Metal state, in which alignment of the Fe spins suppresses inter-orbital
fluctuations producing orbitally selective strong correlations. The spectral
weights of quasiparticles associated with different Fe orbitals m should
then be radically different. Here we use quasiparticle scattering interference
resolved by orbital content to explore these predictions in FeSe. Signatures of
strong, orbitally selective differences of quasiparticle appear on all
detectable bands over a wide energy range. Further, the quasiparticle
interference amplitudes reveal that , consistent with
earlier orbital-selective Cooper pairing studies. Thus, orbital-selective
strong correlations dominate the parent state of iron-based HTS in FeSe.Comment: for movie M1, see
http://www.physik.uni-leipzig.de/~kreisel/osqp/M1.mp4, for movie M2, see
http://www.physik.uni-leipzig.de/~kreisel/osqp/M2.mp4, for movie M3, see
http://www.physik.uni-leipzig.de/~kreisel/osqp/M3.mp4, for movie M4, see
http://www.physik.uni-leipzig.de/~kreisel/osqp/M4.mp4, for movie M5, see
http://www.physik.uni-leipzig.de/~kreisel/osqp/M5.mp
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