207 research outputs found
Optical Stark Effect and Dressed Excitonic States in a Mn-doped Quantum Dot
We report on the observation of spin dependent optically dressed states and
optical Stark effect on an individual Mn spin in a semiconductor quantum dot.
The vacuum-to-exciton or the exciton-to-biexciton transitions in a Mn-doped
quantum dot are optically dressed by a strong laser field and the resulting
spectral signature is measured in photoluminescence. We demonstrate that the
energy of any spin state of a Mn atom can be independently tuned using the
optical Stark effect induced by a control laser. High resolution spectroscopy
reveals a power, polarization and detuning dependent Autler-Townes splitting of
each optical transition of the Mn-doped quantum dot. This experiment
demonstrates a complete optical resonant control of the exciton-Mn system
Optical control of the spin state of two Mn atoms in a quantum dot
We report on the optical spectroscopy of the spin of two magnetic atoms (Mn)
embedded in an individual quantum dot interacting with either a single
electron, a single exciton and single trion. As a result of their interaction
to a common entity, the Mn spins become correlated. The dynamics of this
process is probed by time resolved spectroscopy, that permits to determine the
optical orientation time in the range of a few tens of . In addition, we
show that the energy of the collective spin states of the two Mn atoms can be
tuned through the optical Stark effect induced by a resonant laser field
Spin-phonon coupling in single Mn doped CdTe quantum dot
The spin dynamics of a single Mn atom in a laser driven CdTe quantum dot is
addressed theoretically. Recent experimental
results\cite{Le-Gall_PRL_2009,Goryca_PRL_2009,Le-Gall_PRB_2010}show that it is
possible to induce Mn spin polarization by means of circularly polarized
optical pumping. Pumping is made possible by the faster Mn spin relaxation in
the presence of the exciton. Here we discuss different Mn spin relaxation
mechanisms. First, Mn-phonon coupling, which is enhanced in the presence of the
exciton. Second, phonon-induced hole spin relaxation combined with carrier-Mn
spin flip coupling and photon emission results in Mn spin relaxation. We model
the Mn spin dynamics under the influence of a pumping laser that injects
excitons into the dot, taking into account exciton-Mn exchange and phonon
induced spin relaxation of both Mn and holes. Our simulations account for the
optically induced Mn spin pumping.Comment: 17 pages, 11 figures, submitted to PR
Electron-nuclei spin dynamics in II-VI semiconductor quantum dots
We report on the dynamics of optically induced nuclear spin polarization in
individual CdTe/ZnTe quantum dots loaded with one electron by modulation
doping. The fine structure of the hot trion (charged exciton with an
electron in the -shell) is identified in photoluminescence excitation
spectra. A negative polarisation rate of the photoluminescence, optical pumping
of the resident electron and the built-up of dynamic nuclear spin polarisation
(DNSP) are observed in time-resolved optical pumping experiments when the
quantum dot is excited at higher energy than the hot trion triplet state. The
time and magnetic field dependence of the polarisation rate of the
emission allows to probe the dynamics of formation of the DNSP in the optical
pumping regime. We demonstrate using time-resolved measurements that the
creation of a DNSP at B=0T efficiently prevents longitudinal spin relaxation of
the electron caused by fluctuations of the nuclear spin bath. The DNSP is built
in the microsecond range at high excitation intensity. A relaxation time of the
DNSP in about 10 microseconds is observed at and significantly increases
under a magnetic field of a few milli-Tesla. We discuss mechanisms responsible
for the fast initialisation and relaxation of the diluted nuclear spins in this
system
Subnanosecond spectral diffusion of a single quantum dot in a nanowire
We have studied spectral diffusion of the photoluminescence of a single CdSe
quantum dot inserted in a ZnSe nanowire. We have measured the characteristic
diffusion time as a function of pumping power and temperature using a recently
developed technique [G. Sallen et al, Nature Photon. \textbf{4}, 696 (2010)]
that offers subnanosecond resolution. These data are consistent with a model
where only a \emph{single} carrier wanders around in traps located in the
vicinity of the quantum dot
Decoherence processes during active manipulation of excitonic qubits in semiconductor quantum dots
Using photoluminescence spectroscopy, we have investigated the nature of Rabi
oscillation damping during active manipulation of excitonic qubits in
self-assembled quantum dots. Rabi oscillations were recorded by varying the
pulse amplitude for fixed pulse durations between 4 ps and 10 ps. Up to 5
periods are visible, making it possible to quantify the excitation dependent
damping. We find that this damping is more pronounced for shorter pulse widths
and show that its origin is the non-resonant excitation of carriers in the
wetting layer, most likely involving bound-to-continuum and continuum-to-bound
transitions.Comment: 18 pages, 4 figure
Presión, temperatura y tiempo de procesamiento para mejorar la extracción de aceite de Camelina sativa mediante pretratamiento texturizado de descompresión instantánea controlada (DIC)
Instant Controlled Pressure Drop (DIC) was evaluated as a texturing pre-treatment for the extraction of Camelina sativa (L.) oil. DIC was coupled to Accelerated Solvent Extraction (ASE), Pressing and Dynamic Maceration (DM). DIC optimization was performed by studying the effects of pressure, temperature and processing time on oil yield. DIC + ASE obtained seed-oil yields of 615.9±0.5 against 555.5±0.5 g oil/kg-ddb for untextured seeds (RM). Via pressing, oil yields were 490.9±0.5 and 444.7±0.5 g oil/kg-ddb for textured and untextured seeds, respectively. Through coupling DIC (P: 0.63 MPa and t: 105 s) to the pressing extraction (60 s) of seeds along with 2h of DM of meals, it was possible to reach 605.8 g oil/kg ddb of oil yield. The same results were not obtained for RM seeds, where after 24 h of DM extraction, the oil yield was 554.7 g oil/kg ddb. DIC allowed for an increase in Camelina oil yields, reduced extraction time and valorized pressing meals.La tecnología de Descompresión Instantánea Controlada (DIC) fue evaluada como un pretratamiento para la extracción de aceite de Camelina sativa (L.). El pretratamiento DIC fue acoplado a la Extracción Acelerada de Disolventes (ASE), al Prensado y a la Maceración Dinámica (DM). La optimización de DIC fue llevada a cabo a través del estudio de los efectos de presión, temperatura y tiempo de proceso en el rendimiento del aceite. ASE + DIC permitió alcanzar rendimientos de 615,9±0,5 comparado con 555,5±0,5 g aceite/kg-ddb (base seca) en el caso de las semillas sin texturización (RM). En el caso del prensado, los rendimientos fueron de 490,9±0,5 y 444,7±0,5 g aceite/kg-ddb para las semillas con y sin texturización, respectivamente. Al acoplar el tratamiento DIC (P: 0.63 MPa y t: 105 s) + la extracción por prensado de las semillas (60 s) + 2h de DM de las harinas, fue posible alcanzar un rendimiento de 606,7 g aceite/ kg ddb. No así para las semillas sin tratamiento, en las que posterior a 24 h de extracción por DM, el rendimiento fue de 554,7 g oil/kg ddb. La texturización DIC permitió incrementar los rendimientos del aceite de Camelina, reducir los tiempos de extracción y valorizar las harinas del prensado
Unconventional motional narrowing in the optical spectrum of a semiconductor quantum dot
Motional narrowing refers to the striking phenomenon where the resonance line
of a system coupled to a reservoir becomes narrower when increasing the
reservoir fluctuation. A textbook example is found in nuclear magnetic
resonance, where the fluctuating local magnetic fields created by randomly
oriented nuclear spins are averaged when the motion of the nuclei is thermally
activated. The existence of a motional narrowing effect in the optical response
of semiconductor quantum dots remains so far unexplored. This effect may be
important in this instance since the decoherence dynamics is a central issue
for the implementation of quantum information processing based on quantum dots.
Here we report on the experimental evidence of motional narrowing in the
optical spectrum of a semiconductor quantum dot broadened by the spectral
diffusion phenomenon. Surprisingly, motional narrowing is achieved when
decreasing incident power or temperature, in contrast with the standard
phenomenology observed for nuclear magnetic resonance
Subnanosecond spectral diffusion measurement using photon correlation
Spectral diffusion is a result of random spectral jumps of a narrow line as a
result of a fluctuating environment. It is an important issue in spectroscopy,
because the observed spectral broadening prevents access to the intrinsic line
properties. However, its characteristic parameters provide local information on
the environment of a light emitter embedded in a solid matrix, or moving within
a fluid, leading to numerous applications in physics and biology. We present a
new experimental technique for measuring spectral diffusion based on photon
correlations within a spectral line. Autocorrelation on half of the line and
cross-correlation between the two halves give a quantitative value of the
spectral diffusion time, with a resolution only limited by the correlation
set-up. We have measured spectral diffusion of the photoluminescence of a
single light emitter with a time resolution of 90 ps, exceeding by four orders
of magnitude the best resolution reported to date
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