Quantum turnstile operation of single-molecule magnets

The time-dependent transport through single-molecule magnets coupled to magnetic or non-magnetic electrodes is studied in the framework of the generalized master equation method. We investigate the transient regime induced by the periodic switching of the source and drain contacts. If the electrodes have opposite magnetizations the quantum turnstile operation allows the stepwise writing of intermediate excited states. In turn, the transient currents provide a way to read these states. Within our approach we take into account both the uniaxial and transverse anisotropy. The latter may induce additional quantum tunneling processes which affect the efficiency of the proposed read-and-write scheme. An equally weighted mixture of molecular spin states can be prepared if one of the electrodes is ferromagnetic.Comment: 19 pages, 6 figure

Superconductivity and Physical Properties of CaPd2Ge2 Single Crystals

We present the superconducting and normal state properties of CaPd2Ge2 single crystal investigated by magnetic susceptibility \chi, isothermal magnetization M, heat capacity C_p, in-plane electrical resistivity \rho and London penetration depth \lambda versus temperature T and magnetic field H measurements. Bulk superconductivity is inferred from the \rho(T) and C_p(T) data. The \rho(T) data exhibit metallic behavior and undergoes a superconducting transition with T_c onset = 1.98 K and zero resistivity state at T_c 0 = 1.67 K. The \chi(T) reveal the onset of superconductivity at 2.0 K. For T>2.0 K, the \chi(T) and M(H) are weakly anisotropic paramagnetic with \chi_ab > \chi_c. The C_p(T) confirm the bulk superconductivity below T_c = 1.69(3) K. The superconducting state electronic heat capacity is analyzed within the framework of a single-band \alpha-model of BCS superconductivity and various normal and superconducting state parameters are estimated. Within the \alpha-model, the C_p(T) data and the ab plane \lambda(T) data consistently indicate a moderately anisotropic s-wave gap with \Delta(0)/k_B T_c ~ 1.6, somewhat smaller than the BCS value of 1.764. The relationship of the heat capacity jump at T_c and the penetration depth measurement to the anisotropy in the s-wave gap is discussed.Comment: 12 pages, 9 figures, 2 Tables; Submitted to PR

Effects of screening on the two-dimensional electron transport properties in modulation doped heterostructures

Cataloged from PDF version of article.The effects of screening on the polar optical phonon scattering rates and on the transport properties of the two-dimensional electron gas in AlGaAs/GaAs modulation doped heterostructures have been investigated through Monte Carlo simulations incorporating the three valleys of the conduction band, size quantization in the Gamma valley and the lowest three subbands in the quantum-well. At typical sheet densities observed in modulation doped field-effect transistors, screening considerably affects the electron transport properties under moderately large fields and at low temperatures, by lowering the intrasubband polar-optical phonon scattering rates especially in the first subband. The results show that screening, which is usually ignored in device Monte Carlo simulations, should be included in the simulation in order to be able to predict the device performance correctly. (C) 1998 Elsevier Science Ltd. All rights reserved

Wiedemann-Franz law and non-vanishing temperature scale across the field-tuned quantum critical point of YbRh2Si2

The in-plane thermal conductivity kappa(T) and electrical resistivity rho(T) of the heavy-fermion metal YbRh2Si2 were measured down to 50 mK for magnetic fields H parallel and perpendicular to the tetragonal c axis, through the field-tuned quantum critical point, Hc, at which antiferromagnetic order ends. The thermal and electrical resistivities, w(T) and rho(T), show a linear temperature dependence below 1 K, typical of the non-Fermi liquid behavior found near antiferromagnetic quantum critical points, but this dependence does not persist down to T = 0. Below a characteristic temperature T* ~ 0.35 K, which depends weakly on H, w(T) and rho(T) both deviate downward and converge in the T = 0 limit. We propose that T* marks the onset of short-range magnetic correlations, persisting beyond Hc. By comparing samples of different purity, we conclude that the Wiedemann-Franz law holds in YbRh2Si2, even at Hc, implying that no fundamental breakdown of quasiparticle behavior occurs in this material. The overall phenomenology of heat and charge transport in YbRh2Si2 is similar to that observed in the heavy-fermion metal CeCoIn5, near its own field-tuned quantum critical point.Comment: 8 figures, 8 page

Dynamical screening effects in hot-electron scattering from electron-hole plasma and LO-phonon modes in quantum wires

Cataloged from PDF version of article.We present a fully dynamical and finite temperature study of the hot-electron momentum relaxation rate and the power loss in a coupled system of electron-hole plasma and bulk LO-phonons in a quantum wire structure. Interactions of the scattered electron with neutral plasma components and phonons are treated on an equal footing within the random-phase approximation. Coupled mode effects substantially change the transport properties of the system at low temperatures. Particularly, the ''plasmon-like'' and ''LO-phonon-like'' excitations yield comparable rates which, as a consequence of the singular nature of the 1D density of states, can be large at the threshold. This is in contrast to room temperature results where only the LO-phonon mode contributes significantly to the rate. The density and temperature dependence of the power loss reveals that dynamical screening effects are important, and energy-momentum conservation cannot be satisfied above a certain density for a given initial energy. Copyright (C) 1996 Elsevier Science Lt

Interplay between superconductivity and itinerant magnetism in underdoped Ba1−x_{1-x}Kx_xFe2_2As2_2 (x=x= 0.2) probed by the response to controlled point-like disorder

The response of superconductors to controlled introduction of point-like disorder is an important tool to probe their microscopic electronic collective behavior. In the case of iron-based superconductors (IBS), magnetic fluctuations presumably play an important role in inducing high temperature superconductivity. In some cases, these two seemingly incompatible orders coexist microscopically. Therefore, understanding how this unique coexistence state is affected by disorder can provide important information about the microscopic mechanisms involved. In one of the most studied pnictide family, hole-doped Ba$_{1-x}$K$_x$Fe$_2$As$_2$ (BaK122), this coexistence occurs over a wide range of doping levels, 0.16~$\lesssim x \lesssim$~0.25. We used relativistic 2.5 MeV electrons to induce vacancy-interstitial (Frenkel) pairs that act as efficient point-like scattering centers. Upon increasing dose of irradiation, the superconducting transition temperature $T_c$ decreases dramatically. In the absence of nodes in the order parameter this provides a strong support for a sign-changing $s_{\pm}$ pairing. Simultaneously, in the normal state, there is a strong violation of the Matthiessen's rule and a decrease (surprisingly, at the same rate as $T_c$) of the magnetic transition temperature $T_{sm}$, which indicates the itinerant nature of the long-range magnetic order. Comparison of the hole-doped BaK122 with electron-doped Ba(Fe$_x$Co$_{1-x}$)$_2$As$_2$ (FeCo122) with similar $T_{sm}\sim$110~K, $x=$0.02, reveals significant differences in the normal states, with no apparent Matthiessen's rule violation above $T_{sm}$ on the electron-doped side. We interpret these results in terms of the distinct impact of impurity scattering on the competing itinerant antiferromagnetic and $s_{\pm}$ superconducting orders