1,026 research outputs found
Origin of Rashba-splitting in the quantized subbands at Bi2Se3 surface
We study the band structure of the topological
insulator (111) surface using angle-resolved photoemission spectroscopy. We
examine the situation where two sets of quantized subbands exhibiting different
Rashba spin-splitting are created via bending of the conduction (CB) and the
valence (VB) bands at the surface. While the CB subbands are strongly Rashba
spin-split, the VB subbands do not exhibit clear spin-splitting. We find that
CB and VB experience similar band bending magnitudes, which means, a
spin-splitting discrepancy due to different surface potential gradients can be
excluded. On the other hand, by comparing the experimental band structure to
first principles LMTO band structure calculations, we find that the strongly
spin-orbit coupled Bi 6 orbitals dominate the orbital character of CB,
whereas their admixture to VB is rather small. The spin-splitting discrepancy
is, therefore, traced back to the difference in spin-orbit coupling between CB
and VB in the respective subbands' regions
Interplay Between Yu-Shiba-Rusinov States and Multiple Andreev Reflections
Motivated by recent scanning tunneling microscopy experiments on single
magnetic impurities on superconducting surfaces, we present here a
comprehensive theoretical study of the interplay between Yu-Shiba-Rusinov bound
states and (multiple) Andreev reflections. Our theory is based on a combination
of an Anderson model with broken spin degeneracy and nonequilibrium Green's
function techniques that allows us to describe the electronic transport through
a magnetic impurity coupled to superconducting leads for arbitrary junction
transparency. Using this combination we are able to elucidate the different
tunneling processes that give a significant contribution to the subgap
transport. In particular, we predict the occurrence of a large variety of
Andreev reflections mediated by Yu-Shiba-Rusinov bound states that clearly
differ from the standard Andreev processes in non-magnetic systems. Moreover,
we provide concrete guidelines on how to experimentally identify the subgap
features originating from these tunneling events. Overall, our work provides
new insight into the role of the spin degree of freedom in Andreev transport
physics.Comment: 15 pages, 10 figure
Tracking primary thermalization events in graphene with photoemission at extreme timescales
Direct and inverse Auger scattering are amongst the primary processes that
mediate the thermalization of hot carriers in semiconductors. These two
processes involve the annihilation or generation of an electron-hole pair by
exchanging energy with a third carrier, which is either accelerated or
decelerated. Inverse Auger scattering is generally suppressed, as the
decelerated carriers must have excess energies higher than the band gap itself.
In graphene, which is gapless, inverse Auger scattering is instead predicted to
be dominant at the earliest time delays. Here, femtosecond
extreme-ultraviolet pulses are used to detect this imbalance, tracking both the
number of excited electrons and their kinetic energy with time- and
angle-resolved photoemission spectroscopy. Over a time window of approximately
25 fs after absorption of the pump pulse, we observe an increase in conduction
band carrier density and a simultaneous decrease of the average carrier kinetic
energy, revealing that relaxation is in fact dominated by inverse Auger
scattering. Measurements of carrier scattering at extreme timescales by
photoemission will serve as a guide to ultrafast control of electronic
properties in solids for PetaHertz electronics.Comment: 16 pages, 8 figure
Unusual electronic ground state of a prototype cuprate: band splitting of single CuO_2-plane Bi_2 Sr_(2-x) La_x CuO_(6+delta)
By in-situ change of polarization a small splitting of the Zhang-Rice singlet
state band near the Fermi level has been resolved for optimum doped (x=0.4)
BiSrLaCuO at the (pi,0)-point (R.Manzke et al.
PRB 63, R100504 (2001). Here we treat the momentum dependence and lineshape of
the split band by photoemission in the EDC-mode with very high angular and
energy resolution. The splitting into two destinct emissions could also be
observed over a large portion of the major symmetry line M, giving the
dispersion for the individual contributions. Since bi-layer effects can not be
present in this single-layer material the results have to be discussed in the
context of one-particle removal spectral functions derived from current
theoretical models. The most prominent are microscopic phase separation
including striped phase formation, coexisting antiferromagnetic and
incommensurate charge-density-wave critical fluctuations coupled to electrons
(hot spots) or even spin charge separation within the Luttinger liquid picture,
all leading to non-Fermi liquid like behavior in the normal state and having
severe consequences on the way the superconducting state forms. Especially the
possibilty of observing spinon and holon excitations is discussed.Comment: 5 pages, 4 figure
Charge Stripping Reactions in Mass Spectrometry: A Study of Diatomic and Triatomic Inorganic and Organic Ions
Charge stripping reactions of the type m• + N--+ m2• + N + ehave
been studied for a variety of diatomic and triatomic inorganic
and organic ions. Ionisation energies of the m• ions, IE (m+--+ m2• ),
have been determined, most of them for the first time. The method
is fast and straightforward; it is applicable to both molecular and
fragment .ions. The relative cross-sections for the charge stripping
processes have been also determined; they show llrge variations
from one species to another. Cases of possible interferences, which
are fairly infrequent, are described and discussed
The Use of Renewable and Alternative Fuel in the Heavy Clay Industry
Abstract The heavy clay industry brick is in many countries a very important economic factor with far reaching financial and environmental impacts. In the industrialized countries the use of alternative fuels in the heavy clay industry is rather limited.The European brick industries common current research activity is mainly focused on synthgas from waste streams. In-house research activity by single brick companies does, at least in Europe, not take place at the moment. The situation in the developing and industrializing countries is far different: The use of alternative,fossil and renewable, fuels in these countries is still wide spread. The use of such fuels does sometimes have severe negative impacts on the environment. This paper gives an overview of the use of various renewable and alternative fuels in the heavy clay industry in several countries and the environmental and financial impacts these fuels have or might have on the operation of a typical installation in various parts of the world (Maghreb, Europe, USA, Australia,India, Vietnam). Two examples in which alternative fuels have been or are used, one in an industrializing and one in an industrialized country, are briefly presented. A comparative product life cycle analysis, LCA, is presented
Hidden one-dimensional electronic structure and non-Fermi liquid angle resolved photoemission line shapes of -MoO
We report angle resolved photoemission (ARPES) spectra of
-MoO, a layered metal that undergoes two charge density wave
(CDW) transitions at 109 K and 30 K. We have directly observed the ``hidden
one-dimensional (hidden-1d)'' Fermi surface and an anisotropic gap opening
associated with the 109 K transition, in agreement with the band theoretical
description of the CDW transition. In addition, as in other hidden-1d materials
such as NaMoO, the ARPES line shapes show certain anomalies, which
we discuss in terms of non-Fermi liquid physics and possible roles of disorder.Comment: 3 figures; Erratum added to include missed reference
Tuning independently Fermi energy and spin splitting in Rashba systems: Ternary surface alloys on Ag(111)
By detailed first-principles calculations we show that the Fermi energy and
the Rashba splitting in disordered ternary surface alloys (BiPbSb)/Ag(111) can
be independently tuned by choosing the concentrations of Bi and Pb. The
findings are explained by three fundamental mechanisms, namely the relaxation
of the adatoms, the strength of the atomic spin-orbit coupling, and band
filling. By mapping the Rashba characteristics,i.e.the splitting and the Rashba
energy, and the Fermi energy of the surface states in the complete range of
concentrations. Our results suggest to investigate experimentally effects which
rely on the Rashba spin-orbit coupling in dependence on spin-orbit splitting
and band filling.Comment: 11 pages, 3 figure
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