544 research outputs found
Influence of Domain Wall on Magnetocaloric Effect in GdPt
The resistivity, magnetoresistance and in-field heat capacity measurements
were performed on GdPt intermetallic compound. The magnetocaloric
parameters and were derived from the in-field heat
capacity data. Comparison has been made between the magnetocaloric effect
and difference in resistivity
as a function of temperature. There is distinct difference in the temperature
dependence of and below the ferromagnetic transition
temperature. However after removing the domain wall contribution from , the nature of and dependence as a function of
temperature are similar. Our observation indicates that the domain wall
contribution in magnetocaloric effect is negligible in spite of the fact that
it has significant contribution in magnetotransport.Comment: RevTex 4 pages, 6 figure
Geometrical effects on spin injection: 3D spin drift diffusion model
We discuss a three-dimensional (3D) spin drift diffusion (SDD) model to
inject spin from a ferromagnet (FM) to a normal metal (N) or semiconductor
(SC). Using this model we investigate the problem of spin injection into
isotropic materials like GaAs and study the effect of FM contact area and SC
thickness on spin injection. We find that in order to achieve detectable spin
injection a small contact area or thick SC samples are essential for direct
contact spin injection devices. We investigate the use of thin metal films (Cu)
proposed by S.B. Kumar et al. and show that they are an excellent substitute
for tunnelling barriers (TB) in the regime of small contact area. Since most
tunnelling barriers are prone to pinhole defects, we study the effect of
pinholes in AlO tunnelling barriers and show that the reduction in the
spin-injection ratio () is solely due to the effective area of the
pinholes and there is no correlation between the number of pinholes and the
spin injection ratio.Comment: 5 pages, 6 figures. Accepted by JA
Photoemission investigation of the electronic structure of Fe-Pd and Fe-Pt alloys
A photoemission investigation of Fe-Pd and Fe-Pt transition-metal alloys, using ∼50–150-eV synchrotron radiation, is presented. We consider in particular the spectral distribution of Fe states when approaching the dilute limit. By means of the Cooper minimum in the 4d and 5d photoionization cross section, we identify structures that have mainly Fe minority- or Fe majority-spin character. The relative position of these peaks is discussed in terms of the covalent interaction between Fe 3d and Pd or Pt d states. Also, the strong resemblance between the distribution of Fe states in the Pd-based and in the Pt-based alloys is demonstrated. We find a consistent behavior of interacting d states towards the dilute limit. It is concluded that the Fe states that are observed in the photoemission spectra of the dilute alloys have mainly majority-spin character and are, because of the covalent interaction with host states, widely distributed over the energy range of the host d band. The Fe minority-spin band, which is centered near the Fermi level, gradually empties with increasing Fe dilution
Origin of Middle-Infrared Peaks in Cerium Compounds
We have demonstrated that the middle-infrared (mid-IR) peaks in the optical
conductivity spectra of Ce ( = Pd, Sn, In) can be explained by
first-principle band structure calculation with the spin-orbit interaction. The
mid-IR peak shapes in these materials are not identical to one another:
CePd, CeSn, and CeIn have a triple-peak structure, double-peak
structure and broad single-peak structure, respectively. These peaks can be
theoretically explained by the optical transition from the occupied state to
the spin-orbit splitted Ce state. This result indicates that the mid-IR
peaks originate from the simple band picture with the Ce state near the
Fermi level, not from the conventional cf hybridization gap based on the
periodic Anderson model.Comment: 5 pages, 6 figures. To be published in J. Phys. Soc. Jpn. 78(1)
(2009
Ab initio exchange interactions and magnetic properties of Gd2Fe17 iron sublattice: rhombohedral vs. hexagonal phases
In the framework of the LSDA+U method electronic structure and magnetic
properties of the intermetallic compound Gd2Fe17 for both rhombohedral and
hexagonal phases have been calculated. On top of that, ab initio exchange
interaction parameters within the Fe sublattice for all present nearest and
some next nearest Fe ions have been obtained. It was found that for the first
coordination sphere direct exchange interaction is ferromagnetic. For the
second coordination sphere indirect exchange interaction is observed to be
weaker and of antiferromagnetic type. Employing the theoretical values of
exchange parameters Curie temperatures Tc of both hexagonal and rhombohedral
phases of Gd2Fe17 within Weiss mean-field theory were estimated. Obtained
values of Tc and its increase going from the hexagonal to rhombohedral crystal
structure of Gd2Fe17 agree well with experiment. Also for both structures
LSDA+U computed values of total magnetic moment coincide with experimental
ones.Comment: 20 pages, 2 figures; V2 as published in PR
Change of Magnetic Properties of Th₂Fe₁₇ Due to Interstitial Solution of C and N
The changes in magnetic and crystallographic properties in the series Th2Fe17Cx and Th2Fe 17Nx have been studied. The changes in the latter series were also studied by 57Fe Mössbauer spectroscopy. The ultimate enhancements of the saturation moments in these series are 13% and 24%, respectively. This is much larger than observed previously in the corresponding rare-earth compounds, although the Curie temperature enhancements are of comparable magnitude. In the Th-Fe-C system a novel compound of the BaCd 11 type was found, having a Curie temperature around 370 K
Why the iron magnetization in Gd2Fe14B and the spontaneous magnetization of Y2Fe14B depend on temperature differently
This article may be downloaded for personal use only. Any other use requires prior permission of the author and the American Institute of Physics.It is demonstrated that the temperature dependence of the iron sublattice magnetization in Gd2Fe14B is affected significantly by the Gd-Fe exchange interaction. This is at variance with the common perception that MFe(T) in iron-rich rare-earth intermetallics is determined predominantly by the Fe-Fe exchange. This phenomenon is discussed by considering the modification of the low-energy spin-wave spectrum of Gd2Fe14B, as compared to that of Y2Fe14B, under the influence of the Gd-Fe interaction. The result is of particular significance for evaluating the temperature dependence of the magnetocrystalline anisotropy of iron or cobalt compounds with anisotropic rare earths (e.g., Nd2Fe14B) and in turn, of the hard magnetic properties of such compounds
Can antiferromagnetism and superconductivity coexist in the high-field paramagnetic superconductor Nd(O,F)FeAs?
We present measurements of the temperature and field dependencies of the
magnetization M(T,H) of Nd(O0.89F0.11)FeAs at fields up to 33T, which show that
superconductivity with the critical temperature Tc ~ 51K cannot coexist with
antiferromagnetic ordering. Although M(T,H) at 55 < T < 140K exhibits a clear
Curie-Weiss temperature dependence corresponding to the Neel temperature TN ~
11-12K, the behavior of M(T,H) below Tc is only consistent with either
paramagnetism of weakly interacting magnetic moments or a spin glass state. We
suggest that the anomalous magnetic behavior of an unusual high-field
paramagnetic superconductor Nd(O1-xFx)FeAs is mostly determined by the magnetic
Nd ions.Comment: 4 pages, 4 figure
Geometric, electronic, and magnetic structure of CoFeSi: Curie temperature and magnetic moment measurements and calculations
In this work a simple concept was used for a systematic search for new
materials with high spin polarization. It is based on two semi-empirical
models. Firstly, the Slater-Pauling rule was used for estimation of the
magnetic moment. This model is well supported by electronic structure
calculations. The second model was found particularly for Co based Heusler
compounds when comparing their magnetic properties. It turned out that these
compounds exhibit seemingly a linear dependence of the Curie temperature as
function of the magnetic moment. Stimulated by these models, CoFeSi was
revisited. The compound was investigated in detail concerning its geometrical
and magnetic structure by means of X-ray diffraction, X-ray absorption and
M\"o\ss bauer spectroscopies as well as high and low temperature magnetometry.
The measurements revealed that it is, currently, the material with the highest
magnetic moment () and Curie-temperature (1100K) in the classes of
Heusler compounds as well as half-metallic ferromagnets. The experimental
findings are supported by detailed electronic structure calculations
Geometrical quadrupolar frustration in DyB
Physical properties of DyB have been studied by magnetization, specific
heat, and ultrasonic measurements. The magnetic entropy change and the
ultrasonic properties in the intermediate phase II indicate that the degeneracy
of internal degrees of freedom is not fully lifted in spite of the formation of
magnetic order. The ultrasonic attenuation and the huge softening of
in phase II suggests existence of electric-quadrupolar (orbital) fluctuations
of the 4-electron. These unusual properties originate from the geometrical
quadrupolar frustration.Comment: 4 pages, 4 figures, accepted for publication in Journal of the
Physical Society of Japa
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