15 research outputs found
Erratum: "Nucleation and growth of nickel nanoclusters on graphene Moiré on Rh(111)" [Appl. Phys. Lett. 96, 093115 (2010)an]
Andreev experiments on superconductor/ferromagnet point contacts
Andreev reflection is a smart tool to investigate the spin polarization P of the current through point contacts
between a superconductor and a ferromagnet. We compare different models to extract P from experimental data
and investigate the dependence of P on different contact parameters
Andreev experiments on superconductor/ferromagnet point contacts
Andreev reflection is a smart tool to investigate the spin polarisation P of
the current through point contacts between a superconductor and a ferromagnet.
We compare different models to extract P from experimental data and investigate
the dependence of P on different contact parameters.Comment: 14 pages, 5 figures, accepted for publication in Fizika Nizkikh
Temperatu
Nucleation and growth of nickel nanoclusters on graphene Moiré on Rh (111)
Regularly sized Ni nanoclusters (NCs) have been grown on a graphene Moiré on Rh(111). Using scanning tunneling microscopy, we determine that initial growth of Ni at 150 K leads to preferential nucleation of monodispersed NCs at specific sites of the Moiré superstructure. However, a defined long-range ordering of NCs with increasing coverage is not observed. Room temperature Ni deposition leads to the formation of flat triangular-shaped islands which are well-matched to the Moiré registry
Erratum: “Nucleation and growth of nickel nanoclusters on graphene Moiré on Rh(111)” [Appl. Phys. Lett. 96, 093115 (2010)an]
In Situ Fabrication Of Quasi-Free-Standing Epitaxial Graphene Nanoflakes On Gold
Addressing the multitude of electronic phenomena theoretically predicted for confined graphene structures requires appropriate in situ fabrication procedures yielding graphene nanoflakes (GNFs) with well-defined geometries and accessible electronic properties. Here, we present a simple strategy to fabricate quasi-free-standing GNFs of variable sizes, performing temperature programmed growth of graphene flakes on the Ir(111) surface and subsequent intercalation of gold. Using scanning tunneling microscopy (STM), we show that epitaxial GNFs on a perfectly ordered Au(111) surface are formed while maintaining an unreconstructed, singly hydrogen-terminated edge structure, as confirmed by the accompanying density functional theory (DFT) calculations. Using tip-induced lateral displacement of GNFs, we demonstrate that GNFs on Au(111) are to a large extent decoupled from the Au(111) substrate. The direct accessibility of the electronic states of a single GNF is demonstrated upon analysis of the quasiparticle interference patterns obtained by low-temperature STM. These findings open up an interesting playground for diverse investigations of graphene nanostructures with possible implications for device fabrication
Size-Selected Epitaxial Nanoislands Underneath Graphene Moiré on Rh(111)
We use in situ scanning tunneling microscopy (STM) to investigate intercalation of the ferromagnetic 3d metals Ni and Fe underneath a graphene monolayer on Rh(111). Upon thermal annealing of graphene/Rh(111) with the deposited metal on top, we observe the formation of epitaxial monatomic nanoislands grown pseudomorphically on Rh(111) and covered by graphene. The size and shape of intercalated nanoislands is strongly influenced by the local spatial variation of the graphene–Rh bonding strength. In particular, the side length of the intercalated nanoislands shows maxima around discrete values imposed by the periodicity of the graphene moiré. Intercalation can be performed efficiently and without any visible damage of the graphene overlayer in the studied temperature range between 670 and 870 K. We identify the main intercalation path to be via diffusion through pre-existing lattice defects in graphene, accompanied by the second mechanism which is based on the material diffusion via metal-generated defects followed by the defect healing of the graphene lattice. We deem these graphene-capped and sharply confined ferromagnetic nanoislands interesting in the fields of spintronics and nanomagnetism
<i>In Situ</i> Fabrication Of Quasi-Free-Standing Epitaxial Graphene Nanoflakes On Gold
Addressing the multitude of electronic phenomena theoretically predicted for confined graphene structures requires appropriate <i>in situ</i> fabrication procedures yielding graphene nanoflakes (GNFs) with well-defined geometries and accessible electronic properties. Here, we present a simple strategy to fabricate quasi-free-standing GNFs of variable sizes, performing temperature programmed growth of graphene flakes on the Ir(111) surface and subsequent intercalation of gold. Using scanning tunneling microscopy (STM), we show that epitaxial GNFs on a perfectly ordered Au(111) surface are formed while maintaining an unreconstructed, singly hydrogen-terminated edge structure, as confirmed by the accompanying density functional theory (DFT) calculations. Using tip-induced lateral displacement of GNFs, we demonstrate that GNFs on Au(111) are to a large extent decoupled from the Au(111) substrate. The direct accessibility of the electronic states of a single GNF is demonstrated upon analysis of the quasiparticle interference patterns obtained by low-temperature STM. These findings open up an interesting playground for diverse investigations of graphene nanostructures with possible implications for device fabrication
The local magnetic properties of [Mn<sup>III</sup><sub>6</sub> Cr<sup>III</sup>]<sup>3+</sup> and [Fe<sup>III</sup><sub>6</sub> Cr<sup>III</sup>]<sup>3+</sup> single-molecule magnets deposited on surfaces studied by spin-polarized photoemission and XMCD with circularly polarized synchrotron radiation
Heinzmann U, Helmstedt A, Dohmeier N, et al. The local magnetic properties of [(Mn6CrIII)-Cr-III](3+) [ and [(Fe6CrIII)-Cr-III](3+) single-molecule magnets deposited on surfaces studied by spin-polarized photoemission and XMCD with circularly polarized synchrotron radiation. In: Collisions involving condensed matter [Abstracts]. Journal of Physics Conference Series. Vol 488. Bristol: Iop Publishing; 2014.It is demonstrated that local magnetic moments of single molecule magnets (SMM) normally studied by XMCD at very low temperatures and high magnetic fields can be measured by means of spin-resolved electron emission in the paramagnetic phase at room temperature by use of circularly polarized radiation