1,109 research outputs found
Quantum shot-noise at local tunneling contacts on mesoscopic multiprobe conductors
New experiments that measure the low-frequency shot-noise spectrum at local
tunneling contacts on mesoscopic structures are proposed. The current
fluctuation spectrum at a single tunneling tip is determined by local partial
densities of states. The current-correlation spectrum between two tunneling
tips is sensitive to non-diagonal density of states elements which are
expressed in terms of products of scattering states of the conductor. Thus such
an experiment permits to investigate correlations of electronic wave functions.
We present specific results for a clean wire with a single barrier and for
metallic diffusive conductors.Comment: 4 pages REVTeX, 2 figure
Carbon fibre tips for scanning probe microscopy based on quartz tuning fork force sensors
We report the fabrication and the characterization of carbon fibre tips for
their use in combined scanning tunnelling and force microscopy based on
piezoelectric quartz tuning fork force sensors. We find that the use of carbon
fibre tips results in a minimum impact on the dynamics of quartz tuning fork
force sensors yielding a high quality factor and consequently a high force
gradient sensitivity. This high force sensitivity in combination with high
electrical conductivity and oxidation resistance of carbon fibre tips make them
very convenient for combined and simultaneous scanning tunnelling microscopy
and atomic force microscopy measurements. Interestingly, these tips are quite
robust against occasionally occurring tip crashes. An electrochemical
fabrication procedure to etch the tips is presented that produces a sub-100 nm
apex radius in a reproducible way which can yield high resolution images.Comment: 14 pages, 10 figure
Dynamic image potential at an Al(111) surface
We evaluate the electronic self-energy Sigma(E) at an Al(111) surface using the GW space-time method. This self-energy automatically includes the image potential V-im not present in any local-density approximation for exchange and correlation. We solve the energy-dependent quasiparticle equations and calculate the effective local potential experienced by electrons in the near-surface region. The relative contribution of exchange proves to be very different for states above the Fermi level. The image-plane position for interacting electrons is closer to the surface than for the purely electrostatic effects felt by test charges, and, like its classical counterpart, is drawn inwards by the effects of atomic structure
Investigation of the (001) cleavage plane of potassium bromide with an atomic force microscope at 4.2 K in ultra-high vacuum
We have imaged the (001) surface of KBr with a UHV atomic force microscope at 4.2 K and 300 K. The sample was prepared by cleaving it in UHV along the (001) plane. We achieved atomic resolution at 4.2 K and resolved both the potassium and the bromium ions. We show atomically resolved images of flat terraces as large as 25 nm by 25 nm. Force-versus-distance measurements were taken, and the influence of the loading force acting between sample and cantilever on the appearance of friction effects and sample damage was studied
Theory for an electrostatic imaging mechanism allowing atomic resolution of ionic crystals by atomic force microscopy
An electrostatic imaging mechanism is presented which allows atomic resolution of the surface of ionic crystals by atomic force microscopy (AFM). In the x-y plane the electrostatic field due to the ion charges reflects the periodicity of the surface lattice. If the tip of the AFM stylus is polarizable, an attractive force between tip and sample will exist and allow imaging of the surface in a noncontact mode. It is shown that the decay length of the electrostatic interaction in the z direction is sufficiently short for atomic resolution to be achieved not only with a hypothetical tip consisting of only one atom but also by a more realistic tip of parabolic shape with a radius of 30 nm. The theory is applied to the (001) surface of KBr
Static and dynamic properties of frictional phenomena in a one-dimensional system with randomness
Static and dynamic frictional phenomena at the interface with random
impurities are investigated in a two-chain model with incommensurate structure.
Static frictional force is caused by the impurity pinning and/or by the pinning
due to the regular potential, which is responsible for the breaking of
analyticity transition for impurity-free cases. It is confirmed that the static
frictional force is always finite in the presence of impurities, in contrast to
the impurity-free system. The nature of impurity pinning is discussed in
connection with that in density waves. The kinetic frictional force of a steady
sliding state is also investigated numerically. The relationship between the
sliding velocity dependence of the kinetic frictional force and the strength of
impurity potential is discussed.Comment: RevTex, 14 pages, 6 PostScript figures, to appear in Phys. Rev.
Folding of a donor–acceptor polyrotaxane by using noncovalent bonding interactions
Mechanically interlocked compounds, such as bistable catenanes and bistable rotaxanes, have been used to bring about actuation in nanoelectromechanical systems (NEMS) and molecular electronic devices (MEDs). The elaboration of the structural features of such rotaxanes into macromolecular materials might allow the utilization of molecular motion to impact their bulk properties. We report here the synthesis and characterization of polymers that contain π electron-donating 1,5-dioxynaphthalene (DNP) units encircled by cyclobis(paraquat-p-phenylene) (CBPQT4+), a π electron-accepting tetracationic cyclophane, synthesized by using the copper(I)-catalyzed azide-alkyne cycloaddition (CuAAC). The polyrotaxanes adopt a well defined “folded” secondary structure by virtue of the judicious design of two DNP-containing monomers with different binding affinities for CBPQT4+. This efficient approach to the preparation of polyrotaxanes, taken alongside the initial investigations of their chemical properties, sets the stage for the preparation of a previously undescribed class of macromolecular architectures
Theory of oscillations in the STM conductance resulting from subsurface defects (Review Article)
In this review we present recent theoretical results concerning
investigations of single subsurface defects by means of a scanning tunneling
microscope (STM). These investigations are based on the effect of quantum
interference between the electron partial waves that are directly transmitted
through the contact and the partial waves scattered by the defect. In
particular, we have shown the possibility imaging the defect position below a
metal surface by means of STM. Different types of subsurface defects have been
discussed: point-like magnetic and non-magnetic defects, magnetic clusters in a
nonmagnetic host metal, and non-magnetic defects in a s-wave superconductor.
The effect of Fermi surface anisotropy has been analyzed. Also, results of
investigations of the effect of a strong magnetic field to the STM conductance
of a tunnel point contact in the presence of a single defect has been
presented.Comment: 31 pages, 10 figuers Submitted to Low. Temp. Phy
Probing the shape of atoms in real space
The structure of single atoms in real space is investigated by scanning
tunneling microscopy. Very high resolution is possible by a dramatic reduction
of the tip-sample distance. The instabilities which are normally encountered
when using small tip-sample distances are avoided by oscillating the tip of the
scanning tunneling microscope vertically with respect to the sample. The
surface atoms of Si(111)-(7 x 7) with their well-known electronic configuration
are used to image individual samarium, cobalt, iron and silicon atoms. The
resulting images resemble the charge density corresponding to 4f, 3d and 3p
atomic orbitals.Comment: Submitted to Phys. Rev. B, 17 pages, 7 figure
A low‐temperature atomic force/scanning tunneling microscope for ultrahigh vacuum
We have built an ultrahigh vacuum atomic force/scanning tunneling microscope that works at 4.2 K. The microscope is incorporated into a very small chamber (100 ml) which can be evacuated and baked to UHV within a few hours by a specially designed valve. The instrument is about 20×20×70 mm3 in size and sturdy enough to operate without vibration isolation. The deflection of a microfabricated cantilever is detected by electron tunneling. Preliminary results show atomic resolution of HOPG in the STM mode and steps in KBr that range from one to four lattice constants in height at UHV conditions and 4.2 K
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