392 research outputs found
Cationic ordering control of magnetization in Sr2FeMoO6 double perovskite
The role of the synthesis conditions on the cationic Fe/Mo ordering in
Sr2FeMoO6 double perovskite is addressed. It is shown that this ordering can be
controlled and varied systematically. The Fe/Mo ordering has a profound impact
on the saturation magnetization of the material. Using the appropriate
synthesis protocol a record value of 3.7muB/f.u. has been obtained. Mossbauer
analysis reveals the existence of two distinguishable Fe sites in agreement
with the P4/mmm symmetry and a charge density at the Fe(m+) ions significantly
larger than (+3) suggesting a Fe contribution to the spin-down conduction band.
The implications of these findings for the synthesis of Sr2FeMoO6 having
optimal magnetoresistance response are discussed.Comment: 9 pages, 4 figure
Growth and magnetic properties of multiferroic LaxBi1-xMnO3 thin films
A comparative study of LaxBi1-xMnO3 thin films grown on SrTiO3 substrates is reported. It is shown that these films grow epitaxially in a narrow pressure-temperature range. A detailed structural and compositional characterization of the films is performed within the growth window. The structure and the magnetization of this system are investigated. We find a clear correlation between the magnetization and the unit-cell volume that we ascribe to Bi deficiency and the resultant introduction of a mixed valence on the Mn ions. On these grounds, we show that the reduced magnetization of LaxBi1-xMnO3 thin films compared to the bulk can be explained quantitatively by a simple model, taking into account the deviation from nominal composition and the Goodenough-Kanamori-Anderson rules of magnetic interactions
Fractal dimension and size scaling of domains in thin films of multiferroic BiFeO3
We have analyzed the morphology of ferroelectric domains in very thin films
of multiferroic BiFeO3. Unlike the more common stripe domains observed in
thicker films BiFeO3 or in other ferroics, the domains tend not to be straight,
but irregular in shape, with significant domain wall roughening leading to a
fractal dimensionality. Also contrary to what is usually observed in other
ferroics, the domain size appears not to scale as the square root of the film
thickness. A model is proposed in which the observed domain size as a function
of film thickness can be directly linked to the fractal dimension of the
domains.Comment: 4 pages, 3 figure
Spin-polarized tunneling spectroscopy in tunnel junctions with half-metallic electrodes
We have studied the magnetoresistance (TMR) of tunnel junctions with
electrodes of La2/3Sr1/3MnO3 and we show how the variation of the conductance
and TMR with the bias voltage can be exploited to obtain a precise information
on the spin and energy dependence of the density of states. Our analysis leads
to a quantitative description of the band structure of La2/3Sr1/3MnO3 and
allows the determination of the gap delta between the Fermi level and the
bottom of the t2g minority spin band, in good agreement with data from
spin-polarized inverse photoemission experiments. This shows the potential of
magnetic tunnel junctions with half-metallic electrodes for spin-resolved
spectroscopic studies.Comment: To appear in Physical Review Letter
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