263 research outputs found
Ultrafast spin dynamics and critical behavior in half-metallic ferromagnet : Sr_2FeMoO_6
Ultrafast spin dynamics in ferromagnetic half-metallic compound Sr_2FeMoO_6
is investigated by pump-probe measurements of magneto-optical Kerr effect.
Half-metallic nature of this material gives rise to anomalous thermal
insulation between spins and electrons, and allows us to pursue the spin
dynamics from a few to several hundred picoseconds after the optical
excitation. The optically detected magnetization dynamics clearly shows the
crossover from microscopic photoinduced demagnetization to macroscopic critical
behavior with universal power law divergence of relaxation time for wide
dynamical critical region.Comment: 14 pages, 4 figures. Abstract and Figures 1 & 3 are correcte
Study of molecular spin-crossover complex Fe(phen)2(NCS)2 thin films
We report on the growth by evaporation under high vacuum of high-quality thin
films of Fe(phen)2(NCS)2 (phen=1,10-phenanthroline) that maintain the expected
electronic structure down to a thickness of 10 nm and that exhibit a
temperature-driven spin transition. We have investigated the current-voltage
characteristics of a device based on such films. From the space charge-limited
current regime, we deduce a mobility of 6.5x10-6 cm2/V?s that is similar to the
low-range mobility measured on the widely studied
tris(8-hydroxyquinoline)aluminium organic semiconductor. This work paves the
way for multifunctional molecular devices based on spin-crossover complexes
Efficient metallic spintronic emitters of ultrabroadband terahertz radiation
Terahertz electromagnetic radiation is extremely useful for numerous
applications such as imaging and spectroscopy. Therefore, it is highly
desirable to have an efficient table-top emitter covering the 1-to-30-THz
window whilst being driven by a low-cost, low-power femtosecond laser
oscillator. So far, all solid-state emitters solely exploit physics related to
the electron charge and deliver emission spectra with substantial gaps. Here,
we take advantage of the electron spin to realize a conceptually new terahertz
source which relies on tailored fundamental spintronic and photonic phenomena
in magnetic metal multilayers: ultrafast photo-induced spin currents, the
inverse spin-Hall effect and a broadband Fabry-P\'erot resonance. Guided by an
analytical model, such spintronic route offers unique possibilities for
systematic optimization. We find that a 5.8-nm-thick W/CoFeB/Pt trilayer
generates ultrashort pulses fully covering the 1-to-30-THz range. Our novel
source outperforms laser-oscillator-driven emitters such as ZnTe(110) crystals
in terms of bandwidth, terahertz-field amplitude, flexibility, scalability and
cost.Comment: 18 pages, 10 figure
Control of defect-mediated tunneling barrier heights in ultrathin MgO films
The impact of oxygen vacancies on local tunneling properties across
rf-sputtered MgO thin films was investigated by optical absorption spectroscopy
and conducting atomic force microscopy. Adding O to the Ar plasma during
MgO growth alters the oxygen defect populations, leading to improved local
tunneling characteristics such as a lower density of current hotspots and a
lower tunnel current amplitude. We discuss a defect-based potential landscape
across ultrathin MgO barriers.Comment: 4 pages, 4 figure
Nonequilibrium Magnetization Dynamics of Nickel
Ultrafast magnetization dynamics of nickel has been studied for different
degrees of electronic excitation, using pump-probe second-harmonic generation
with 150 fs/800 nm laser pulses of various fluences. Information about the
electronic and magnetic response to laser irradiation is obtained from sums and
differences of the SHG intensity for opposite magnetization directions. The
classical M(T)-curve can be reproduced for delay times larger than the electron
thermalization time of about 280 fs, even when electrons and lattice have not
reached thermal equilibrium. Further we show that the transient magnetization
reaches its minimum approx. 50 fs before electron thermalization is completed.Comment: 8 pages, 5 figures, revte
Multicolor two-photon light-sheet microscopy
International audienceTwo-photon microscopy is the most effective approach for deep-tissue fluorescence cellular imaging; however, its application to high-throughput or high-content imaging is often hampered by low pixel rates, challenging multicolor excitation and potential cumulative photodamage. To overcome these limitations, we extended our prior work and combined two-photon scanned light-sheet..
Observation of the spin-charge thermal isolation of ferromagnetic Ga_{0.94}Mn_{0.06}As by time-resolved magneto-optical measurement
The dynamics of magnetization under femtosecond optical excitation is studied
in a ferromagnetic semiconductor Ga_{0.94}Mn_{0.06}As with a time-resolved
magneto-optical Kerr effect measurement with two color probe beams. The
transient reflectivity change indicates the rapid rise of the carrier
temperature and relaxation to a quasi-thermal equilibrium within 1 ps, while a
very slow rise of the spin temperature of the order of 500ps is observed. This
anomalous behavior originates from the thermal isolation between the charge and
spin systems due to the spin polarization of carriers (holes) contributing to
ferromagnetism. This constitutes experimental proof of the half-metallic nature
of ferromagnetic Ga_{0.94}Mn_{0.06}As arising from double exchange type
mechanism originates from the d-band character of holes
Ultrafast Spin Dynamics in Nickel
The spin dynamics in Ni is studied by an exact diagonalization method on the
ultrafast time scale. It is shown that the femtosecond relaxation of the
magneto-optical response results from exchange interaction and spin-orbit
coupling. Each of the two mechanisms affects the relaxation process
differently. We find that the intrinsic spin dynamics occurs during about 10 fs
while extrinsic effects such as laser-pulse duration and spectral width can
slow down the observed dynamics considerably. Thus, our theory indicates that
there is still room to accelerate the spin dynamics in experiments.Comment: 4 pages, Latex, 4 postscript figure
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