10 research outputs found
Magnetic field-dependent interplay between incoherent and Fermi liquid transport mechanisms in low-dimensional tau phase organic conductors
We present an electrical transport study of the 2-dimensional (2D) organic
conductor tau-(P-(S,S)-DMEDT-TTF)_2(AuBr)_2(AuBr_2)_y (y = 0.75) at low
temperatures and high magnetic fields. The inter-plane resistivity rho_zz
increases with decreasing temperature, with the exception of a slight anomaly
at 12 K. Under a magnetic field B, both rho_zz and the in-plane resistivity
plane rho_xx show a pronounced negative and hysteretic magnetoresistance with
Shubnikov de Haas (SdH)oscillations being observed in some (high
quality)samples above 15 T. Contrary to the predicted single, star-shaped,
closed orbit Fermi surface from band structure calculations (with an expected
approximate area of 12.5% of A_FBZ), two fundamental frequencies F_l and F_h
are detected in the SdH signal. These orbits correspond to 2.4% and 6.8% of the
area of the first Brillouin zone(A_FBZ), with effective masses F_l = 4.0 +/-
0.5 and F_h = 7.3 +/- 0.1. The angular dependence, in tilted magnetic fields of
F_l and F_h, reveals the 2D character of the FS and Angular dependent
magnetoresistance (AMRO) further suggests a FS which is strictly 2-D where the
inter-plane hopping t_c is virtually absent or incoherent. The Hall constant
R_xy is field independent, and the Hall mobility increases by a factor of 3
under moderate magnetic fields. Our observations suggest a unique physical
situation where a stable 2D Fermi liquid state in the molecular layers are
incoherently coupled along the least conducting direction. The magnetic field
not only reduces the inelastic scattering between the 2D metallic layers, but
it also reveals the incoherent nature of interplane transport in the AMRO
spectrum. The apparent ferromagnetism of the hysteretic magnetoresistance
remains an unsolved problem.Comment: 33 pages, 11 figure
Underwater excimer laser ablation of polymers
In this paper, we study the photoablation kinetic of poly (ethylene terephthalate) (PET), polycarbonate (PC), polyimide (PI) and polystyrene (PS) in both air and water. Compared to the results obtained in air, we highlight the decrease of the ablation threshold (AT) of polyesters in contact with water as a function of polymer chemical structure. In order to check the expected hydrolytic reaction of polyesters near the ablation threshold, the chemical modification of the polymer surfaces, as well the composition of the ablation products, were investigated after irradiation near the fluence of ablation threshold in air (air-F t ) by X-ray photoelectron spectroscopy (XPS) and confocal Raman microspectroscopy. The morphology of polymers obtained by underwater irradiation and near the air-F t was also examined using scanning electron microscopy (SEM). To understand the process and its dynamics in contact with water, we consider the model of temperature at the polymer-water interface based on the semi-analytical solution of the transit heat-diffusion equation
Nine loci for ocular axial length identified through genome-wide association studies, including shared loci with refractive error
10.1016/j.ajhg.2013.06.016American Journal of Human Genetics932264-277AJHG