228 research outputs found
Electron-photon scattering mediated by localized plasmons: A quantitative analysis by eigen-response theory
We show that the scattering interaction between a high energy electron and a
photon can be strongly enhanced by different types of localized plasmons in a
non-trivial way. The scattering interaction is predicted by an eigen-response
theory, numerically verified by finite-difference-time-domain simulation, and
experimentally verified by cathodoluminescence spectroscopy. We find that the
scattering interaction associated with dark plasmons can be as strong as that
of bright plasmons. Such a strong interaction may offer new opportunities to
improve single-plasmon detection and high-resolution characterization
techniques for high quality plasmonic materials.Comment: 4 pages, 4 figures (excluding Supporting Information
Bias and temperature dependence of the 0.7 conductance anomaly in Quantum Point Contacts
The 0.7 (2e^2/h) conductance anomaly is studied in strongly confined, etched
GaAs/GaAlAs quantum point contacts, by measuring the differential conductance
as a function of source-drain and gate bias as well as a function of
temperature. We investigate in detail how, for a given gate voltage, the
differential conductance depends on the finite bias voltage and find a
so-called self-gating effect, which we correct for. The 0.7 anomaly at zero
bias is found to evolve smoothly into a conductance plateau at 0.85 (2e^2/h) at
finite bias. Varying the gate voltage the transition between the 1.0 and the
0.85 (2e^2/h) plateaus occurs for definite bias voltages, which defines a gate
voltage dependent energy difference . This energy difference is
compared with the activation temperature T_a extracted from the experimentally
observed activated behavior of the 0.7 anomaly at low bias. We find \Delta =
k_B T_a which lends support to the idea that the conductance anomaly is due to
transmission through two conduction channels, of which the one with its subband
edge \Delta below the chemical potential becomes thermally depopulated as the
temperature is increased.Comment: 9 pages (RevTex) with 9 figures (some in low resolution
Threshold features in transport through a 1D constriction
Suppression of electron current through a 1D channel of length
connecting two Fermi liquid reservoirs is studied taking into account the
Umklapp electron-electron interaction induced by a periodic potential. This
interaction causes Hubbard gaps for . In the perturbative
regime where ( charge velocity), and for small deviations
of the electron density from its commensurate values
can diverge with some exponent as voltage or temperature decreases above
, while it goes to zero below . This results
in a nonmonotonous behavior of the conductance.Comment: Final variant published in PRL, 79, 1714; minor correction
Hard Instances of the Constrained Discrete Logarithm Problem
The discrete logarithm problem (DLP) generalizes to the constrained DLP,
where the secret exponent belongs to a set known to the attacker. The
complexity of generic algorithms for solving the constrained DLP depends on the
choice of the set. Motivated by cryptographic applications, we study sets with
succinct representation for which the constrained DLP is hard. We draw on
earlier results due to Erd\"os et al. and Schnorr, develop geometric tools such
as generalized Menelaus' theorem for proving lower bounds on the complexity of
the constrained DLP, and construct sets with succinct representation with
provable non-trivial lower bounds
Is there a d.c. Josephson Effect in Bilayer Quantum Hall Systems?
We argue on the basis of phenomenological and microscopic considerations that
there is no d.c. Josephson effect in ordered bilayer quantum Hall systems, even
at T=0. Instead the tunnel conductance is strongly enhanced, approaching a
finite value proportional to the square of the order parameter as the
interlayer tunneling amplitude vanishes.Comment: 5 pages, 2 figure
Charge carrier localised in zero-dimensional (CH3NH3)3Bi2I9 clusters
A metal-organic hybrid perovskite (CH3NH3PbI3) with three-dimensional framework of metal-halide octahedra has been reported as a low-cost, solution-processable absorber for a thin-film solar cell with a power-conversion efficiency over 20%. Low-dimensional layered perovskites with metal halide slabs separated by the insulating organic layers are reported to show higher stability, but the efficiencies of the solar cells are limited by the confinement of excitons. In order to explore the confinement and transport of excitons in zero-dimensional metalâorganic hybrid materials, a highly orientated film of (CH3NH3)3Bi2I9 with nanometre-sized core clusters of Bi2I93â surrounded by insulating CH3NH3+ was prepared via solution processing. The (CH3NH3)3Bi2I9 film shows highly anisotropic photoluminescence emission and excitation due to the large proportion of localised excitons coupled with delocalised excitons from intercluster energy transfer. The abrupt increase in photoluminescence quantum yield at excitation energy above twice band gap could indicate a quantum cutting due to the low dimensionality.Publisher PDFPeer reviewe
Interfacial Profile and Propagation of Frontal Photopolymerization Waves
We investigate the frontal photopolymerization
of a thiolâene
system with a combination of experiments and modeling, focusing on
the interfacial conversion profile and its planar wave propagation.
We spatially resolve the solid-to-liquid front by FT-IR and AFM mechanical
measurements, supplemented by differential scanning calorimetry. A
simple coarse-grained model is found to describe remarkably well the
frontal kinetics and the sigmoidal interface, capturing the effects
of UV light exposure time (or dose) and temperature, as well as the
front position and resulting patterned dimensions after development.
Analytical solutions for the conversion profile enable the description
of all conditions with a single master curve in the moving frame of
the front position. Building on this understanding, we demonstrate
the design and fabrication of gradient polymer materials, with tunable
properties <i>along</i> the direction of illumination, which
can be coupled with lateral patterning by modulated illumination or
grayscale lithography
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