Compensation of Effective Field in the Field-Induced Superconductor k-(BETS)2FeBr4 Observed by 77Se NMR

We report results of 77Se NMR frequency shift in the normal state of the organic charge-transfer-salt k-(BETS)2FeBr4 which shows magnetic field-induced superconductivity (FISC). From a simple mean field analysis, we determined the field and the temperature dependences of the magnetization m_{pi} of the \pi conduction electrons on BETS molecules. We found that the Fe spins are antiferromagnetically coupled to the pi electrons and determined the exchange field to be J = -2.3T/mu_B. The exchange field from the fully saturated Fe moments (5 mu_B) is compensated by an external field of 12T. This is close to the central field of the FISC phase, consistent with the Jaccarino-Peter local field-compensation mechanism for FISC (Phys. Rev. Lett. 9, 290 (1962))

Multiscale expansion of the lattice potential KdV equation on functions of infinite slow-varyness order

We present a discrete multiscale expansion of the lattice potential Korteweg-de Vries (lpKdV) equation on functions of infinite order of slow-varyness. To do so we introduce a formal expansion of the shift operator on many lattices holding at all orders. The lowest secularity condition from the expansion of the lpKdV equation gives a nonlinear lattice equation, depending on shifts of all orders, of the form of the nonlinear Schr\"odinger (NLS) equationComment: 9 pages, submitted to Journ. Phys.

The Law and Economics of Proportionality in Discovery

This paper analyzes the proportionality standard in discovery. Many believe the Advisory Committee\u27s renewed emphasis on this standard has the potential to infuse litigation practice with considerably more attention to questions related to the costs and benefits of discovery. We discuss the history and rationale of proportionality\u27s inclusion in Rule 26, adopting an analytical framework that focuses on how costs and benefits can diverge in litigation generally, and discovery in particular. Finally, we use this framework to understand the mechanics and challenges involved in deploying the six factors included in the proportionality standard. Throughout, we emphasize that the proportionality standard requires both difficult-to-answer positive questions and unavoidably normative judgments

Properties of the quaternary half-metal-type Heusler alloy Co2_2Mn1−x_{1-x}Fex_xSi

This work reports on the bulk properties of the quaternary Heusler alloy Co$_2$Mn$_{1-x}$Fe$_x$Si with the Fe concentration $x=$. All samples, which were prepared by arc melting, exhibit $L2_1$ long range order over the complete range of Fe concentration. Structural and magnetic properties of Co$_2$Mn$_{1-x}$Fe$_x$Si Heusler alloys were investigated by means of X-ray diffraction, high and low temperature magnetometry, M{\"o\ss}bauer spectroscopy, and differential scanning calorimetry. The electronic structure was explored by means of high energy photo emission spectroscopy at about 8 keV photon energy. This ensures true bulk sensitivity of the measurements. The magnetization of the Fe doped Heusler alloys is in agreement with the values of the magnetic moments expected for a Slater-Pauling like behavior of half-metallic ferromagnets. The experimental findings are discussed on the hand of self-consistent calculations of the electronic and magnetic structure. To achieve good agreement with experiment, the calculations indicate that on-site electron-electron correlation must be taken into account, even at low Fe concentration. The present investigation focuses on searching for the quaternary compound where the half-metallic behavior is stable against outside influences. Overall, the results suggest that the best candidate may be found at an iron concentration of about 50%.Comment: 26 pages, 9 figures Phys. Rev. B accepte

Axiomatic Holonomy Maps and Generalized Yang-Mills Moduli Space

This article is a follow-up of ``Holonomy and Path Structures in General Relativity and Yang-Mills Theory" by Barrett, J. W. (Int.J.Theor.Phys., vol.30, No.9, 1991). Its main goal is to provide an alternative proof of this part of the reconstruction theorem which concerns the existence of a connection. A construction of connection 1-form is presented. The formula expressing the local coefficients of connection in terms of the holonomy map is obtained as an immediate consequence of that construction. Thus the derived formula coincides with that used in "On Loop Space Formulation of Gauge Theories" by Chan, H.-M., Scharbach, P. and Tsou S.T. (Ann.Phys., vol.167, 454-472, 1986). The reconstruction and representation theorems form a generalization of the fact that the pointed configuration space of the classical Yang-Mills theory is equivalent to the set of all holonomy maps. The point of this generalization is that there is a one-to-one correspondence not only between the holonomy maps and the orbits in the space of connections, but also between all maps from the loop space on $M$ to group $G$ fulfilling some axioms and all possible equivalence classes of $P(M,G)$ bundles with connection, where the equivalence relation is defined by bundle isomorphism in a natural way.Comment: amslatex, 7 pages, no figure

New electronic orderings observed in cobaltates under the influence of misfit periodicities

We study with ARPES the electronic structure of CoO2 slabs, stacked with rock-salt (RS) layers exhibiting a different (misfit) periodicity. Fermi Surfaces (FS) in phases with different doping and/or periodicities reveal the influence of the RS potential on the electronic structure. We show that these RS potentials are well ordered, even in incommensurate phases, where STM images reveal broad stripes with width as large as 80\AA. The anomalous evolution of the FS area at low dopings is consistent with the localization of a fraction of the electrons. We propose that this is a new form of electronic ordering, induced by the potential of the stacked layers (RS or Na in NaxCoO2) when the FS becomes smaller than the Brillouin Zone of the stacked structure

Direct observation of localization in the minority-spin-band electrons of magnetite below the Verwey temperature

Two-dimensional spin-uncompensated momentum density distributions, $\rho_{\rm s}^{2D}({\bf p})$s, were reconstructed in magnetite at 12K and 300K from several measured directional magnetic Compton profiles. Mechanical de-twinning was used to overcome severe twinning in the single crystal sample below the Verwey transition. The reconstructed $\rho_{\rm s}^{2D}({\bf p})$ in the first Brillouin zone changes from being negative at 300 K to positive at 12 K. This result provides the first clear evidence that electrons with low momenta in the minority spin bands in magnetite are localized below the Verwey transition temperature.Comment: 13 pages, 4 figures, accepted in Physical Review

DNA Nucleobase Synthesis at Titan Atmosphere Analog by Soft X-rays

Titan, the largest satellite of Saturn, has an atmosphere chiefly made up of N2 and CH4 and includes traces of many simple organic compounds. This atmosphere also partly consists of haze and aerosol particles which during the last 4.5 gigayears have been processed by electric discharges, ions, and ionizing photons, being slowly deposited over the Titan surface. In this work, we investigate the possible effects produced by soft X-rays (and secondary electrons) on Titan aerosol analogs in an attempt to simulate some prebiotic photochemistry. The experiments have been performed inside a high vacuum chamber coupled to the soft X-ray spectroscopy beamline at the Brazilian Synchrotron Light Source, Campinas, Brazil. In-situ sample analyses were performed by a Fourier transform infrared spectrometer. The infrared spectra have presented several organic molecules, including nitriles and aromatic CN compounds. After the irradiation, the brownish-orange organic residue (tholin) was analyzed ex-situ by gas chromatographic (GC/MS) and nuclear magnetic resonance (1H NMR) techniques, revealing the presence of adenine (C5H5N5), one of the constituents of the DNA molecule. This confirms previous results which showed that the organic chemistry on the Titan surface can be very complex and extremely rich in prebiotic compounds. Molecules like these on the early Earth have found a place to allow life (as we know) to flourish.Comment: To appear in Journal of Physical Chemistry A.; Number of pages: 6; Number of Figures: 5; Number of Tables: 1; Number of references:49; Full paper at http://pubs.acs.org/doi/abs/10.1021/jp902824

Superconductivity in an organic insulator at very high magnetic fields

We investigate by electrical transport the field-induced superconducting state (FISC) in the organic conductor $\lambda$-(BETS)$_2$FeCl$_4$. Below 4 K, antiferromagnetic-insulator, metallic, and eventually superconducting (FISC) ground states are observed with increasing in-plane magnetic field. The FISC state survives between 18 and 41 T, and can be interpreted in terms of the Jaccarino-Peter effect, where the external magnetic field {\em compensates} the exchange field of aligned Fe$^{3+}$ ions. We further argue that the Fe$^{3+}$ moments are essential to stabilize the resulting singlet, two-dimensional superconducting stateComment: 9 pages 3 figure