185 research outputs found

    Analysis of feasibility of a new core catcher for the in-vessel core melt retention strategy

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    This study deals with the feasibility study of a new in-vessel core melt retention (IVCMR) strategy capable to extend the coping period in the event of adverse situations, involving the melting of the core. Since Fukushima accident, many studies have been carried out to resolve the severe accident mitigation issues related to the corium stabilization inside and outside the reactor vessel. This is in fact one of the most relevant safety issues to secure LWRs from the point of view of severe accident mitigation and containment integrity. As for the corium stabilization inside the reactor vessel, in this study it is proposed a new IVCMR concept, developed at the University of Pisa, based on the adoption of an original core catcher design made of batches of ceramic material. By profiting of its low thermal conductivity, this core catcher is capable to retard the heat-up of the lower head of the vessel during the phase of relocation of the corium. To support the feasibility of its design analytical and numerical analyses have been performed assuming homogeneous pool condition. Results show that the adoption of the proposed core catcher solution extends the severe accident coping period: after 1 h from the initiating event, the maximum temperature of the vessel wall is below the limit for which localized failure may appear

    Nonlinear lattice dynamics as a basis for enhanced superconductivity in YBa2Cu3O6.5

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    THz-frequency optical pulses can resonantly drive selected vibrational modes in solids and deform their crystal structure. In complex oxides, this method has been used to melt electronic orders, drive insulator to metal transitions or induce superconductivity. Strikingly, coherent interlayer transport strongly reminiscent of superconductivity can be transiently induced up to room temperature in YBa2Cu3O6+x. By combining femtosecond X-ray diffraction and ab initio density functional theory calculations, we determine here the crystal structure of this exotic non-equilibrium state. We find that nonlinear lattice excitation in normal-state YBa2Cu3O6+x at 100 K causes a staggered dilation/contraction of the Cu-O2 intra/inter- bilayer distances, accompanied by anisotropic changes in the in-plane O-Cu-O bond buckling. Density functional theory calculations indicate that these motions cause dramatic changes in the electronic structure. Amongst these, the enhancement in the dx2-y2 character of the in-plane electronic structure is likely to favor superconductivity.Comment: 28 pages, including Supplemen

    Preliminary analysis of an aged RPV subjected to station blackout

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    Today, 46% of operating Nuclear Power Plants (NPP) have a lifetime between 31 and 40 years, while 19% have been in operation for more than 40 years. Long Term Operation (LTO) is an urgent requirement for all of the nuclear industry. The aim of this study is to assess the performance of a reactor pressure vessel (RPV) subjected to a station blackout (SBO) event. Alterations suffered by the material properties and creep at elevated temperatures are considered. In this study, coupling between MELCOR and Finite Element Method (FEM) codes is carried out. In the Finite Element (FE) model, the combined effects of ageing and creep are implemented through degraded material properties and a viscoplastic model. The reliability of the model is validated by comparing the FOREVER/C1 experimental results. The results show that the RPV lower head bends downwards with a maximum radial expansion of about 260 mm and RPV thermomechanical properties are reduced by more than 50% at high temperatures. The effects of ageing, creep and long heat-up strongly affect the resistance of the RPV system until the point of compromising it in the absence of/delayed emergency intervention. Aged RPV at end-of-life may collapse earlier, and in less time, with the same accidental conditions

    Tunable Charge and Spin Order in PrNiO3_3 Thin Films and Superlattices

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    We have used polarized Raman scattering to probe lattice vibrations and charge ordering in 12 nm thick, epitaxially strained PrNiO3_3 films, and in superlattices of PrNiO3_3 with the band-insulator PrAlO3_3. A carefully adjusted confocal geometry was used to eliminate the substrate contribution to the Raman spectra. In films and superlattices under tensile strain, which undergo a metal-insulator transition upon cooling, the Raman spectra reveal phonon modes characteristic of charge ordering. These anomalous phonons do not appear in compressively strained films, which remain metallic at all temperatures. For superlattices under compressive strain, the Raman spectra show no evidence of anomalous phonons indicative of charge ordering, while complementary resonant x-ray scattering experiments reveal antiferromagnetic order associated with a modest increase in resistivity upon cooling. This confirms theoretical predictions of a spin density wave phase driven by spatial confinement of the conduction electrons.Comment: PRL, in pres

    Momentum-dependent charge correlations in YBa2_2Cu3_3O6+δ_{6+\delta} superconductors probed by resonant x-ray scattering: Evidence for three competing phases

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    We have used resonant x-ray scattering to determine the momentum dependent charge correlations in YBa2_2Cu3_3O6.55_{6.55} samples with highly ordered chain arrays of oxygen acceptors (ortho-II structure). The results reveal nearly critical, biaxial charge density wave (CDW) correlations at in-plane wave vectors (0.315, 0) and (0, 0.325). The corresponding scattering intensity exhibits a strong uniaxial anisotropy. The CDW amplitude and correlation length are enhanced as superconductivity is weakened by an external magnetic field. Analogous experiments were carried out on a YBa2_2Cu3_3O6.6_{6.6} crystal with a dilute concentration of spinless (Zn) impurities, which had earlier been shown to nucleate incommensurate magnetic order. Compared to pristine crystals with the same doping level, the CDW amplitude and correlation length were found to be strongly reduced. These results indicate a three-phase competition between spin-modulated, charge-modulated, and superconducting states in underdoped YBa2_2Cu3_3O6+δ_{6+\delta}.Comment: 6 pages, 3 figures revised version, to appear in Phys. Rev. Let

    Quantitative determination of bond order and lattice distortions in nickel oxide heterostructures by resonant x-ray scattering

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    We present a combined study of Ni KK-edge resonant x-ray scattering and density functional calculations to probe and distinguish electronically driven ordering and lattice distortions in nickelate heterostructures. We demonstrate that due to the low crystal symmetry, contributions from structural distortions can contribute significantly to the energy-dependent Bragg peak intensities of a bond-ordered NdNiO3_3 reference film. For a LaNiO3_3-LaAlO3_3 superlattice that exhibits magnetic order, we establish a rigorous upper bound on the bond-order parameter. We thus conclusively confirm predictions of a dominant spin density wave order parameter in metallic nickelates with a quasi-two-dimensional electronic structure

    Charge order driven by Fermi-arc instability in Bi2201

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    The understanding of the origin of superconductivity in cuprates has been hindered by the apparent diversity of intertwining electronic orders in these materials. We combined resonant x-ray scattering (REXS), scanning-tunneling microscopy (STM), and angle-resolved photoemission spectroscopy (ARPES) to observe a charge order that appears consistently in surface and bulk, and in momentum and real space within one cuprate family, Bi2201. The observed wave vectors rule out simple antinodal nesting in the single-particle limit but match well with a phenomenological model of a many-body instability of the Fermi arcs. Combined with earlier observations of electronic order in other cuprate families, these findings suggest the existence of a generic charge-ordered state in underdoped cuprates and uncover its intimate connection to the pseudogap regime.Comment: A high resolution version can be found at http://www.phas.ubc.ca/~quantmat/ARPES/PUBLICATIONS/Articles/Bi2201_CDW_REXS_STM.pdf
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