814 research outputs found

    Interplane charge dynamics in a valence-bond dynamical mean-field theory of cuprate superconductors

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    We present calculations of the interplane charge dynamics in the normal state of cuprate superconductors within the valence-bond dynamical mean-field theory. We show that by varying the hole doping, the c-axis optical conductivity and resistivity dramatically change character, going from metallic-like at large doping to insulating-like at low-doping. We establish a clear connection between the behavior of the c-axis optical and transport properties and the destruction of coherent quasiparticles as the pseudogap opens in the antinodal region of the Brillouin zone at low doping. We show that our results are in good agreement with spectroscopic and optical experiments.Comment: 5 pages, 3 figure

    Magnetic exchange interaction between rare-earth and Mn ions in multiferroic hexagonal manganites

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    We report a study of magnetic dynamics in multiferroic hexagonal manganite HoMnO3 by far-infrared spectroscopy. Low-temperature magnetic excitation spectrum of HoMnO3 consists of magnetic-dipole transitions of Ho ions within the crystal-field split J=8 manifold and of the triangular antiferromagnetic resonance of Mn ions. We determine the effective spin Hamiltonian for the Ho ion ground state. The magnetic-field splitting of the Mn antiferromagnetic resonance allows us to measure the magnetic exchange coupling between the rare-earth and Mn ions.Comment: accepted for publication in Physical Review Letter

    Charge dynamics in the half-metallic ferromagnet CrO\u3csub\u3e2\u3c/sub\u3e

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    Infrared spectroscopy is used to investigate the electronic structure and charge carrier relaxation in crystalline films of CrO2 which is the simplest of all half-metallic ferromagnets. Chromium dioxide is a bad metal at room temperature but it has a remarkably low residual resistivity (\u3c5 \u3eμΩ cm) despite the small spectral weight associated with free carrier absorption. The infrared measurements show that low residual resistivity is due to the collapse of the scattering rate at ω\u3c2000 \u3ecm-1. The blocking of the relaxation channels at low v and T can be attributed to the unique electronic structure of a half-metallic ferromagnet. In contrast to other ferromagnetic oxides, the intraband spectral weight is constant below the Curie temperature

    Optical characterization of Bi2_2Se3_3 in a magnetic field: infrared evidence for magnetoelectric coupling in a topological insulator material

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    We present an infrared magneto-optical study of the highly thermoelectric narrow-gap semiconductor Bi2_2Se3_3. Far-infrared and mid-infrared (IR) reflectance and transmission measurements have been performed in magnetic fields oriented both parallel and perpendicular to the trigonal cc axis of this layered material, and supplemented with UV-visible ellipsometry to obtain the optical conductivity σ1(ω)\sigma_1(\omega). With lowering of temperature we observe narrowing of the Drude conductivity due to reduced quasiparticle scattering, as well as the increase in the absorption edge due to direct electronic transitions. Magnetic fields HcH \parallel c dramatically renormalize and asymmetrically broaden the strongest far-IR optical phonon, indicating interaction of the phonon with the continuum free-carrier spectrum and significant magnetoelectric coupling. For the perpendicular field orientation, electronic absorption is enhanced, and the plasma edge is slightly shifted to higher energies. In both cases the direct transition energy is softened in magnetic field.Comment: Final versio

    Plasmonic Hot Spots in Triangular Tapered Graphene Microcrystals

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    Recently, plasmons in graphene have been observed experimentally using scattering scanning near-field optical microscopy. In this paper, we develop a simplified analytical approach to describe the behavior in triangular samples. Replacing Coulomb interaction by a short-range one reduces the problem to a Helmholtz equation, amenable to analytical treatment. We demonstrate that even with our simplifications, the system still exhibits the key features seen in the experiment.Comment: 4 pages, 3 figure

    Modeling of Plasmonic and Polaritonic Effects in Photocurrent Nanoscopy

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    We present a basic framework for modeling collective mode effects in photocurrent measurements performed on two-dimensional materials using nano-optical scanned probes. We consider photothermal, photovoltaic, and bolometric contributions to the photocurrent. We show that any one of these can dominate depending on frequency, temperature, applied bias, and sample geometry. Our model is able to account for periodic spatial oscillations (fringes) of the photocurrent observed near sample edges or inhomogeneities. For the case of a non-absorbing substrate, we find a direct relation between the spectra measured by the photocurrent nanoscopy and its parental scanning technique, near-field optical microscopy.Comment: 16 pages, 7 figure
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