KEWPIE2: A cascade code for the study of dynamical decay of excited nuclei

Submitted to Computer Physics CommunicationsInternational audienceKEWPIE — a cascade code devoted to investigating the dynamical decay of excited nuclei, specially designed for treating very low probability events related to the synthesis of super-heavy nuclei formed in fusion-evaporation reactions — has been improved and rewritten in C++ programing language to become KEWPIE2. The current version of the code comprises various nuclear models concerning the light-particle emission, fission process and statistical properties of excited nuclei. General features of the code, such as the numerical scheme and the main physical ingredients, are described in detail. Some typical calculations having been performed in the present paper clearly show that theoretical predictions are generally in accordance with experimental data. Furthermore, since the values of some input parameters cannot be determined neither theoretically nor experimentally, a sensibility analysis is presented. To this end, we systematically investigate the effects of using different parameter values and reaction models on the final results. As expected, in the case of heavy nuclei, the fission process has the most crucial role to play in theoretical predictions. This work would be essential for numerical modeling of fusion-evaporation reactions

Origin and age of an ongoing radioactive contamination of soils near La hague reprocessing plant based on ^239+240Pu/²³⁸Pu and ²⁴¹Am/²⁴¹Pu current ratios and ⁹⁰Sr and Ln(III) soil contents.

Nuclear reprocessing plants are sources of environmental contamination by gaseous or liquid discharges. Numerous radionuclides are of concern, with actinides and <sup>90</sup> Sr being the most radiotoxic. Environmental radioactivity survey programs mostly use γ-spectrometry to track contaminations because γ-spectrometry is very cost effective and can be carried out on raw samples. On the other hand, the determination of β- or α-emitting radionuclides in environmental samples requires rather sophisticated analytical methods, and are thus dedicated to specific goals. However, measuring radionuclides such as Pu, Am, and Sr often provides more information about the presence of a current or prior contamination and on its origin, based on the isotopic composition of the samples. We found that the analysis of <sup>241</sup> Pu, <sup>239+240</sup> Pu, <sup>241</sup> Am, and <sup>90</sup> Sr of a few selected soil samples taken near the nuclear reprocessing plant of La Hague, France, revealed the presence of a previous environmental contamination originating from several incidents in La Hague site involving atmospheric transfer and leaks in flooded waste pits. The <sup>241</sup> Am- <sup>241</sup> Pu dating method indicated a contamination period prior to 1983. The presence of elevated levels of light non-radioactive lanthanides and yttrium in the soil samples confirmed the involvement of cold fuel. Our results demonstrate how long-lived actinides are likely to reveal a long-term contamination of the environment by spent fuel. Our study indicates that there is a requirement to use more sophisticated tools than γ-spectrometry when surveying the environments surrounding industrial plants for nuclear power and nuclear reprocessing with a potential for the accidental release of radioactivity into the environment

Dynamics of massive systems and synthesis of superheavy elements

International audienceFor the synthesis of superheavy elements, it is indisensable to divide process into two steps : overcoming the Coulomb barrier and passing over the conditional saddle or the ridgeline. To facilitate the understanding of the mechanism which explains the fusion hindrance, we first emply an analytic model with an inverted parabola for the saddle. Then, results by realistic calculations are given for the cold fusion. Ambiguities of the model are also discussed for future investigations. Since the model is general, it is applied to incident channels with neutron-rich projectile and/or targets. These are necessary for synthesis of nuclides on so-called superheavy island around Z=114 and N=18

Memory effects on descent from nuclear fission barrier

Non-Markovian transport equations for nuclear large amplitude motion are derived from the collisional kinetic equation. The memory effects are caused by the Fermi surface distortions and depend on the relaxation time. It is shown that the nuclear collective motion and the nuclear fission are influenced strongly by the memory effects at the relaxation time $\tau \geq 5\cdot 10^{-23}{\rm s}$. In particular, the descent of the nucleus from the fission barrier is accompanied by characteristic shape oscillations. The eigenfrequency and the damping of the shape oscillations depend on the contribution of the memory integral in the equations of motion. The shape oscillations disappear at the short relaxation time regime at $\tau \to 0$, which corresponds to the usual Markovian motion in the presence of friction forces. We show that the elastic forces produced by the memory integral lead to a significant delay for the descent of the nucleus from the barrier. Numerical calculations for the nucleus $^{236}$U shows that due to the memory effect the saddle-to-scission time grows by a factor of about 3 with respect to the corresponding saddle-to-scission time obtained in liquid drop model calculations with friction forces.Comment: 22 pages, 8 figures, submitted to Phys. Rev.

Analysis of the Fusion Hindrance in Mass-symmetric Heavy Ion Reactions

The fusion hindrance, which is also denominated by the term extra-push, is studied on mass-symmetric systems by the use of the liquid drop model with the two-center parameterization. Following the idea that the fusion hindrance exists only if the liquid drop barrier (saddle point) is located at the inner side of the contact point after overcoming the outer Coulomb barrier, the reactions in which two barriers are overlapped with each other are determined. It is shown that there are many systems where the fusion hindrance does not exist for the atomic number of projectile or target nucleus $Z\leq43$, while for $Z>43$, all of the mass-symmetric reactions are fusion-hindered.Comment: 6 pages, 4 figures. to be published in Sci. in China

Quasi-fission reactions as a probe of nuclear viscosity

Fission fragment mass and angular distributions were measured from the ^{64}Ni+^{197}Au reaction at 418 MeV and 383 MeV incident energy. A detailed data analysis was performed, using the one-body dissipation theory implemented in the code HICOL. The effect of the window and the wall friction on the experimental observables was investigated. Friction stronger than one-body was also considered. The mass and angular distributions were consistent with one-body dissipation. An evaporation code DIFHEAT coupled to HICOL was developed in order to predict reaction time scales required to describe available data on pre-scission neutron multiplicities. The multiplicity data were again consistent with one-body dissipation. The cross-sections for touch, capture and quasi-fission were also obtained.Comment: 25 pages REVTeX, 3 tables, 13 figures, submitted to Phys. Rev

Search for a long lived component in the reaction U+U near the Coulomb barrier

Expérience GANILInternational audienceWe performed an experiment to search for a signature of a long living component in the collision of $^{238}$U + $^{238}$U between 6.09 and 7.35A MeV. The experiment was performed at GANIL using the spectrometer VAMOS, tuned for observing reactions with kinematics similar to fusion-fission events. Theoretical calculations indicate that if a long living component would exist for this reaction, the most probable fission channel of such a giant system would be via the emissionof quasi-lead nuclei. We detected events of such a category in the focal plane of VAMOS. These events present an excitation function growing as a function of the bombarding energy

Fission barrier of superheavy nuclei and persistence of shell effects at high spin: Cases of No 254 and Th 220

We report on the first measurement of the fission barrier height in a heavy shell-stabilized nucleus. The fission barrier height of No254 is measured to be Bf=6.0±0.5 MeV at spin 15 and, by extrapolation, Bf=6.6±0.9 MeV at spin 0. This information is deduced from the measured distribution of entry points in the excitation energy versus spin plane. The same measurement is performed for Th220 and only a lower limit of the fission barrier height can be determined: Bf(I)>8 MeV. Comparisons with theoretical fission barriers test theories that predict properties of superheavy elements