Electronic dynamics and frequency-dependent effects in circularly polarized strong-field physics

We analyze, quantum mechanically, the dynamics of ionization with a strong, circularly polarized, laser field. We show that the main source for non-adiabatic effects is connected to an effective barrier lowering due to the laser frequency. Such non-adiabatic effects manifest themselves through ionization rates and yields that depart up to more than one order of magnitude from a static-field configuration. Beyond circular polarization, these results show the limits of standard instantaneous - static-field like - interpretation of laser-matter interaction and the great need for including time dependent electronic dynamics

Circularly Polarized Molecular High Harmonic Generation Using a Bicircular Laser

We investigate the process of circularly polarized high harmonic generation in molecules using a bicircular laser field. In this context, we show that molecules offer a very robust framework for the production of circularly polarized harmonics, provided their symmetry is compatible with that of the laser field. Using a discrete time-dependent symmetry analysis, we show how all the features (harmonic order and polarization) of spectra can be explained and predicted. The symmetry analysis is generic and can easily be applied to other target and/or field configurations

Resonantly enhanced pair production in a simple diatomic model

A new mechanism for the production of electron-positron pairs from the interaction of a laser field and a fully stripped diatomic molecule in the tunneling regime is presented. When the laser field is turned off, the Dirac operator has resonances in both the positive and the negative energy continua while bound states are in the mass gap. When this system is immersed in a strong laser field, the resonances move in the complex energy plane: the negative energy resonances are pushed to higher energies while the bound states are Stark shifted. It is argued here that there is a pair production enhancement at the crossing of resonances by looking at a simple 1-D model: the nuclei are modeled simply by Dirac delta potential wells while the laser field is assumed to be static and of finite spatial extent. The average rate for the number of electron-positron pairs produced is evaluated and the results are compared to the single nucleus and to the free cases. It is shown that positrons are produced by the Resonantly Enhanced Pair Production (REPP) mechanism, which is analogous to the resonantly enhanced ionization of molecular physics. This phenomenon could be used to increase the number of pairs produced at low field strength, allowing the study of the Dirac vacuum.Comment: 11 pages, 4 figure

Quantum-classical correspondence in circularly polarized high harmonic generation

Using numerical simulations, we show that atomic high order harmonic generation, HHG, with a circularly polarized laser field offers an ideal framework for quantum-classical correspondence in strong field physics. With an appropriate initialization of the system, corresponding to a superposition of ground and excited state(s), simulated HHG spectra display a narrow strip of strong harmonic radiation preceded by a gap of missing harmonics in the lower part of the spectrum. In specific regions of the spectra, HHG tends to lock to circularly polarized harmonic emission. All these properties are shown to be closely related to a set of key classical periodic orbits that organize the recollision dynamics in an intense, circularly polarized field

Asymmetry of above-threshold ionization of metal clusters in two-color laser fields: A time-dependent density-functional study

URL:http://link.aps.org/doi/10.1103/PhysRevA.69.063415 DOI:10.1103/PhysRevA.69.063415Above threshold ionization (ATI) spectra of small metal clusters (e.g., Na4 and Na4+) are calculated numerically using a spherical jellium model and time-dependent density functional theory for two-color (1064 and 532 nm) ultrashort (25 fs) laser pulses as a function of phase difference between the two fields. ATI spectra and ionized electron fluxes are obtained in the two opposite directions of the linearly polarized laser fields. The asymmetry, defined as the difference in electron yield, is shown to depend strongly on the carrier-envelope phase of the second-harmonic (2ω) field. The ATI spectra allow one to identify the range of kinetic energies of the ionized electrons where the asymmetry mainly occurs. Comparisons are made between calculations with and without self-interaction correction and also with previous exact numerical solutions of the one-electron systems H and H2+ [A. D. Bandrauk and S. Chelkowski, Phys. Rev. Lett. 84, 3562 (2000)] where such asymmetry effects had first been observed. We find that ATI spectra in the clusters generally have much longer energy plateaus than in previously studied one-electron systems, with cutoffs up to 30-40 times the ponderomotive energy Up. In high-harmonic generation spectra, on the other hand, no extended plateaus are observed.Acknowledgment is made to the donors of the Petroleum Research Fund, administered by the ACS, as well as to the University of Missouri Research Board, for partial support of this research

Visualizing quantum entanglement and the EPR paradox during the photodissociation of a diatomic molecule using two ultrashort laser pulses

We investigate theoretically the dissociative ionization of a H2+ molecule using two ultrashort laser (pump-probe) pulses. The pump pulse prepares a dissociating nuclear wave packet on an ungerade surface of H2+. Next, an UV (or XUV) probe pulse ionizes this dissociating state at large (R = 20 - 100 bohr) internuclear distance. We calculate the momenta distributions of protons and photoelectrons which show a (two-slit-like) interference structure. A general, simple interference formula is obtained which depends on the electron and protons momenta, as well as on the pump-probe delay on the pulses durations and polarizations. This interference can be interpreted as visualization of an electron state delocalized over the two-centres. This state is an entangled state of a hydrogen atom with a momentum p and a proton with an opposite momentum. -p dissociating on the ungerade surface of H2+. This pump-probe scheme can be used to reveal the nonlocality of the electron which intuitively should be localized on just one of the protons separated by the distance R much larger than the atomic Bohr orbit

Coherent destruction of tunneling, dynamic localization and the Landau-Zener formula

We clarify the internal relationship between the coherent destruction of tunneling (CDT) for a two-state model and the dynamic localization (DL) for a one-dimensional tight-binding model, under the periodical driving field. The time-evolution of the tight-binding model is reproduced from that of the two-state model by a mapping of equation of motion onto a set of ${\rm SU}(2)$ operators. It is shown that DL is effectively an infinitely large dimensional representation of the CDT in the ${\rm SU}(2)$ operators. We also show that both of the CDT and the DL can be interpreted as a result of destructive interference in repeated Landau-Zener level-crossings.Comment: 5 pages, no figur