67 research outputs found
Supercell Altermagnets
Altermagnets are compensated magnets with unconvetional , and -wave
spin-channel order in reciprocal space. So far the search for new altermagnetic
candidates has been focused on materials in which the magnetic unit cell is
identical to the non-magnetic one, i.e. magnetic structures with zero
propagation vector. Here, we substantially broaden the family of altermagnetic
candidates by predicting supercell altermagnets. Their magnetic unit cell is
constructed by enlarging the paramagnetic primitive unit cell, resulting in a
non-zero propagation vector for the magnetic structure. This connection of the
magnetic configuration to the ordering of sublattices gives an extra degree of
freedom to supercell altermagnets, which can allow for the control over the
order parameter spatial orientation. We identify realistic candidates MnSe
with a -wave order, and RbCoBr, CsCoCr, and BaMnO with -wave
order. We demonstrate the reorientation of the order parameter in MnSe,
which has two different magnetic configurations, whose energy difference is
only 5 meV, opening the possibility of controlling the orientation of the
altermagnetic order parameter by external perturbations.Comment: 10 pages, 4 figure
Writing and Reading antiferromagnetic MnAu: N\'eel spin-orbit torques and large anisotropic magnetoresistance
Antiferromagnets are magnetically ordered materials which exhibit no net
moment and thus are insensitive to magnetic fields. Antiferromagnetic
spintronics aims to take advantage of this insensitivity for enhanced
stability, while at the same time active manipulation up to the natural THz
dynamic speeds of antiferromagnets is possible, thus combining exceptional
storage density and ultra-fast switching. However, the active manipulation and
read-out of the N\'eel vector (staggered moment) orientation is challenging.
Recent predictions have opened up a path based on a new spin-orbit torque,
which couples directly to the N\'eel order parameter. This N\'eel spin-orbit
torque was first experimentally demonstrated in a pioneering work using
semimetallic CuMnAs. Here we demonstrate for MnAu, a good conductor with a
high ordering temperature suitable for applications, reliable and reproducible
switching using current pulses and readout by magnetoresistance measurements.
The symmetry of the torques agrees with theoretical predictions and a large
read-out magnetoresistance effect of more than ~ is reproduced by
ab initio transport calculations.Comment: 5 pages, 4 figure
Strain control of band topology and surface states in antiferromagnetic EuCdAs
Topological semimetal antiferromagnets provide a rich source of exotic
topological states which can be controlled by manipulating the orientation of
the N\'eel vector, or by modulating the lattice parameters through strain. We
investigate via density functional theory calculations, the
effects of shear strain on the bulk and surface states n two antiferromagnetic
EuCdAs phases with out-of-plane and in-plane spin configurations. When
magnetic moments are along the -axis, a longitudinal or
diagonal shear strain can tune the Dirac semimetal phase to an axion insulator
phase, characterized by the parity-based invariant . For an
in-plane magnetic order, the axion insulator phase remains robust under all
shear strains. We further find that for both magnetic orders, the bulk gap
increases and a surface gap opens on the (001) surface up to 16 meV. Because of
a nonzero index and gapped states on the (001) surface, hinge modes
are expected to happen on the side surface states between those gapped surface
states. This result can provide a valuable insight in the realization of the
long-sought axion states.Comment: 5 pages, 4 figure
Anisotropic magnetotransport realized in doped hematite
Conventional antiferromagnetic materials have long been recognized for their
time-reversal symmetry, resulting in a zero anomalous Hall coefficient.
However, a paradigm shift occurs when examining easy-axis antiferromagnets and
their spin-flop transition. This transition introduces a magnetic canted
moment, leading to the emergence of a non-zero anomalous Hall signal and the
generation of a non-dissipative transversal current. While high symmetry
systems typically manifest an isotropic Hall effect, our study unveils the
extraordinary behavior exhibited by hematite that becomes conductive due to
small Ti doping. We investigate the magnetotransport in Titanium-doped
hematite, uncovering a highly pronounced and unconventional symmetry. Notably,
this effect displays a remarkable dependence on the crystal orientation of the
material. We establish a compelling correlation between our experimental
observations and the predicted anomalous Hall effect in altermagnets through
symmetry analysis. This study expands our understanding of the Hall effect in
antiferromagnetic materials and sheds light on the intricate interplay between
crystal orientation and unconventional Hall phenomena
Electric control of Dirac quasiparticles by spin-orbit torque in an antiferromagnet
Spin orbitronics and Dirac quasiparticles are two fields of condensed matter physics initiated independently about a decade ago. Here we predict that Dirac quasiparticles can be controlled by the spin-orbit torque reorientation of the Néel vector in an antiferromagnet. Using CuMnAs as an example, we formulate symmetry criteria allowing for the coexistence of topological Dirac quasiparticles and Néel spin-orbit torques. We identify the nonsymmorphic crystal symmetry protection of Dirac band crossings whose on and off switching is mediated by the Néel vector reorientation. We predict that this concept verified by minimal model and density functional calculations in the CuMnAs semimetal antiferromagnet can lead to a topological metal-insulator transition driven by the Néel vector and to the topological anisotropic magnetoresistance
Symmetry and topology in antiferromagnetic spintronics
Antiferromagnetic spintronics focuses on investigating and using
antiferromagnets as active elements in spintronics structures. Last decade
advances in relativistic spintronics led to the discovery of the staggered,
current-induced field in antiferromagnets. The corresponding N\'{e}el
spin-orbit torque allowed for efficient electrical switching of
antiferromagnetic moments and, in combination with electrical readout, for the
demonstration of experimental antiferromagnetic memory devices. In parallel,
the anomalous Hall effect was predicted and subsequently observed in
antiferromagnets. A new field of spintronics based on antiferromagnets has
emerged. We will focus here on the introduction into the most significant
discoveries which shaped the field together with a more recent spin-off
focusing on combining antiferromagnetic spintronics with topological effects,
such as antiferromagnetic topological semimetals and insulators, and the
interplay of antiferromagnetism, topology, and superconductivity in
heterostructures.Comment: Book chapte
Spontaneous anomalous Hall effect arising from an unconventional compensated magnetic phase in a semiconductor
The anomalous Hall effect, commonly observed in metallic magnets, has been
established to originate from the time-reversal symmetry breaking by an
internal macroscopic magnetization in ferromagnets or by a non-collinear
magnetic order. Here we observe a spontaneous anomalous Hall signal in the
absence of an external magnetic field in an epitaxial film of MnTe, which is a
semiconductor with a collinear antiparallel magnetic ordering of Mn moments and
a vanishing net magnetization. The anomalous Hall effect arises from an
unconventional phase with strong time-reversal symmetry breaking and
alternating spin polarization in real-space crystal structure and
momentum-space electronic structure. The anisotropic crystal environment of
magnetic Mn atoms due to the non-magnetic Te atoms is essential for
establishing the unconventional phase and generating the anomalous Hall effect.Comment: 34 pages, 14 figure
Band structure of CuMnAs probed by optical and photoemission spectroscopy
The tetragonal phase of CuMnAs progressively appears as one of the key materials for antiferromagnetic spintronics due to efficient current-induced spin-torques whose existence can be directly inferred from crystal symmetry. Theoretical understanding of spintronic phenomena in this material, however, relies on the detailed knowledge of electronic structure (band structure and corresponding wave functions) which has so far been tested only to a limited extent. We show that AC permittivity (obtained from ellipsometry) and UV photoelectron spectra agree with density functional calculations. Together with the x-ray diffraction and precession electron diffraction tomography, our analysis confirms recent theoretical claim [Phys. Rev. B 96, 094406 (2017)] that copper atoms occupy lattice positions in the basal plane of the tetragonal unit cell
Altermagnetic lifting of Kramers spin degeneracy
Lifted Kramers spin-degeneracy has been among the central topics of
condensed-matter physics since the dawn of the band theory of solids. It
underpins established practical applications as well as current frontier
research, ranging from magnetic-memory technology to topological quantum
matter. Traditionally, lifted Kramers spin-degeneracy has been considered to
originate from two possible internal symmetry-breaking mechanisms. The first
one refers to time-reversal symmetry breaking by magnetization of ferromagnets,
and tends to be strong due to the non-relativistic exchange-coupling origin.
The second mechanism applies to crystals with broken inversion symmetry, and
tends to be comparatively weaker as it originates from the relativistic
spin-orbit coupling. A recent theory work based on spin-symmetry classification
has identified an unconventional magnetic phase, dubbed altermagnetic, that
allows for lifting the Kramers spin degeneracy without net magnetization and
inversion-symmetry breaking. Here we provide the confirmation using
photoemission spectroscopy and ab initio calculations. We identify two distinct
unconventional mechanisms of lifted Kramers spin degeneracy generated by the
altermagnetic phase of centrosymmetric MnTe with vanishing net magnetization.
Our observation of the altermagnetic lifting of the Kramers spin degeneracy can
have broad consequences in magnetism. It motivates exploration and exploitation
of the unconventional nature of this magnetic phase in an extended family of
materials, ranging from insulators and semiconductors to metals and
superconductors, that have been either identified recently or perceived for
many decades as conventional antiferromagnets
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