Spiral spin-liquid and the emergence of a vortex-like state in MnSc2_2S4_4

Spirals and helices are common motifs of long-range order in magnetic solids, and they may also be organized into more complex emergent structures such as magnetic skyrmions and vortices. A new type of spiral state, the spiral spin-liquid, in which spins fluctuate collectively as spirals, has recently been predicted to exist. Here, using neutron scattering techniques, we experimentally prove the existence of a spiral spin-liquid in MnSc$_2$S$_4$ by directly observing the 'spiral surface' - a continuous surface of spiral propagation vectors in reciprocal space. We elucidate the multi-step ordering behavior of the spiral spin-liquid, and discover a vortex-like triple-q phase on application of a magnetic field. Our results prove the effectiveness of the $J_1$-$J_2$ Hamiltonian on the diamond lattice as a model for the spiral spin-liquid state in MnSc$_2$S$_4$, and also demonstrate a new way to realize a magnetic vortex lattice.Comment: 10 pages, 11 figure

Magnetic state in URu2Si2, UPd2Al3 and UNi2Al3 probed by point contacts

The antiferromagnetic (AFM) state has been investigated in the three heavy-fermion compounds URu2Si2, UPd2Al3, and UNi2Al3 by measuring dV/dI(V) curves of point contacts at different temperatures (1.5-20 K) and magnetic fields (0-28 T). The zero-bias maximum in dV/dI(V) for URu2Si2 points to a partially gapped Fermi-surface related to the itinerant nature of the AFM state contrary to UPd2Al3 where analogous features have not been found. The AFM state in UNi2Al3 has more similarities with URu2Si2. For URu2Si2, the same critical field of about 40 T along the easy c axis is found for all features in dV/dI(V) corresponding to the Neel temperature, the gap in the electronic density of states, and presumably the ordered moments.Comment: 10 pages incl. 5 figures, LaTex 2

Disorder-to-order transition in the magnetic and electronic properties of URh_2Ge_2

We present a study of annealing effects on the physical properties of tetragonal single--crystalline URh_2Ge_2. This system, which in as-grown form was recently established as the first metallic 3D random-bond heavy-fermion spin glass, is transformed by an annealing treatment into a long-range antiferromagnetically (AFM) ordered heavy-fermion compound. The transport properties, which in the as-grown material were dominated by the structural disorder, exhibit in the annealed material signs of typical metallic behavior along the crystallographic a axis. From our study URh_2Ge_2 emerges as exemplary material highlighting the role and relevance of structural disorder for the properties of strongly correlated electron systems. We discuss the link between the magnetic and electronic behavior and how they are affected by the structural disorder.Comment: Phys. Rev. B, in print (scheduled 1 Mar 2000

Field-induced quantum fluctuations in the heavy fermion superconductor CeCu2Ge2

Quantum-mechanical fluctuations in strongly correlated electron systems cause unconventional phenomena such as non-Fermi liquid behavior, and arguably high temperature superconductivity. Here we report the discovery of a field-tuned quantum critical phenomenon in stoichiometric CeCu2Ge2, a spin density wave ordered heavy fermion metal that exhibits unconventional superconductivity under ~ 10 GPa of applied pressure. Our finding of the associated quantum critical spin fluctuations of the antiferromagnetic spin density wave order, dominating the local fluctuations due to single-site Kondo effect, provide new information about the underlying mechanism that can be important in understanding superconductivity in this novel compound.Comment: Heavy Fermion, Quantum Critical Phenomeno

Influence of a magnetic field on the antiferromagnetic order in UPt_3

A neutron diffraction experiment was performed to investigate the effect of a magnetic field on the antiferromagnetic order in the heavy fermion superconductor UPt_3. Our results show that a field in the basal plane of up to 3.2 Tesla, higher than H_c2(0), has no effect: it can neither select a domain nor rotate the moment. This has a direct impact on current theories for the superconducting phase diagram based on a coupling to the magnetic order.Comment: 7 pages, RevTeX, 3 postscript figures, submitted to Phys. Rev.

Orbital state and magnetic properties of LiV_2 O_4

LiV_2 O_4 is one of the most puzzling compounds among transition metal oxides because of its heavy fermion like behavior at low temperatures. In this paper we present results for the orbital state and magnetic properties of LiV_2 O_4 obtained from a combination of density functional theory within the local density approximation and dynamical mean-field theory (DMFT). The DMFT equations are solved by quantum Monte Carlo simulations. The trigonal crystal field splits the V 3d orbitals such that the a_{1g} and e_{g}^{pi} orbitals cross the Fermi level, with the former being slightly lower in energy and narrower in bandwidth. In this situation, the d-d Coulomb interaction leads to an almost localization of one electron per V ion in the a_{1g} orbital, while the e_{g}^{pi} orbitals form relatively broad bands with 1/8 filling. 2The theoretical high-temperature paramagnetic susceptibility chi(T) follows a Curie-Weiss law with an effective paramagnetic moment p_{eff}=1.65 in agreement with the experimental results.Comment: 11 pages, 10 figures, 2 table

Surface critical behavior of bcc binary alloys

The surface critical behavior of bcc binary alloys undergoing a continuous B2-A2 order-disorder transition is investigated in the mean-field (MF) approximation. Our main aim is to provide clear evidence for the fact that surfaces which break the two-sublattice symmetry generically display the critical behavior of the NORMAL transition, whereas symmetry-preserving surfaces exhibit ORDINARY surface critical behavior. To this end we analyze the lattice MF equations for both types of surfaces in terms of nonlinear symplectic maps and derive a Ginzburg-Landau model for the symmetry-breaking (100) surface. The crucial feature of the continuum model is the emergence of an EFFECTIVE ORDERING (``staggered'') SURFACE FIELD, which depends on temperature and the other lattice model parameters, and which explains the appearance of NORMAL critical behavior for symmetry-breaking surfaces.Comment: 16 pages, REVTeX 3.0, 13 EPSF figures, submitted to Phys. Rev.

Formation of heavy quasiparticle state in two-band Hubbard model

A realization of heavy fermion state is investigated on the basis of two-band Hubbard model. By means of the slave-boson mean-field approximation, it is shown that for the intermediate electron density, n_e=1.5, the inter-band Coulomb repulsion U strongly emphasizes initially small difference between bands, and easily stabilizes integral valence in the lower band. As a result, a strong renormalization takes place in the lower band and the mixing strength between two bands. It gives rise to a sharp peak at the Fermi level in the quasiparticle density of states, as that obtained in the periodic Anderson model. In contrast to a simple insight that the Hund's-rule coupling J reduces the characteristic energy, it turns out to be almost irrelevant to the renormalization for J<U. The required conditions are suitable for LiV_2O_4, the first observed heavy fermion compound in transition metal oxide.Comment: 5 pages, 4 figures, to be published in Phys. Rev.

Staggered Pairing Phenomenology for UPd_2Al_3 and UNi_2Al_3

We apply the staggered-pairing Ginzburg-Landau phenomenology to describe superconductivity in UPd_2Al_3 and UNi_2Al_3. The phenomenology was applied successfully to UPt_3 so it explains why these materials have qualitatively different superconducting phase diagrams although they have the same point-group symmetry. UPd_2Al_3 and UNi_2Al_3 have a two-component superconducting order parameter transforming as an H-point irreducible representation of the space group. Staggered superconductivity can induce charge-density waves characterized by new Bragg peaks suggesting experimental tests of the phenomenology.Comment: 4 pages, REVTeX, 2 Postscript figure

Heavy-Mass Behavior of Ordered Perovskites ACu3Ru4O12 (A = Na, Ca, La)

We synthesized ACu3Ru4O12 (A = Na, Na0.5Ca0.5, Ca, Ca0.5La0.5, La) and measured their DC magnetization, AC susceptibility, specific heat, and resistivity, in order to investigate the effects of the hetero-valent substitution. A broad peak in the DC magnetization around 200 K was observed only in CaCu3Ru4O12, suggesting the Kondo effect due to localized Cu2+ ions. However, the electronic specific heat coefficients exhibit large values not only for CaCu3Ru4O12 but also for all the other samples. Moreover, the Wilson ratio and the Kadowaki-Woods ratio of our samples are all similar to the values of other heavy-fermion compounds. These results question the Kondo effect as the dominant origin of the mass enhancement, and rather indicate the importance of correlations among itinerant Ru electrons.Comment: 6 pages, 6 figures, to be published in J. Phys. Soc. Jp