Defects induced ferromagnetism in Mn doped ZnO

Single phase Mn doped (2 at %) ZnO samples have been synthesized by solid-state reaction technique. Before the final sintering at 500 C, the mixed powders have been milled for different milling periods (6, 24, 48 and 96 hours). The grain sizes of the samples are very close to each other (~ 32 \pm 4 nm). However, the defective state of the samples is different from each other as manifested from the variation of magnetic properties and electrical resistivity with milling time. All the samples have been found to be ferromagnetic with clear hysteresis loops at room temperature. The maximum value for saturation magnetization (0.11 {\mu}_B / Mn atom) was achieved for 96 hours milled sample. Electrical resistivity has been found to increase with increasing milling time. The most resistive sample bears the largest saturation magnetization. Variation of average positron lifetime with milling time bears a close similarity with that of the saturation magnetization. This indicates the key role played by open volume vacancy defects, presumably zinc vacancies near grain surfaces, in inducing ferromagnetic order in Mn doped ZnO. To attain optimum defect configuration favorable for ferromagnetism in this kind of samples proper choice of milling period and annealing conditions is required.Comment: Accepted in Journal of Magnetism and Magnetic Material

Magnetically soft, high moment grain-refined Fe films: application to magnetic tunnel junctions

The effect of N-doping on the microstructure and magnetic properties of thin Fe layers has been employed to construct all Fe-electrode magnetic tunnel junctions that displayed the tunneling magnetoresistance (TMR) effect. Using low nitrogen doses, a reduction in coercivity was achieved due to grain refinement, without a concurrent decrease in the saturation magnetization of the Fe films caused by the formation of crystalline iron nitride phases. It was demonstrated that this N-induced grain refinement can be applied beneficially to control the switching field of the "free" layer in magnetic trilayer structures. In general the ability to control magnetic softness without reducing saturation magnetization will prove important for incorporating high spin-polarized materials into spin valves and TMR devices

Quantum phase diagram of an exactly solved mixed spin ladder

We investigate the quantum phase diagram of the exactly solved mixed spin-(1/2,1) ladder via the thermodynamic Bethe ansatz (TBA). In the absence of a magnetic field the model exhibits three quantum phases associated with su(2), su(4) and su(6) symmetries. In the presence of a strong magnetic field, there is a third and full saturation magnetization plateaux within the strong antiferromagnetic rung coupling regime. Gapless and gapped phases appear in turn as the magnetic field increases. For weak rung coupling, the fractional magnetization plateau vanishs and exhibits new quantum phase transitions. However, in the ferromagnetic coupling regime, the system does not have a third saturation magnetization plat eau. The critical behaviour in the vicinity of the critical points is also derived systematically using the TBA.Comment: 20 pages, 2 figure