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(Photo)Electrocatalytic CO2 Reduction at the Defective Anatase TiO2 (101) Surface
Excessive carbon dioxide (CO2) emissions by combustion of fossil fuels are linked to global warming and rapid climate change. One promising route to lowering the concentration of CO2 in the atmosphere is to reduce it to useful small molecules via photoelectrocatalytic hydrogenation, which would enable solar energy storage with a zero-carbon emission cycle and perform a more efficient separation of the photogenerated electron and hole pair than pure photocatalysis. Indeed, photoelectrocatalytic CO2 reduction has been an intense focus of research. Using the density functional theory (DFT), we studied the CO2 reduction reaction on the defective anatase TiO2 (101) surface, at both the solvent/catalyst and the electrolyte/catalyst interfaces. The analysis of the electronic structure of the surface shows a contrast between the solvent/catalyst and the electrolyte/catalyst interfaces, which results in the two corresponding catalytic cycles being distinct. Our study explains at the electronic and mechanistic levels why methanol is the main product in the presence of the electrolyte and why the overpotential is not only controlled by the reaction process but also by the diffusion process
Micromagnetic simulations of current-induced magnetization switching in Co/Cu/Co nanopillars
Author name used in this publication: S. Q. Shi2007-2008 > Academic research: refereed > Publication in refereed journalVersion of RecordPublishe
Current-induced magnetization dynamics in Co/Cu/Co nanopillars
Author name used in this publication: S. Q. Shi2007-2008 > Academic research: refereed > Publication in refereed journalVersion of RecordPublishe
Elastoplastic phase field model for microstructure evolution
2005-2006 > Academic research: refereed > Publication in refereed journalVersion of RecordPublishe
Seroprevalence of Mycoplasma bovis infection in dairy cows in subtropical southern China
The seroprevalence of Mycoplasma bovis infection in dairy cows in Guangxi Zhuang Autonomous Region (GZAR) in subtropical southern China was surveyed between June 2009 and March 2010. A total of 455 serum samples of dairy cows were collected from 6 districts in 4 different cities, and examined for M. bovis antibodies with the indirect enzyme-linked immunosorbent assay (ELISA) using a commercially available kit. The overall seroprevalence of M. bovis infection in dairy cows was 7.69% (35/455). Three year-old dairy cows had the highest seroprevalence (15.0%), followed by dairy cows of 4 year-old (11.1%). Dairy cows with the history of 5 pregnancies had the highest seroprevalence (33.3%). However, no statistically significant association was found between M. bovis infection and age or number of pregnancies (p > 0.05). All the aborting dairy cows were negative for M. bovis antibodies, suggesting that bovine abortion may have no association with M. bovis infection in GZAR. These results indicate that M. bovis infection in dairy cows was widespread in GZAR, and integrated strategies and measures should be performed to control and prevent M. bovis infection and disease outbreak.Key words: Mycoplasma bovis, seroprevalence, dairy cows, Guangxi Zhuang Autonomous Region (GZAR), China, enzyme-linked immunosorbent assay (ELISA)
Real-time counting of single electron tunneling through a T-shaped double quantum dot system
Real-time detection of single electron tunneling through a T-shaped double
quantum dot is simulated, based on a Monte Carlo scheme. The double dot is
embedded in a dissipative environment and the presence of electrons on the
double dot is detected with a nearby quantum point contact. We demonstrate
directly the bunching behavior in electron transport, which leads eventually to
a super-Poissonian noise. Particularly, in the context of full counting
statistics, we investigate the essential difference between the dephasing
mechanisms induced by the quantum point contact detection and the coupling to
the external phonon bath. A number of intriguing noise features associated with
various transport mechanisms are revealed.Comment: 8 pages, 5 figure
Simulation of multilevel cell spin transfer switching in a full-Heusler alloy spin-valve nanopillar
Author name used in this publication: Shi, S. Q.2012-2013 > Academic research: refereed > Publication in refereed journalVersion of RecordPublishe
Male germ cell-specific protein Trs4 binds to multiple proteins
Temperature-related sequence 4 (Trs4) has been identified as a testis-specific gene with expression sensitive to the abdominal temperature changes induced by artificial cryptorchidism. In murine testes, Trs4 mRNA was detected in round spermatids and its protein was localized mainly in the elongating spermatids as well as in the acrosomes and tails of mature spermatozoa. Using a yeast two-hybrid screening system, we identified Rshl-2, Gstmu1, and Ddc8 as putative binding partners of the Trs4 protein in mouse testes. Their interactions were confirmed by in vivo and in vitro binding assays. Further studies demonstrated that Ddc8, a newly identified gene with unknown functions, displayed a similar expression pattern with Trs4 in mouse testes. In particular, Trs4, Ddc8, and Rshl-2 proteins were co-localized to the tails of mature spermatozoa. These results suggested that Trs4 might be involved in diverse processes of spermiogenesis and/or fertilization through interactions with its multiple binding partners. © 2009 Elsevier Inc.postprin
Experimental bond behaviour of GFRP and masonry bricks under impulsive loading
Fibre Reinforced Polymers have become a popular material for strengthening of masonry structures. The performance of this technique is strongly dependent on the bond between the FRP and the substrate. Understanding the strain rate effect on these materials and strengthening techniques is important for proper design and proper modelling of these systems under impacts or blast loads. This work aims to study the behaviour of the bond between GFRP and brick at different strain rates. A Drop Weight Impact Machine specially developed for pull-off tests (single shear tests) is used with different masses and different heights introducing different deformation rates. The strain rate effect on the failure mode, shear capacity and effective bond length is determined from the experimental results. Empirical relations of dynamic increase factors (DIF) for these materials and techniques are also presented.This work was performed under Project CH-SECURE (PTDC/EMC/120118/2010)
funded by the Portuguese Foundation of Science and Technology – FCT. The authors
acknowledge the support. The first author also acknowledges the support from his PhD
FCT grant with the reference SFRH/BD/45436/2008
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