An automated and versatile ultra-low temperature SQUID magnetometer

We present the design and construction of a SQUID-based magnetometer for operation down to temperatures T = 10 mK, while retaining the compatibility with the sample holders typically used in commercial SQUID magnetometers. The system is based on a dc-SQUID coupled to a second-order gradiometer. The sample is placed inside the plastic mixing chamber of a dilution refrigerator and is thermalized directly by the 3He flow. The movement though the pickup coils is obtained by lifting the whole dilution refrigerator insert. A home-developed software provides full automation and an easy user interface.Comment: RevTex, 10 pages, 10 eps figures. High-resolution figures available upon reques

Unconventional antiferromagnetic correlations of the doped Haldane gap system Y2_2BaNi1−x_{1-x}Znx_xO5_5

We make a new proposal to describe the very low temperature susceptibility of the doped Haldane gap compound Y$_2$BaNi$_{1-x}$Zn$_x$O$_5$. We propose a new mean field model relevant for this compound. The ground state of this mean field model is unconventional because antiferromagnetism coexists with random dimers. We present new susceptibility experiments at very low temperature. We obtain a Curie-Weiss susceptibility $\chi(T) \sim C / (\Theta+T)$ as expected for antiferromagnetic correlations but we do not obtain a direct signature of antiferromagnetic long range order. We explain how to obtain the ``impurity'' susceptibility $\chi_{imp}(T)$ by subtracting the Haldane gap contribution to the total susceptibility. In the temperature range [1 K, 300 K] the experimental data are well fitted by $T \chi_{imp}(T) = C_{imp} (1 + T_{imp}/T )^{-\gamma}$. In the temperature range [100 mK, 1 K] the experimental data are well fitted by $T \chi_{imp}(T) = A \ln{(T/T_c)}$, where $T_c$ increases with $x$. This fit suggests the existence of a finite N\'eel temperature which is however too small to be probed directly in our experiments. We also obtain a maximum in the temperature dependence of the ac-susceptibility $\chi'(T)$ which suggests the existence of antiferromagnetic correlations at very low temperature.Comment: 19 pages, 17 figures, revised version (minor modifications

Classical and nonclassical randomness in quantum measurements

The space of positive operator-valued measures on the Borel sets of a compact (or even locally compact) Hausdorff space with values in the algebra of linear operators acting on a d-dimensional Hilbert space is studied from the perspectives of classical and non-classical convexity through a transform $\Gamma$ that associates any positive operator-valued measure with a certain completely positive linear map of the homogeneous C*-algebra $C(X)\otimes B(H)$ into $B(H)$. This association is achieved by using an operator-valued integral in which non-classical random variables (that is, operator-valued functions) are integrated with respect to positive operator-valued measures and which has the feature that the integral of a random quantum effect is itself a quantum effect. A left inverse $\Omega$ for $\Gamma$ yields an integral representation, along the lines of the classical Riesz Representation Theorem for certain linear functionals on $C(X)$, of certain (but not all) unital completely positive linear maps $\phi:C(X)\otimes B(H) \rightarrow B(H)$. The extremal and C*-extremal points of the space of POVMS are determined.Comment: to appear in Journal of Mathematical Physic

Decomposition of time-covariant operations on quantum systems with continuous and/or discrete energy spectrum

Every completely positive map G that commutes which the Hamiltonian time evolution is an integral or sum over (densely defined) CP-maps G_\sigma where \sigma is the energy that is transferred to or taken from the environment. If the spectrum is non-degenerated each G_\sigma is a dephasing channel followed by an energy shift. The dephasing is given by the Hadamard product of the density operator with a (formally defined) positive operator. The Kraus operator of the energy shift is a partial isometry which defines a translation on R with respect to a non-translation-invariant measure. As an example, I calculate this decomposition explicitly for the rotation invariant gaussian channel on a single mode. I address the question under what conditions a covariant channel destroys superpositions between mutually orthogonal states on the same orbit. For channels which allow mutually orthogonal output states on the same orbit, a lower bound on the quantum capacity is derived using the Fourier transform of the CP-map-valued measure (G_\sigma).Comment: latex, 33 pages, domains of unbounded operators are now explicitly specified. Presentation more detailed. Implementing the shift after the dephasing is sometimes more convenien

Non-equilibrium quasi-stationary states in a magnetized plasma

International audienceNon-equilibrium quasi-stationary states resulting from curvature driven interchange instabilities and drift-wave instabilities in a low beta, weakly ionized, magnetized plasma are investigated in the context of laboratory experiments in a toroidal configuration. Analytic modelling, numerical simulations and experimental results are discussed with emphasis on identifying the unstable modes and understanding the physics of anomalous particle and energy fluxes and their linkage to self-organized pressure profiles

Density functional theory calculations and vibrational spectroscopy on iron spin-crossover compounds

Iron complexes with a suitable ligand field undergo spin-crossover (SCO), which can be induced reversibly by temperature, pressure or even light. Therefore, these compounds are highly interesting candidates for optical information storage, for display devices and pressure sensors. The SCO phenomenon can be conveniently studied by spectroscopic techniques like Raman and infrared spectroscopy as well as nuclear inelastic scattering, a technique which makes use of the M\"ossbauer effect. This review covers new developments which have evolved during the last years like, e.g. picosecond infrared spectroscopy and thin film studies but also gives an overviewon newtechniques for the theoretical calculation of spin transition phenomena and vibrational spectroscopic data of SCO complexes

Optimal discrimination of quantum operations

We address the problem of discriminating with minimal error probability two given quantum operations. We show that the use of entangled input states generally improves the discrimination. For Pauli channels we provide a complete comparison of the optimal strategies where either entangled or unentangled input states are used.Comment: 4 pages, no figure

Generalized Bell Inequality Experiments and Computation

We consider general settings of Bell inequality experiments with many parties, where each party chooses from a finite number of measurement settings each with a finite number of outcomes. We investigate the constraints that Bell inequalities place upon the correlations possible in a local hidden variable theories using a geometrical picture of correlations. We show that local hidden variable theories can be characterized in terms of limited computational expressiveness, which allows us to characterize families of Bell inequalities. The limited computational expressiveness for many settings (each with many outcomes) generalizes previous results about the many-party situation each with a choice of two possible measurements (each with two outcomes). Using this computational picture we present generalizations of the Popescu-Rohrlich non-local box for many parties and non-binary inputs and outputs at each site. Finally, we comment on the effect of pre-processing on measurement data in our generalized setting and show that it becomes problematic outside of the binary setting, in that it allows local hidden variable theories to simulate maximally non-local correlations such as those of these generalised Popescu-Rohrlich non-local boxes.Comment: 16 pages, 2 figures, supplemental material available upon request. Typos corrected and references adde

Decoherence and Entanglement Dynamics in Fluctuating Fields

We study pure phase damping of two qubits due to fluctuating fields. As frequently employed, decoherence is thus described in terms of random unitary (RU) dynamics, i.e., a convex mixture of unitary transformations. Based on a separation of the dynamics into an average Hamiltonian and a noise channel, we are able to analytically determine the evolution of both entanglement and purity. This enables us to characterize the dynamics in a concurrence-purity (CP) diagram: we find that RU phase damping dynamics sets constraints on accessible regions in the CP plane. We show that initial state and dynamics contribute to final entanglement independently.Comment: 10 pages, 5 figures, added minor changes in order to match published versio

Domain Wall Spin Dynamics in Kagome Antiferromagnets

We report magnetization and neutron scattering measurements down to 60 mK on a new family of Fe based kagome antiferromagnets, in which a strong local spin anisotropy combined with a low exchange path network connectivity lead to domain walls intersecting the kagome planes through strings of free spins. These produce unfamiliar slow spin dynamics in the ordered phase, evolving from exchange-released spin-flips towards a cooperative behavior on decreasing the temperature, probably due to the onset of long-range dipolar interaction. A domain structure of independent magnetic grains is obtained that could be generic to other frustrated magnets.Comment: 5 pages, 4 figure