Interplay between shear loading and structural aging in a physical gel

We show that the aging of the mechanical relaxation of a gelatin gel exhibits the same scaling phenomenology as polymer and colloidal glasses. Besides, gelatin is known to exhibit logarithmic structural aging (stiffening). We find that stress accelerates this process. However, this effect is definitely irreducible to a mere age shift with respect to natural aging. We suggest that it is interpretable in terms of elastically-aided elementary (coil$\to$helix) local events whose dynamics gradually slows down as aging increases geometric frustration

Activated sampling in complex materials at finite temperature: the properly-obeying-probability activation-relaxation technique

While the dynamics of many complex systems is dominated by activated events, there are very few simulation methods that take advantage of this fact. Most of these procedures are restricted to relatively simple systems or, as with the activation-relaxation technique (ART), sample the conformation space efficiently at the cost of a correct thermodynamical description. We present here an extension of ART, the properly-obeying-probability ART (POP-ART), that obeys detailed balance and samples correctly the thermodynamic ensemble. Testing POP-ART on two model systems, a vacancy and an interstitial in crystalline silicon, we show that this method recovers the proper thermodynamical weights associated with the various accessible states and is significantly faster than MD in the diffusion of a vacancy below 700 K.Comment: 10 pages, 3 figure

Thermodynamics of the Spin Luttinger-Liquid in a Model Ladder Material

The phase diagram in temperature and magnetic field of the metal-organic, two-leg, spin-ladder compound (C5H12N)2CuBr4 is studied by measurements of the specific heat and the magnetocaloric effect. We demonstrate the presence of an extended spin Luttinger-liquid phase between two field-induced quantum critical points and over a broad range of temperature. Based on an ideal spin-ladder Hamiltonian, comprehensive numerical modelling of the ladder specific heat yields excellent quantitative agreement with the experimental data across the complete phase diagram.Comment: 4 pages, 4 figures, updated refs and minor changes to the text, version accepted for publication in Phys. Rev. Let

Magnetic properties of (VO)_2P_2O_7: two-plane structure and spin-phonon interactions

Detailed experiments on single-crystal (VO)_2P_2O_7 continue to reveal new and unexpected features. We show that a model composed of two, independent planes of spin chains with frustrated magnetic coupling is consistent with nuclear magnetic resonance and inelastic neutron scattering measurements. The pivotal role of PO_4 groups in mediating intrachain exchange interactions explains both the presence of two chain types and their extreme sensitivity to certain lattice vibrations, which results in the strong magnetoelastic coupling observed by light scattering. We compute the respective modifications of the spin and phonon dynamics due to this coupling, and illustrate their observable consequences on the phonon frequencies, magnon dispersions, static susceptibility and specific heat.Comment: 10 pages, 9 figure

Physics of the Insulating Phase in the Dilute Two-Dimensional Electron Gas

We propose to use the radio-frequency single-electron transistor as an extremely sensitive probe to detect the time-periodic ac signal generated by sliding electron lattice in the insulating state of the dilute two-dimensional electron gas. We also propose to use the optically-pumped NMR technique to probe the electron spin structure of the insulating state. We show that the electron effective mass and spin susceptibility are strongly enhanced by critical fluctuations of electron lattice in the vicinity of the metal-insulator transition, as observed in experiment.Comment: 5 pages, 2 figures, uses jetpl.cls (included). v.4: After publication in JETP Letters, two plots comparing theory and experiment are added, and a minor error is correcte

Self-organization with equilibration: a model for the intermediate phase in rigidity percolation

Recent experimental results for covalent glasses suggest the existence of an intermediate phase attributed to the self-organization of the glass network resulting from the tendency to minimize its internal stress. However, the exact nature of this experimentally measured phase remains unclear. We modify a previously proposed model of self-organization by generating a uniform sampling of stress-free networks. In our model, studied on a diluted triangular lattice, an unusual intermediate phase appears, in which both rigid and floppy networks have a chance to occur, a result also observed in a related model on a Bethe lattice by Barre et al. [Phys. Rev. Lett. 94, 208701 (2005)]. Our results for the bond-configurational entropy of self-organized networks, which turns out to be only about 2% lower than that of random networks, suggest that a self-organized intermediate phase could be common in systems near the rigidity percolation threshold.Comment: 9 pages, 6 figure

Magnetic Properties of (VO)_2P_2O_7 from Frustrated Interchain Coupling

Neutron-scattering experiments on (VO)_2P_2O_7 reveal both a gapped magnon dispersion and an unexpected, low-lying second mode. The proximity and intensity of these modes suggest a frustrated coupling between the alternating spin chains. We deduce the minimal model containing such a frustration, and show that it gives an excellent account of the magnon dispersion, static susceptibility and electron spin resonance absorption. We consider two-magnon states which bind due to frustration, and demonstrate that these may provide a consistent explanation for the second mode.Comment: RevTeX, 5 pages, 6 figures, compressed from first versio

Self-organized criticality in the intermediate phase of rigidity percolation

Experimental results for covalent glasses have highlighted the existence of a new self-organized phase due to the tendency of glass networks to minimize internal stress. Recently, we have shown that an equilibrated self-organized two-dimensional lattice-based model also possesses an intermediate phase in which a percolating rigid cluster exists with a probability between zero and one, depending on the average coordination of the network. In this paper, we study the properties of this intermediate phase in more detail. We find that microscopic perturbations, such as the addition or removal of a single bond, can affect the rigidity of macroscopic regions of the network, in particular, creating or destroying percolation. This, together with a power-law distribution of rigid cluster sizes, suggests that the system is maintained in a critical state on the rigid/floppy boundary throughout the intermediate phase, a behavior similar to self-organized criticality, but, remarkably, in a thermodynamically equilibrated state. The distinction between percolating and non-percolating networks appears physically meaningless, even though the percolating cluster, when it exists, takes up a finite fraction of the network. We point out both similarities and differences between the intermediate phase and the critical point of ordinary percolation models without self-organization. Our results are consistent with an interpretation of recent experiments on the pressure dependence of Raman frequencies in chalcogenide glasses in terms of network homogeneity.Comment: 20 pages, 18 figure

Structure of 12Be: intruder d-wave strength at N=8

The breaking of the N=8 shell-model magic number in the 12Be ground state has been determined to include significant occupancy of the intruder d-wave orbital. This is in marked contrast with all other N=8 isotones, both more and less exotic than 12Be. The occupancies of the 0 hbar omega neutron p1/2-orbital and the 1 hbar omega, neutron d5/2 intruder orbital were deduced from a measurement of neutron removal from a high-energy 12Be beam leading to bound and unbound states in 11Be.Comment: 5 pages, 2 figure

Search for the \pi Resonance in Two Particle Tunneling Experiments of YBCO Superconductors

A recent theory of the resonant neutron scattering peaks in YBCO superconductors predicts the existence of a sharp spin triplet two particle collective mode (the ``\pi resonance") in the normal state. In this paper, we propose an experiment in which the \pi resonance could be probed directly in a two particle tunneling measurement.Comment: 10 pages, LATEX , 3 ps figure