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P2-type Na2/3Ni1/3Mn2/3O2 Cathode Material with Excellent Rate and Cycling Performance for Sodium-Ion Batteries
P2-type Na2/3Ni1/3Mn2/3O2 is an air-stable cathode material for sodium-ion batteries. However, it suffers irreversible P2-O2 phase transition in 4.2-V plateau and shows poor cycling stability and rate capability within this plateau. To evaluate the practicability of this material in 2.3–4.1 V voltage range, single-crystal micro-sized P2-type Na2/3Ni1/3Mn2/3O2 with high rate capability and cycling stability is synthesized via polyvinylpyrrolidone (PVP)-combustion method. The electrochemical performance is evaluated by galvanostatic charge-discharge tests. The kinetics of Na+ intercalation/deintercalation is studied detailly with potential intermittent titration technique (PITT), galvanostatic intermittent titration technique (GITT) and cyclic voltammetry (CV). The discharge capacity at 0.1 C in 2.3–4.1 V is 87.6 mAh g−1. It can deliver 91.5% capacity at 40 C rate and keep 89% after 650 cycles at 5C. The calculated theoretical energy density of full cell with hard carbon anode is 210 Wh kg−1. The moderate energy density associated with high power density and long cycle life is acceptable for load adjustment of new-energy power, showing the prospect of practical application
Energy Spectra of Anti-nucleons in Finite Nuclei
The quantum vacuum in a many-body system of finite nuclei has been
investigated within the relativistic Hartree approach which describes the bound
states of nucleons and anti-nucleons consistently. The contributions of the
Dirac sea to the source terms of the meson-field equations are taken into
account up to the one-nucleon loop and one-meson loop. The tensor couplings for
the - and -meson are included in the model. The overall nucleon
spectra of shell-model states are in agreement with the data. The calculated
anti-nucleon spectra in the vacuum differ about 20 -- 30 MeV with and without
the tensor-coupling effects.Comment: 4 pages, to appear in the Proceedings of MENU 2004 (Beijing, Aug. 29
-- Sept. 4, 2004
Quantum Reciprocity Conjecture for the Non-Equilibrium Steady State
By considering the lack of history dependence in the non-equilibrium steady
state of a quantum system we are led to conjecture that in such a system, there
is a set of quantum mechanical observables whose retarded response functions
are insensitive to the arrow of time, and which consequently satisfy a quantum
analog of the Onsager reciprocity relations. Systems which satisfy this
conjecture can be described by an effective Free energy functional. We
demonstrate that the conjecture holds in a resonant level model of a multi-lead
quantum dot.Comment: References revised to take account of related work on Onsager
reciprocity in mesoscopics by Christen, and in hydrodynamics by Mclennan,
Dufty and Rub
Fractal Characterizations of MAX Statistical Distribution in Genetic Association Studies
Two non-integer parameters are defined for MAX statistics, which are maxima
of simpler test statistics. The first parameter, , is the
fractional number of tests, representing the equivalent numbers of independent
tests in MAX. If the tests are dependent, . The second
parameter is the fractional degrees of freedom of the chi-square
distribution that fits the MAX null distribution. These two
parameters, and , can be independently defined, and can be
non-integer even if is an integer. We illustrate these two parameters
using the example of MAX2 and MAX3 statistics in genetic case-control studies.
We speculate that is related to the amount of ambiguity of the model
inferred by the test. In the case-control genetic association, tests with low
(e.g. ) are able to provide definitive information about the disease
model, as versus tests with high (e.g. ) that are completely uncertain
about the disease model. Similar to Heisenberg's uncertain principle, the
ability to infer disease model and the ability to detect significant
association may not be simultaneously optimized, and seems to measure the
level of their balance
The Luminosity Function of high-redshift QSOs - A combined analysis of GOODS and SDSS
Aims: In this work the luminosity function of QSOs is measured in the
redshift range 3.5<z<5.2 for the absolute magnitude interval -21<M_{145}<-28.
The determination of the faint end of the luminosity function at these
redshifts provides important constraints on models of joint evolution of
galaxies and AGNs. Methods: We have defined suitable criteria to select faint
QSOs in the GOODS fields, checking in detail their effectiveness and
completeness. Spectroscopic follow-up of the resulting QSO candidates has been
carried out. The confirmed sample of faint QSOs is compared with a brighter one
derived from the SDSS. We have used a Monte-Carlo technique to estimate the
properties of the luminosity function, checking various parameterizations for
its shape and evolution. Results: Models based on Pure Density Evolution show
better agreement with observation than models based on Pure Luminosity
Evolution. However a different break magnitude with respect to z~2.1 is
required at 3.5<z<5.2. Models with a steeper faint end score a higher
probability. We do not find any evidence for a flattening of the bright end at
redshift z>3.5. Conclusions: The estimated space density evolution of QSOs
indicates a suppression of the formation and/or feeding of Supermassive Black
Holes at these redshifts. The QSO contribution to the UV background is
insufficient to ionize the IGM at 3.5<z<5.2.Comment: 17 pages, 13 ps figures, A&A accepted. Updated to journal versio
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