Violation of the Wiedemann-Franz law in clean graphene layers

The Wiedemann-Franz law, connecting the electronic thermal conductivity to the electrical conductivity of a disordered metal, is generally found to be well satisfied even when electron-electron (e-e) interactions are strong. In ultra-clean conductors, however, large deviations from the standard form of the law are expected, due to the fact that e-e interactions affect the two conductivities in radically different ways. Thus, the standard Wiedemann-Franz ratio between the thermal and the electric conductivity is reduced by a factor $1+\tau/\tau_{\rm th}^{\rm ee}$, where $1/\tau$ is the momentum relaxation rate, and $1/\tau_{\rm th}^{\rm ee}$ is the relaxation time of the thermal current due to e-e collisions. Here we study the density and temperature dependence of $1/\tau_{\rm th}^{\rm ee}$ in the important case of doped, clean single layers of graphene, which exhibit record-high thermal conductivities. We show that at low temperature $1/\tau_{\rm th}^{\rm ee}$ is $8/5$ of the quasiparticle decay rate. We also show that the many-body renormalization of the thermal Drude weight coincides with that of the Fermi velocity.Comment: 6 pages, 5 appendices (13 pages

Acoustic plasmons and "soundarons" in graphene on a metal gate

We demonstrate that single-layer graphene in the presence of a metal gate displays a gapless collective (plasmon) mode that has a linear dispersion at long wavelengths. We calculate exactly the acoustic-plasmon group velocity at the level of the random phase approximation and carry out microscopic calculations of the one-body spectral function of such system. Despite screening exerted by the metal, we find that graphene's quasiparticle spectrum displays a very rich structure characterized by composite hole-acoustic plasmon satellite bands (that we term for brevity "soundarons"), which can be observed by e.g. angle-resolved photoemission spectroscopy.Comment: 6 pages, 7 figure

Many-body orbital paramagnetism in doped graphene sheets

The orbital magnetic susceptibility (OMS) of a gas of noninteracting massless Dirac fermions is zero when the Fermi energy is away from the Dirac point. Making use of diagrammatic perturbation theory, we calculate exactly the OMS of massless Dirac fermions to first order in the Coulomb interaction demonstrating that it is finite and positive. Doped graphene sheets are thus unique systems in which the OMS is completely controlled by many-body effects.Comment: 4 pages, 2 figures, submitte

Theory of Coulomb drag for massless Dirac fermions

Coulomb drag between two unhybridized graphene sheets separated by a dielectric spacer has recently attracted considerable theoretical interest. We first review, for the sake of completeness, the main analytical results which have been obtained by other authors. We then illustrate pedagogically the minimal theory of Coulomb drag between two spatially-separated two-dimensional systems of massless Dirac fermions which are both away from the charge-neutrality point. This relies on second-order perturbation theory in the screened interlayer interaction and on Boltzmann transport theory. In this theoretical framework and in the low-temperature limit, we demonstrate that, to leading (i.e. quadratic) order in temperature, the drag transresistivity is completely insensitive to the precise intralayer momentum-relaxation mechanism (i.e. to the functional dependence of the scattering time on energy). We also provide analytical results for the low-temperature drag transresistivity for both cases of "thick" and "thin" spacers and for arbitrary values of the dielectric constants of the media surrounding the two Dirac-fermion layers. Finally, we present numerical results for the low-temperature drag transresistivity in the case in which one of the media surrounding the Dirac-fermion layers has a frequency-dependent dielectric constant. We conclude by suggesting an experiment that can potentially allow for the observation of departures from the canonical Fermi-liquid quadratic-in-temperature behavior of the transresistivity.Comment: 20 pages, 4 figure

Linear response of doped graphene sheets to vector potentials

URL:http://link.aps.org/doi/10.1103/PhysRevB.80.075418 DOI:10.1103/PhysRevB.80.075418A two-dimensional gas of massless Dirac fermions (MDFs) is a very useful model to describe low-energy electrons in monolayer graphene. Because the MDF current operator is directly proportional to the (sublattice) pseudospin operator, the MDF current-current response function, which describes the response to a vector potential, happens to coincide with the pseudospin-pseudospin response function. In this work, we present analytical results for the wave vector- and frequency-dependent longitudinal and transverse pseudospin-pseudospin response functions of noninteracting MDFs. The transverse response in the static limit is then used to calculate the noninteracting orbital magnetic susceptibility. These results are a starting point for the construction of approximate pseudospin-pseudospin response functions that would take into account electron-electron interactions (for example at the random-phase-approximation level). They also constitute a very useful input for future applications of current-density-functional theory to graphene sheets subjected to time and spatially varying vector potentials.M.P. was partially supported by the CNR-INFM “SeedProjects.” G.V. acknowledges support from NSF Grant No.DMR-0705460

Negative local resistance caused by viscous electron backflow in graphene

Graphene hosts a unique electron system in which electron-phonon scattering is extremely weak but electron-electron collisions are sufficiently frequent to provide local equilibrium above liquid nitrogen temperature. Under these conditions, electrons can behave as a viscous liquid and exhibit hydrodynamic phenomena similar to classical liquids. Here we report strong evidence for this transport regime. We find that doped graphene exhibits an anomalous (negative) voltage drop near current injection contacts, which is attributed to the formation of submicrometer-size whirlpools in the electron flow. The viscosity of graphene's electron liquid is found to be ~0.1 m$^2$ /s, an order of magnitude larger than that of honey, in agreement with many-body theory. Our work shows a possibility to study electron hydrodynamics using high quality graphene

On Coulomb drag in double layer systems

We argue, for a wide class of systems including graphene, that in the low temperature, high density, large separation and strong screening limits the drag resistivity behaves as d^{-4}, where d is the separation between the two layers. The results are independent of the energy dispersion relation, the dependence on momentum of the transport time, and the wave function structure factors. We discuss how a correct treatment of the electron-electron interactions in an inhomogeneous dielectric background changes the theoretical analysis of the experimental drag results of Ref. [1]. We find that a quantitative understanding of the available experimental data [1] for drag in graphene is lacking.Comment: http://iopscience.iop.org/0953-8984/24/33/335602

Plasmons and Coulomb drag in Dirac/Schroedinger hybrid electron systems

We show that the plasmon spectrum of an ordinary two-dimensional electron gas (2DEG) hosted in a GaAs heterostructure is significantly modified when a graphene sheet is placed on the surface of the semiconductor in close proximity to the 2DEG. Long-range Coulomb interactions between massive electrons and massless Dirac fermions lead to a new set of optical and acoustic intra-subband plasmons. Here we compute the dispersion of these coupled modes within the Random Phase Approximation, providing analytical expressions in the long-wavelength limit that shed light on their dependence on the Dirac velocity and Dirac-fermion density. We also evaluate the resistivity in a Coulomb-drag transport setup. These Dirac/Schroedinger hybrid electron systems are experimentally feasible and open new research opportunities for fundamental studies of electron-electron interaction effects in two spatial dimensions.Comment: 7 pages, 4 figure

Many-Body Orbital Paramagnetism in Doped Graphene Sheets

URL:http://link.aps.org/doi/10.1103/PhysRevLett.104.225503 DOI:10.1103/PhysRevLett.104.225503The orbital magnetic susceptibility of a gas of noninteracting massless Dirac fermions is zero when the Fermi energy is away from the Dirac point. Making use of diagrammatic perturbation theory, we calculate exactly the orbital magnetic susceptibility of massless Dirac fermions to first order in the Coulomb interaction demonstrating that it is finite and positive. Doped graphene sheets are thus unique systems in which the orbital magnetic susceptibility is completely controlled by many-body effects.We acknowledge financial support by the 2009/2010 CNR-CSIC scientific cooperation project (M. P.), by the NSF Grant No. DMR-0705460 (G.V.), and by FOM, the Netherlands (M. I. K.)