1,117 research outputs found

    Kinetic Anomalies in Addition-Aggregation Processes

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    We investigate irreversible aggregation in which monomer-monomer, monomer-cluster, and cluster-cluster reactions occur with constant but distinct rates K_{MM}, K_{MC}, and K_{CC}, respectively. The dynamics crucially depends on the ratio gamma=K_{CC}/K_{MC} and secondarily on epsilon=K_{MM}/K_{MC}. For epsilon=0 and gamma<2, there is conventional scaling in the long-time limit, with a single mass scale that grows linearly in time. For gamma >= 2, there is unusual behavior in which the concentration of clusters of mass k, c_k decays as a stretched exponential in time within a boundary layer k<k* propto t^{1-2/gamma} (k* propto ln t for gamma=2), while c_k propto t^{-2} in the bulk region k>k*. When epsilon>0, analogous behaviors emerge for gamma<2 and gamma >= 2.Comment: 6 pages, 2 column revtex4 format, for submission to J. Phys.

    Charge-transfer metal-insulator transitions in the spin-one-half Falicov-Kimball model

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    The spin-one-half Falicov-Kimball model is solved exactly on an infinite-coordination-number Bethe lattice in the thermodynamic limit. This model is a paradigm for a charge-transfer metal-insulator transition where the occupancy of localized and delocalized electronic orbitals rapidly changes at the metal-insulator transition (rather than the character of the electronic states changing from insulating to metallic as in a Mott-Hubbard transition). The exact solution displays both continuous and discontinuous (first-order) transitions.Comment: 22 pages including 4 figures(eps), RevTe

    A Survey of Numerical Solutions to the Coagulation Equation

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    We present the results of a systematic survey of numerical solutions to the coagulation equation for a rate coefficient of the form A_ij \propto (i^mu j^nu + i^nu j^mu) and monodisperse initial conditions. The results confirm that there are three classes of rate coefficients with qualitatively different solutions. For nu \leq 1 and lambda = mu + nu \leq 1, the numerical solution evolves in an orderly fashion and tends toward a self-similar solution at large time t. The properties of the numerical solution in the scaling limit agree with the analytic predictions of van Dongen and Ernst. In particular, for the subset with mu > 0 and lambda < 1, we disagree with Krivitsky and find that the scaling function approaches the analytically predicted power-law behavior at small mass, but in a damped oscillatory fashion that was not known previously. For nu \leq 1 and lambda > 1, the numerical solution tends toward a self-similar solution as t approaches a finite time t_0. The mass spectrum n_k develops at t_0 a power-law tail n_k \propto k^{-tau} at large mass that violates mass conservation, and runaway growth/gelation is expected to start at t_crit = t_0 in the limit the initial number of particles n_0 -> \infty. The exponent tau is in general less than the analytic prediction (lambda + 3)/2, and t_0 = K/[(lambda - 1) n_0 A_11] with K = 1--2 if lambda > 1.1. For nu > 1, the behaviors of the numerical solution are similar to those found in a previous paper by us. They strongly suggest that there are no self-consistent solutions at any time and that runaway growth is instantaneous in the limit n_0 -> \infty. They also indicate that the time t_crit for the onset of runaway growth decreases slowly toward zero with increasing n_0.Comment: 41 pages, including 14 figures; accepted for publication in J. Phys.

    IDLaS-NL – A platform for running customized studies on individual differences in Dutch language skills via the internet

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    We introduce the Individual Differences in Language Skills (IDLaS-NL) web platform, which enables users to run studies on individual differences in Dutch language skills via the internet. IDLaS-NL consists of 35 behavioral tests, previously validated in participants aged between 18 and 30 years. The platform provides an intuitive graphical interface for users to select the tests they wish to include in their research, to divide these tests into different sessions and to determine their order. Moreover, for standardized administration the platform provides an application (an emulated browser) wherein the tests are run. Results can be retrieved by mouse click in the graphical interface and are provided as CSV-file output via email. Similarly, the graphical interface enables researchers to modify and delete their study configurations. IDLaS-NL is intended for researchers, clinicians, educators and in general anyone conducting fundamental research into language and general cognitive skills; it is not intended for diagnostic purposes. All platform services are free of charge. Here, we provide a description of its workings as well as instructions for using the platform. The IDLaS-NL platform can be accessed at www.mpi.nl/idlas-nl

    Asymptotics of self-similar solutions to coagulation equations with product kernel

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    We consider mass-conserving self-similar solutions for Smoluchowski's coagulation equation with kernel K(ξ,η)=(ξη)λK(\xi,\eta)= (\xi \eta)^{\lambda} with λ(0,1/2)\lambda \in (0,1/2). It is known that such self-similar solutions g(x)g(x) satisfy that x1+2λg(x)x^{-1+2\lambda} g(x) is bounded above and below as x0x \to 0. In this paper we describe in detail via formal asymptotics the qualitative behavior of a suitably rescaled function h(x)=hλx1+2λg(x)h(x)=h_{\lambda} x^{-1+2\lambda} g(x) in the limit λ0\lambda \to 0. It turns out that h1+Cxλ/2cos(λlogx)h \sim 1+ C x^{\lambda/2} \cos(\sqrt{\lambda} \log x) as x0x \to 0. As xx becomes larger hh develops peaks of height 1/λ1/\lambda that are separated by large regions where hh is small. Finally, hh converges to zero exponentially fast as xx \to \infty. Our analysis is based on different approximations of a nonlocal operator, that reduces the original equation in certain regimes to a system of ODE

    Phase diagram of the quarter-filled extended Hubbard model on a two-leg ladder

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    We investigate the ground-state phase diagram of the quarter-filled Hubbard ladder with nearest-neighbor Coulomb repulsion V using the Density Matrix Renormalization Group technique. The ground-state is homogeneous at small V, a ``checkerboard'' charge--ordered insulator at large V and not too small on-site Coulomb repulsion U, and is phase-separated for moderate or large V and small U. The zero-temperature transition between the homogeneous and the charge-ordered phase is found to be second order. In both the homogeneous and the charge-ordered phases the existence of a spin gap mainly depends on the ratio of interchain to intrachain hopping. In the second part of the paper, we construct an effective Hamiltonian for the spin degrees of freedom in the strong-coupling charge-ordered regime which maps the system onto a frustrated spin chain. The opening of a spin gap is thus connected with spontaneous dimerization.Comment: 12 pages, 13 figures, submitted to PRB, presentation revised, new results added (metallic phase at small U and V

    Temporal variation in out-of-hospital cardiac arrest occurrence in individuals with or without diabetes

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    Objective: Out-of-hospital cardiac arrest (OHCA) occurrence has been shown to exhibit a circadian rhythm, following the circadian rhythm of acute myocardial infarction (AMI) occurrence. Diabetes mellitus (DM) is associated with changes in circadian rhythm. We aimed to compare the temporal variation of OHCA occurrence over the day and week between OHCA patients with DM and those without.Methods: In two population-based OHCA registries (Amsterdam Resuscitation Studies [ARREST] 2010-2016, n = 4163, and Danish Cardiac Arrest Registry [DANCAR], 2010-2014, n = 12,734), adults (≥18y) with presumed cardiac cause of OHCA and available medical history were included. Single and double cosinor analysis was performed to model circadian variation of OHCA occurrence. Stratified analysis of circadian variation was performed in patients with AMI as immediate cause of OHCA.Results: DM patients (22.8% in ARREST, 24.2% in DANCAR) were older and more frequently had cardiovascular risk factors or previous cardiovascular disease. Both cohorts showed 24 h-rhythmicity, with significant amplitudes in single and double cosinor functions (P-range &lt; 0.001). In both registries, a morning peak (10:00-11:00) and an evening peak (20:00-21:00) was observed in both DM and non-DM patients. No septadian variation was observed in either DM or non-DM patients (P-range 0.13-84).Conclusions: In these two population-based OHCA registries, we observed a similar circadian rhythm of OHCA occurrence in DM and non-DM patients.</p

    Scaling Theory for Migration-Driven Aggregate Growth

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    We give a comprehensive rate equation description for the irreversible growth of aggregates by migration from small to large aggregates. For a homogeneous rate K(i;j) at which monomers migrate from aggregates of size i to those of size j, that is, K(ai;aj) ~ a^{lambda} K(i,j), the mean aggregate size grows with time as t^{1/(2-lambda)} for lambda<2. The aggregate size distribution exhibits distinct regimes of behavior which are controlled by the scaling properties of the migration rate from the smallest to the largest aggregates. Our theory applies to diverse phenomena, such as the distribution of city populations, late stage coarsening of non-symmetric binary systems, and models for wealth exchange.Comment: 4 pages, 2-column revtex format. Revision to appear in PRL. Various changes in response to referee comments. Figure from version 1 deleted but is available at http://physics.bu.edu/~redne

    Multi-band Gutzwiller wave functions for general on-site interactions

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    We introduce Gutzwiller wave functions for multi-band models with general on-site Coulomb interactions. As these wave functions employ correlators for the exact atomic eigenstates they are exact both in the non-interacting and in the atomic limit. We evaluate them in infinite lattice dimensions for all interaction strengths without any restrictions on the structure of the Hamiltonian or the symmetry of the ground state. The results for the ground-state energy allow us to derive an effective one-electron Hamiltonian for Landau quasi-particles, applicable for finite temperatures and frequencies within the Fermi-liquid regime. As applications for a two-band model we study the Brinkman-Rice metal-to-insulator transition at half band-filling, and the transition to itinerant ferromagnetism for two specific fillings, at and close to a peak in the density of states of the non-interacting system. Our new results significantly differ from those for earlier Gutzwiller wave functions where only density-type interactions were included. When the correct spin symmetries for the two-electron states are taken into account, the importance of the Hund's-rule exchange interaction is even more pronounced and leads to paramagnetic metallic ground states with large local magnetic moments. Ferromagnetism requires fairly large interaction strengths, and the resulting ferromagnetic state is a strongly correlated metal.Comment: 37 pages, 10 figures; accepted for publication in Phys. Rev. B 57 (March 15, 1998

    Phase separation and enhanced charge-spin coupling near magnetic transitions

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    The generic changes of the electronic compressibility in systems which show magnetic instabilities is studied. It is shown that, when going into the ordered phase, the compressibility is reduced by an amount comparable to the its original value, making charge instabilities also possible. We discuss, within this framework, the tendency towards phase separation of the double exchange systems, the pyrochlores, and other magnetic materials
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