Histogram of Fuzzy Local Spatio-Temporal Descriptors for Video Action Recognition

Feature extraction plays a vital role in visual action recognition. Many existing gradient-based feature extractors, including histogram of oriented gradients (HOG), histogram of optical flow (HOF), motion boundary histograms (MBH), and histogram of motion gradients (HMG), build histograms for representing different actions over the spatio-temporal domain in a video. However, these methods require to set the number of bins for information aggregation in advance. Varying numbers of bins usually lead to inherent uncertainty within the process of pixel voting with regard to the bins in the histogram. This paper proposes a novel method to handle such uncertainty by fuzzifying these feature extractors. The proposed approach has two advantages: i) it better represents the ambiguous boundarie between the bins and thus the fuzziness of th spatio-temporal visual information entailed in videos, and ii) the contribution of each pixel is flexibly controlled by a fuzziness parameter for various scenarios. The proposed family of fuzzy descriptors and a combination of them were evaluate on two publicly available datasets, demonstrating that the proposed approach outperforms the original counterparts and other state-of-the-art methods

Femtosecond Photon-Mediated Plasma Enhances Photosynthesis of Plasmonic Nanostructures and Their SERS Applications

Laser ablation in liquid has proven to be a universal and green method to synthesize nanocrystals and fabricate functional nanostructures. This study demonstrates the superiority of femtosecond laser-mediated plasma in enhancing photoredox of metal cations for controllable fabrication of plasmonic nanostructures in liquid. Through employing upstream high energetic plasma during laser-induced microexplosions, single/three-electron photoreduction of metallic cations can readily occur without chemical reductants or capping agents. Experimental evidences demonstrate that this process exhibits higher photon utilization efficiency in yield of colloidal metal nanoparticles than direct irradiation of metallic precursors. Photogenerated hydrated electrons derived from strong ionization of silicon and water are responsible for this enhanced consequences. Furthermore, these metallic nanoparticles are accessible to self-assemble into nanoplates for silver and nanospheres for gold, favored by surface-tension gradients between laser irradiated and unirradiated regions. These metallic nanostructures exhibit excellent surface-enhanced Raman spectroscopy performance in trace detection of Rhodamine 6G (R6G), 4-mercaptobenzoic acid (4-MBA), and mercapto-5-nitrobenzimidazole molecules with high sensitivity (down to 10–12 mol L–1, 30 × 10–15 m for R6G), good reproducibility (relative standard deviation \u3c 7%), and good dual-analyte detection ability with mixture ratios of R6G to 4-MBA ranging from 20 to 0.025. The conceptual importance of this plasma-enhanced-photochemical process may provide exciting opportunities in photochemical reactions, plasmofluidics, and material synthesis. Includes Supplementary Material

Black Hole Mass Estimates and Rapid Growth of Supermassive Black Holes in Luminous z∼z \sim 3.5 Quasars

We present new near-infrared (IR) observations of the H$\beta\ \lambda4861$ and MgII $\lambda2798$ lines for 32 luminous quasars with $3.2<z<3.9$ using the Palomar Hale 200 inch telescope and the Large Binocular Telescope. We find that the MgII Full Width at Half Maximum (FWHM) is well correlated with the H$\beta$ FWHM, confirming itself as a good substitute for the H$\beta$ FWHM in the black hole mass estimates. The continuum luminosity at 5100 \AA\ well correlates with the continuum luminosity at 3000 \AA\ and the broad emission line luminosities (H$\beta$ and MgII). With simultaneous near-IR spectroscopy of the H$\beta$ and MgII lines to exclude the influences of flux variability, we are able to evaluate the reliability of estimating black hole masses based on the MgII line for high redshift quasars. With the reliable H$\beta$ line based black hole mass and Eddington ratio estimates, we find that the $z\sim3.5$ quasars in our sample have black hole masses $1.90\times10^{9} M_{\odot} \lesssim M_{\rm BH} \lesssim 1.37\times10^{10} M_{\odot}$, with a median of $\sim 5.14\times10^{9} M_{\odot}$ and are accreting at Eddington ratios between 0.30 and 3.05, with a median of $\sim1.12$. Assuming a duty cycle of 1 and a seed black hole mass of $10^{4} M_{\odot}$, we show that the $z\sim3.5$ quasars in this sample can grow to their estimated black hole masses within the age of the Universe at their redshifts.Comment: 38 pages, 6 figures, accepted for publication in Ap

An ultra-luminous quasar with a twelve-billion-solar-mass black hole at redshift 6.30

So far, roughly 40 quasars with redshifts greater than z=6 have been discovered. Each quasar contains a black hole with a mass of about one billion solar masses ($10^9 M_\odot$). The existence of such black holes when the Universe was less than 1 billion years old presents substantial challenges to theories of the formation and growth of black holes and the coevolution of black holes and galaxies. Here we report the discovery of an ultra-luminous quasar, SDSS J010013.02+280225.8, at redshift z=6.30. It has an optical and near-infrared luminosity a few times greater than those of previously known z>6 quasars. On the basis of the deep absorption trough on the blue side of the Ly $\alpha$ emission line in the spectrum, we estimate the proper size of the ionized proximity zone associated with the quasar to be 26 million light years, larger than found with other z>6.1 quasars with lower luminosities. We estimate (on the basis of a near-infrared spectrum) that the black hole has a mass of $\sim 1.2 \times 10^{10} M_\odot$, which is consistent with the $1.3 \times 10^{10} M_\odot$ derived by assuming an Eddington-limited accretion rate.Comment: 24 pages, 4 figures plus 4 extended data figures, published in Nature on 26 February 201

Photonic Hook-Assisted Contrast-Enhanced Super-Resolution Imaging Using Janus Microspheres

Microsphere-assisted imaging is a promising label- free super-resolution imaging technique. Its performance is sig- nificantly affected by the photonic nanojet (PNJ) of microspheres. Recently, a new type of curved PNJ, i.e. the photonic hook (PH), was discovered, which shows promising potential for various applications. This Letter presented a contrast-enhanced super- resolution imaging technique utilizing the PHs generated by Janus microspheres. We demonstrated that the Janus micro- spheres can be fabricated using a one-step deposition process, they exhibit superior imaging performance to pristine micro- spheres, and their field-of-view and imaging contrast can be easily adjusted by changing the coating thickness. In addition, we demonstrated that the imaging contrast of Janus microspheres can be further enhanced by using polarized illumination

Focusing light with a metal film coated patchy particle

Microsphere-assisted super-resolution imaging is a promising technique that can significantly enhance the resolution of conventional optical microscopes. The focus of a classical microsphere is called photonic nanojet, which is a symmetric high-intensity electromagnetic field. Recently, patchy microspheres have been reported to have superior imaging performance than pristine microspheres, and coating microspheres with metal films leads to the formation of photonic hooks, which can enhance the imaging contrast of microspheres. Understanding the influence of metal patches on the near-field focusing of patchy particles is important for the rational design of a nanostructured microlens. In this work, we theoretically and experimentally showed that the light waves can be focused and engineered using patchy particles. When coating dielectric particles with Ag films, light beams with a hook-like structure or S-shaped structure can be generated. Simulation results show that the waveguide ability of metal films and the geometric asymmetry of patchy particles cause the formation of S-shaped light beams. Compared with classical photonic hooks, S-shaped photonic hooks have a longer effective length and a smaller beam waist at far-field region. Experiments were also carried out to demonstrate the generation of classical and S-shaped photonic hooks from patchy microspheres

An ultra-luminous quasar at z=5.363 with a ten billion solar mass black hole and a Metal-Rich DLA at z~5

We report the discovery of an ultra-luminous quasar J030642.51+185315.8 (hereafter J0306+1853) at redshift 5.363, which hosts a super-massive black hole (SMBH) with $M_{BH} = (1.07 \pm 0.27) \times10^{10}~M_\odot$. With an absolute magnitude $M_{1450}=-28.92$ and bolometric luminosity $L_{bol}\sim3.4\times10^{14} L_{\odot}$, J0306+1853 is one of the most luminous objects in the early Universe. It is not likely to be a beamed source based on its small flux variability, low radio loudness and normal broad emission lines. In addition, a $z=4.986$ Damped Ly$\alpha$ system (DLA) with $\rm [M/H]=-1.3\pm0.1$, among the most metal rich DLAs at $z \gtrsim 5$, is detected in the absorption spectrum of this quasar. This ultra-luminous quasar puts strong constraint on the bright-end of quasar luminosity function and massive-end of black hole mass function. It will provide a unique laboratory to the study of BH growth and the co-evolution between BH and host galaxy with multi-wavelength follow-up observations. The future high resolution spectra will give more insights to the DLA and other absorption systems along the line-of-sight of J0306+1853.Comment: 5 pages, 3 figures, accepted for publication in ApJ

CIV emission line properties and uncertainties in black hole mass estimates of z ~ 3.5 quasars

Using a high luminosity ($L_{\rm bol} \sim 10^{47.5} - 10^{48.3}$ erg s$^{-1}$), high redshift ($3.2 < z < 3.8$) quasar sample of 19 quasars with optical and near-infrared spectroscopy, we investigate the reliability of the CIV-based black hole mass estimates ($M_{\rm BH}$). The median logarithm of the CIV- and H$\beta$-based $M_{\rm BH}$ ratios is 0.110 dex with the scatter of 0.647 dex. The CIV-to-H$\beta$ BH mass differences are significantly correlated with the CIV FWHMs, blueshifts and asymmetries. Corrections of the CIV FWHM using the blueshift and asymmetry reduce the scatter of the mass differences by $\sim$ 0.04-0.2 dex. Quasars in our sample accrete at the Eddington ratio $R_{\rm EDD}>0.3$ and cover a considerable range of blueshifts, with 18/19 of the quasars showing CIV blueshifts (with the median value of 1126 km s$^{-1}$) and 14/19 of the quasars showing CIV blueshifts larger than 500 km s$^{-1}$. It suggests that not all quasars with high Eddington ratios show large blueshifts. The Baldwin effect between the CIV rest-frame equivalent width (REW) and the continuum luminosity at 1350 \overset{\lower.5em\circ}{\mathrm{A}} is not seen, likely due to the limited luminosity range of our sample. We find a lack of flux in the red wing of the composite spectrum with larger CIV blueshift, and detect a higher ratio of [OIII] quasars with REW$_{\rm [OIII]}>5$ \overset{\lower.5em\circ}{\mathrm{A}} in the subsample with lower CIV blueshift. It is more likely that they are caused by the combination of the Eddington ratio and the orientation effect.Comment: 17 pages, 12 figures with additional 6 pages and 2 figures in the appendix. Accepted for publication in Ap

Generation of Photonic Hooks under Point-Source Illumination from Patchy Microcylinders

Photonic hook (PH) is a new type of non-evanescent light beam with subwavelength curved structures. It has shown promising applications in super-resolution imaging and has the potential to be used in micromachining, optical trapping, etc. PHs are generally produced by illuminating mesoscale asymmetric particles with optical plane waves. In this work, we used the finite-difference time-domain (FDTD) method to investigate the PH phenomenon under point-source illumination. We found that the PHs can be effectively generated from point-source illuminated patchy particles. By changing the background refractive index, particle diameters and the position and coverage ratio of Ag patches, the characteristics of the PHs can be effectively tuned. Moreover, the structure of the intensity distribution of the light field generated from small and large particles can have an opposite bending direction due to the near-field light-matter interaction

Preparation of Monolayer MoS\u3csub\u3e2\u3c/sub\u3e Quantum Dots using Temporally Shaped Femtosecond Laser Ablation of Bulk MoS\u3csub\u3e2\u3c/sub\u3e Targets in Water

Zero-dimensional MoS2 quantum dots (QDs) possess distinct physical and chemical properties, which have garnered them considerable attention and facilitates their use in a broad range of applications. In this study, we prepared monolayer MoS2 QDs using temporally shaped femtosecond laser ablation of bulk MoS2 targets in water. The morphology, crystal structures, chemical, and optical properties of the MoS2 QDs were characterized by transmission electron microscopy, X-ray diffraction, Raman spectroscopy, X-ray photoelectron spectroscopy, UV–vis absorption spectra, and photoluminescence spectra. The analysis results show that highly pure, uniform, and monolayer MoS2 QDs can be successfully prepared. Moreover, by temporally shaping a conventional single pulse into a two-subpulse train, the production rate of MoS2 nanomaterials (including nanosheets, nanoparticles, and QDs) and the ratio of small size MoS2 QDs can be substantially improved. The underlying mechanism is a combination of multilevel photoexfoliation of monolayer MoS2 and water photoionization–enhanced light absorption. The as-prepared MoS2 QDs exhibit excellent electrocatalytic activity for hydrogen evolution reactions because of the abundant active edge sites, high specific surface area, and excellent electrical conductivity. Thus, this study provides a simple and green alternative strategy for the preparation of monolayer QDs of transition metal dichalcogenides or other layered materials