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Evaluation of simulated O-3 production efficiency during the KORUS-AQ campaign: Implications for anthropogenic NOx emissions in Korea
We examine O3 production and its sensitivity to precursor gases and boundary layer mixing in Korea by using a 3-D global chemistry transport model and extensive observations during the KORea-US cooperative Air Quality field study in Korea, which occurred in May–June 2016. During the campaign, observed aromatic species onboard the NASA DC-8 aircraft, especially toluene, showed high mixing ratios of up to 10 ppbv, emphasizing the importance of aromatic chemistry in O3 production. To examine the role of VOCs and NOx in O3 chemistry, we first implement a detailed aromatic chemistry scheme in the model, which reduces the normalized mean bias of simulated O3 mixing ratios from –26% to –13%. Aromatic chemistry also increases the average net O3 production in Korea by 37%. Corrections of daytime PBL heights, which are overestimated in the model compared to lidar observations, increase the net O3 production rate by ~10%. In addition, increasing NOx emissions by 50% in the model shows best performance in reproducing O3 production characteristics, which implies that NOx emissions are underestimated in the current emissions inventory. Sensitivity tests show that a 30% decrease in anthropogenic NOx emissions in Korea increases the O3 production efficiency throughout the country, making rural regions ~2 times more efficient in producing O3 per NOx consumed. Simulated O3 levels overall decrease in the peninsula except for urban and other industrial areas, with the largest increase (~6 ppbv) in the Seoul Metropolitan Area (SMA). However, with simultaneous reductions in both NOx and VOCs emissions by 30%, O3 decreases in most of the country, including the SMA. This implies the importance of concurrent emission reductions for both NOx and VOCs in order to effectively reduce O3 levels in Korea
Faithful test of non-local realism with entangled coherent states
We investigate the violation of Leggett's inequality for non-local realism
using entangled coherent states and various types of local measurements. We
prove mathematically the relation between the violation of the
Clauser-Horne-Shimony-Holt form of Bell's inequality and Leggett's one when
tested by the same resources. For Leggett inequalities, we generalize the
non-local realistic bound to systems in Hilbert spaces larger than
bidimensional ones and introduce an optimization technique that allows to
achieve larger degrees of violation by adjusting the local measurement
settings. Our work describes the steps that should be performed to produce a
self-consistent generalization of Leggett's original arguments to
continuous-variable states.Comment: 8 pages, 6 figures, to be published in Phys. Rev.
Effects of squeezing on quantum nonlocality of superpositions of coherent states
We analyze effects of squeezing upon superpositions of coherent states (SCSs)
and entangled coherent states (ECSs) for Bell-inequality tests. We find that
external squeezing can always increase the degrees of Bell violations, if the
squeezing direction is properly chosen, for the case of photon parity
measurements. On the other hand, when photon on/off measurements are used, the
squeezing operation can enhance the degree of Bell violations only for moderate
values of amplitudes and squeezing. We point out that a significant improvement
is required over currently available squeezed SCSs in order to directly
demonstrate a Bell-inequality violation in a real experiment.Comment: 7 pages, 4 figures, accepted for publication in Phys. Rev.
Inverted polymer fullerene solar cells exceeding 10% efficiency with poly(2-ethyl-2-oxazoline) nanodots on electron-collecting buffer layers
Polymer solar cells have been spotlighted due to their potential for low-cost manufacturing but their efficiency is still less than required for commercial application as lightweight/flexible modules. Forming a dipole layer at the electron-collecting interface has been suggested as one of the more attractive approaches for efficiency enhancement. However, only a few dipole layer material types have been reported so far, including only one non-ionic (charge neutral) polymer. Here we show that a further neutral polymer, namely poly(2-ethyl-2-oxazoline) (PEOz) can be successfully used as a dipole layer. Inclusion of a PEOz layer, in particular with a nanodot morphology, increases the effective work function at the electron-collecting interface within inverted solar cells and thermal annealing of PEOz layer leads to a state-of-the-art 10.74% efficiency for single-stack bulk heterojunction blend structures comprising poly[4,8-bis(5-(2-ethylhexyl)thiophen-2-yl)benzo[1,2-b:4,5-b′]dithiophene-alt-3-fluorothieno[3,4-b]thiophene-2-carboxylate] as donor and [6,6]-phenyl-C71-butyric acid methyl ester as acceptor
Preliminary evaluation of a reaction control system for the space station
The challenge, ground rules and criteria, some of the Reaction Control System (RCS) concepts, classical and modern design analysis, and simulation results which are applicable to the space station are presented
Single-photon detection timing jitter in a visible light photon counter
Visible light photon counters (VLPCs) offer many attractive features as
photon detectors, such as high quantum efficiency and photon number resolution.
We report measurements of the single-photon timing jitter in a VLPC, a critical
performance factor in a time-correlated single-photon counting measurement, in
a fiber-coupled closed-cycle cryocooler. The measured timing jitter is 240 ps
full-width-at-half-maximum at a wavelength of 550 nm, with a dark count rate of
25 000 counts per second. The timing jitter increases modestly at longer
wavelengths to 300 ps at 1000 nm, and increases substantially at lower bias
voltages as the quantum efficiency is reduced
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