4,747 research outputs found
Limits to compression with cascaded quadratic soliton compressors
We study cascaded quadratic soliton compressors and address the physical
mechanisms that limit the compression. A nonlocal model is derived, and the
nonlocal response is shown to have an additional oscillatory component in the
nonstationary regime when the group-velocity mismatch (GVM) is strong. This
inhibits efficient compression. Raman-like perturbations from the cascaded
nonlinearity, competing cubic nonlinearities, higher-order dispersion, and
soliton energy may also limit compression, and through realistic numerical
simulations we point out when each factor becomes important. We find that it is
theoretically possible to reach the single-cycle regime by compressing
high-energy fs pulses for wavelengths in a
-barium-borate crystal, and it requires that the system is in the
stationary regime, where the phase mismatch is large enough to overcome the
detrimental GVM effects. However, the simulations show that reaching
single-cycle duration is ultimately inhibited by competing cubic nonlinearities
as well as dispersive waves, that only show up when taking higher-order
dispersion into account.Comment: 16 pages, 5 figures, submitted to Optics Expres
Nonlocal explanation of stationary and nonstationary regimes in cascaded soliton pulse compression
We study soliton pulse compression in materials with cascaded quadratic
nonlinearities, and show that the group-velocity mismatch creates two different
temporally nonlocal regimes. They correspond to what is known as the stationary
and nonstationary regimes. The theory accurately predicts the transition to the
stationary regime, where highly efficient pulse compression is possible.Comment: 3 pages, 2 figures, published verison in Optics Letters. Contains
revised equations, including an updated mode
Ultrafast and octave-spanning optical nonlinearities from strongly phase-mismatched cascaded interactions
Cascaded nonlinearities have attracted much interest, but ultrafast
applications have been seriously hampered by the simultaneous requirements of
being near phase-matching and having ultrafast femtosecond response times. Here
we show that in strongly phase-mismatched nonlinear frequency conversion
crystals the pump pulse can experience a large and extremely broadband
self-defocusing cascaded Kerr-like nonlinearity. The large cascaded
nonlinearity is ensured through interaction with the largest quadratic tensor
element in the crystal, and the strong phase-mismatch ensures an ultrafast
nonlinear response with an octave-spanning bandwidth. We verify this
experimentally by showing few-cycle soliton compression with noncritical
cascaded second-harmonic generation: Energetic 47 fs infrared pulses are
compressed in a just 1-mm long bulk lithium niobate crystal to 17 fs (under 4
optical cycles) with 80% efficiency, and upon further propagation an
octave-spanning supercontinuum is observed. Such ultrafast cascading is
expected to occur for a broad range of pump wavelengths spanning the near- and
mid-IR using standard nonlinear crystals.Comment: resubmitted, revised version, accepted for Phys. Rev. Let
Pulse generation without gain-bandwidth limitation in a laser with self-similar evolution
With existing techniques for mode-locking, the bandwidth of ultrashort pulses from a laser is determined primarily by the spectrum of the gain medium. Lasers with self-similar evolution of the pulse in the gain medium can tolerate strong spectral breathing, which is stabilized by nonlinear attraction to the parabolic self-similar pulse. Here we show that this property can be exploited in a fiber laser to eliminate the gain-bandwidth limitation to the pulse duration. Broad (̃200 nm) spectra are generated through passive nonlinear propagation in a normal-dispersion laser, and these can be dechirped to ̃20-fs duration
Criteria for the experimental observation of multi-dimensional optical solitons in saturable media
Criteria for experimental observation of multi-dimensional optical solitons
in media with saturable refractive nonlinearities are developed. The criteria
are applied to actual material parameters (characterizing the cubic
self-focusing and quintic self-defocusing nonlinearities, two-photon loss, and
optical-damage threshold) for various glasses. This way, we identify operation
windows for soliton formation in these glasses. It is found that two-photon
absorption sets stringent limits on the windows. We conclude that, while a
well-defined window of parameters exists for two-dimensional solitons (spatial
or spatiotemporal), for their three-dimensional spatiotemporal counterparts
such a window \emph{does not} exist, due to the nonlinear loss in glasses.Comment: 8 pages, to appear in Phys. Rev.
A new chiral electro-optic effect: Sum-frequency generation from optically active liquids in the presence of a dc electric field
We report the observation of sum-frequency signals that depend linearly on an
applied electrostatic field and that change sign with the handedness of an
optically active solution. This recently predicted chiral electro-optic effect
exists in the electric-dipole approximation. The static electric field gives
rise to an electric-field-induced sum-frequency signal (an achiral third-order
process) that interferes with the chirality-specific sum-frequency at
second-order. The cross-terms linear in the electrostatic field constitute the
effect and may be used to determine the absolute sign of second- and
third-order nonlinear optical susceptibilities in isotropic media.Comment: Submitted to Physical Revie
Electronic states and optical properties of PbSe nanorods and nanowires
A theory of the electronic structure and excitonic absorption spectra of PbS
and PbSe nanowires and nanorods in the framework of a four-band effective mass
model is presented. Calculations conducted for PbSe show that dielectric
contrast dramatically strengthens the exciton binding in narrow nanowires and
nanorods. However, the self-interaction energies of the electron and hole
nearly cancel the Coulomb binding, and as a result the optical absorption
spectra are practically unaffected by the strong dielectric contrast between
PbSe and the surrounding medium. Measurements of the size-dependent absorption
spectra of colloidal PbSe nanorods are also presented. Using room-temperature
energy-band parameters extracted from the optical spectra of spherical PbSe
nanocrystals, the theory provides good quantitative agreement with the measured
spectra.Comment: 35 pages, 12 figure
Realization of a semiconductor-based cavity soliton laser
The realization of a cavity soliton laser using a vertical-cavity
surface-emitting semiconductor gain structure coupled to an external cavity
with a frequency-selective element is reported. All-optical control of bistable
solitonic emission states representing small microlasers is demonstrated by
injection of an external beam. The control scheme is phase-insensitive and
hence expected to be robust for all-optical processing applications. The
motility of these structures is also demonstrated
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