Experimental Proof of a Magnetic Coulomb Phase

Spin ice materials are magnetic substances in which the spin directions map onto hydrogen positions in water ice. Recently this analogy has been elevated to an electromagnetic equivalence, indicating that the spin ice state is a Coulomb phase, with magnetic monopole excitations analogous to ice's mobile ionic defects. No Coulomb phase has yet been proved in a real magnetic material, as the key experimental signature is difficult to resolve in most systems. Here we measure the scattering of polarised neutrons from the prototypical spin ice Ho2Ti2O7. This enables us to separate different contributions to the magnetic correlations to clearly demonstrate the existence of an almost perfect Coulomb phase in this material. The temperature dependence of the scattering is consistent with the existence of deconfined magnetic monopoles connected by Dirac strings of divergent length.Comment: 18 pages, 4 fig

StepFormer: Self-supervised Step Discovery and Localization in Instructional Videos

Instructional videos are an important resource to learn procedural tasks from human demonstrations. However, the instruction steps in such videos are typically short and sparse, with most of the video being irrelevant to the procedure. This motivates the need to temporally localize the instruction steps in such videos, i.e. the task called key-step localization. Traditional methods for key-step localization require video-level human annotations and thus do not scale to large datasets. In this work, we tackle the problem with no human supervision and introduce StepFormer, a self-supervised model that discovers and localizes instruction steps in a video. StepFormer is a transformer decoder that attends to the video with learnable queries, and produces a sequence of slots capturing the key-steps in the video. We train our system on a large dataset of instructional videos, using their automatically-generated subtitles as the only source of supervision. In particular, we supervise our system with a sequence of text narrations using an order-aware loss function that filters out irrelevant phrases. We show that our model outperforms all previous unsupervised and weakly-supervised approaches on step detection and localization by a large margin on three challenging benchmarks. Moreover, our model demonstrates an emergent property to solve zero-shot multi-step localization and outperforms all relevant baselines at this task.Comment: CVPR'2

Glass Transition in the Polaron Dynamics of CMR Manganites

Neutron scattering measurements on a bilayer manganite near optimal doping show that the short-range polarons correlations are completely dynamic at high T, but then freeze upon cooling to a temperature T* 310 K. This glass transition suggests that the paramagnetic/insulating state arises from an inherent orbital frustration that inhibits the formation of a long range orbital- and charge-ordered state. Upon further cooling into the ferromagnetic-metallic state (Tc=114 K), where the polarons melt, the diffuse scattering quickly develops into a propagating, transverse optic phonon.Comment: 4 pages, 4 figures. Physical Review Letters (in Press

Pressure induced electronic and structural phase evolution in Van der Waals compound FePS3_3

Two-dimensional materials have proven to be a prolific breeding ground of new and unstudied forms of magnetism and unusual metallic states, particularly when tuned between their insulating and metallic phases. In this paper we present work on a new metal to insulator transition system FePS3 . This compound is a two-dimensional van-der-Waals antiferromagnetic Mott insulator. Here we report the discovery of an insulator-metal transition in FePS3, as evidenced by x-ray diffraction and electrical transport measurements, using high pressure as a tuning parameter. Two structural phase transitions are observed in the x-ray diffraction data as a function of pressure and resistivity measurements show evidence of the onset of a metallic state at high pressures. We propose models for the two new structures that can successfully explain the x-ray diffraction patterns