141 research outputs found
High Curie temperature and perpendicular magnetic anisotropy in homoepitaxial InMnAs films
We have prepared the dilute magnetic semiconductor (DMS) InMnAs with
different Mn concentrations by ion implantation and pulsed laser melting. The
Curie temperature of the In1-xMnxAs epilayer depends on the Mn concentration x,
reaching 82 K for x=0.105. The substitution of Mn ions at the Indium sites
induces a compressive strain perpendicular to the InMnAs layer and a tensile
strain along the in-plane direction. This gives rise to a large perpendicular
magnetic anisotropy, which is often needed for the demonstration of electrical
control of magnetization and for spin-transfer-torque induced magnetization
reversal.Comment: 16 pages, 5 figure
Electronic structure, magnetic and dielectric properties of the edge-sharing copper-oxide chain compound NaCuO
We report an experimental study of \nco, a Mott insulator containing chains
of edge-sharing CuO plaquettes, by polarized x-ray absorption spectroscopy
(XAS), resonant magnetic x-ray scattering (RMXS), magnetic susceptibility, and
pyroelectric current measurements. The XAS data show that the valence holes
reside exclusively on the Cu sites within the copper-oxide spin chains
and populate a -orbital polarized within the CuO plaquettes. The RMXS
measurements confirm the presence of incommensurate magnetic order below a
N\'eel temperature of K, which was previously inferred from
neutron powder diffraction and nuclear magnetic resonance data. In conjunction
with the magnetic susceptibility and XAS data, they also demonstrate a new
"orbital" selection rule for RMXS that is of general relevance for magnetic
structure determinations by this technique. Dielectric property measurements
reveal the absence of significant ferroelectric polarization below , which
is in striking contrast to corresponding observations on the isostructural
compound \lco. The results are discussed in the context of current theories of
multiferroicity.Comment: 7 pages, 7 figure
Bandgap narrowing in Mn doped GaAs probed by room-temperature photoluminescence
The electronic band structure of the (Ga,Mn)As system has been one of the
most intriguing problems in solid state physics over the past two decades.
Determination of the band structure evolution with increasing Mn concentration
is a key issue to understand the origin of ferromagnetism. Here we present room
temperature photoluminescence and ellipsometry measurements of
Ga_{100%-x}Mn_{x}As alloy. The up-shift of the valence-band is proven by the
red shift of the room temperature near band gap emission from the
Ga_{100%-x}Mn_{x}As alloy with increasing Mn content. It is shown that even a
doping by 0.02 at.% of Mn affects the valence-band edge and it merges with the
impurity band for a Mn concentration as low as 0.6 at.%. Both X-ray diffraction
pattern and high resolution cross-sectional TEM images confirmed full
recrystallization of the implanted layer and GaMnAs alloy formation.Comment: 24 pages, 7 figures, accepted at Phys. Rev. B 201
Direct observation of t2g orbital ordering in magnetite
Using soft-x-ray diffraction at the site-specific resonances in the Fe L23
edge, we find clear evidence for orbital and charge ordering in magnetite below
the Verwey transition. The spectra show directly that the (001/2) diffraction
peak (in cubic notation) is caused by t2g orbital ordering at octahedral Fe2+
sites and the (001) by a spatial modulation of the t2g occupation.Comment: to appear in Phys. Rev. Let
Iron porphyrin molecules on Cu(001): Influence of adlayers and ligands on the magnetic properties
The structural and magnetic properties of Fe octaethylporphyrin (OEP)
molecules on Cu(001) have been investigated by means of density functional
theory (DFT) methods and X-ray absorption spectroscopy. The molecules have been
adsorbed on the bare metal surface and on an oxygen-covered surface, which
shows a reconstruction. In order to allow
for a direct comparison between magnetic moments obtained from sum-rule
analysis and DFT we calculate the dipolar term , which is also
important in view of the magnetic anisotropy of the molecule. The measured
X-ray magnetic circular dichroism shows a strong dependence on the photon
incidence angle, which we could relate to a huge value of , e.g. on
Cu(001) amounts to -2.07\,\mbo{} for normal incidence leading to a
reduction of the effective spin moment . Calculations have also
been performed to study the influence of possible ligands such as Cl and O
atoms on the magnetic properties of the molecule and the interaction between
molecule and surface, because the experimental spectra display a clear
dependence on the ligand, which is used to stabilize the molecule in the gas
phase. Both types of ligands weaken the hybridization between surface and
porphyrin molecule and change the magnetic spin state of the molecule, but the
changes in the X-ray absorption are clearly related to residual Cl ligands.Comment: 17 figures, full articl
Functional Genomics for Tolerance to Abiotic Stress in Cereals
The world food grain production needs to be doubled by
the year 2050 to meet the ever growing demands of the
population (Tilman et al., 2002). This goal needs to be achieved despite
decreased arable land, dwindling water resources, and the environmental
constraints such as drought, water logging, excess heat, frost, salinity, metal
toxicity and nutrient imbalances, which cause major losses in cereal grain
production. Drought, salinity and cold stress alone are known to cause
nearly 35% of cereal crop losses throughout the world (Quarrie et al., 1999).
The effectiveness of traditional breeding approaches to deal with the
problem is limited due to complex nature of stress tolerance traits and due to
incompatibility barriers encountered during transfer of genes from wild
species to cultivated ones. Therefore, newer strategies need to be used for
developing crop plants tha
CeRuSn: a strongly correlated material with nontrivial topology
Topological insulators form a novel state of matter that provides new
opportunities to create unique quantum phenomena. While the materials used so
far are based on semiconductors, recent theoretical studies predict that also
strongly correlated systems can show non-trivial topological properties,
thereby allowing even the emergence of surface phenomena that are not possible
with topological band insulators. From a practical point of view, it is also
expected that strong correlations will reduce the disturbing impact of defects
or impurities, and at the same increase the Fermi velocities of the topological
surface states. The challenge is now to discover such correlated materials.
Here, using advanced x-ray spectroscopies in combination with band structure
calculations, we infer that CeRuSn is a strongly correlated material
with non-trivial topology.Comment: 10 pages, 6 figures, submitted to Scientific Report
The temperature dependent bandstructure of a ferromagnetic semiconductor film
The electronic quasiparticle spectrum of a ferromagnetic film is investigated
within the framework of the s-f model. Starting from the exact solvable case of
a single electron in an otherwise empty conduction band being exchange coupled
to a ferromagnetically saturated localized spin system we extend the theory to
finite temperatures. Our approach is a moment-conserving decoupling procedure
for suitable defined Green functions. The theory for finite temperatures
evolves continuously from the exact limiting case. The restriction to zero
conduction band occupation may be regarded as a proper model description for
ferromagnetic semiconductors like EuO and EuS. Evaluating the theory for a
simple cubic film cut parallel to the (100) crystal plane, we find some marked
correlation effects which depend on the spin of the test electron, on the
exchange coupling, and on the temperature of the local-moment system.Comment: 11 pages, 9 figure
Connection between charge-density-wave order and charge transport in the cuprate superconductors
Charge-density-wave (CDW) correlations within the quintessential CuO
planes have been argued to either cause [1] or compete with [2] the
superconductivity in the cuprates, and they might furthermore drive the
Fermi-surface reconstruction in high magnetic fields implied by quantum
oscillation (QO) experiments for YBaCuO (YBCO) [3] and
HgBaCuO (Hg1201) [4]. Consequently, the observation of bulk
CDW order in YBCO was a significant development [5,6,7]. Hg1201 features
particularly high structural symmetry and recently has been demonstrated to
exhibit Fermi-liquid charge transport in the relevant temperature-doping range
of the phase diagram, whereas for YBCO and other cuprates this underlying
property of the CuO planes is partially or fully masked [8-10]. It
therefore is imperative to establish if the pristine transport behavior of
Hg1201 is compatible with CDW order. Here we investigate Hg1201 ( = 72 K)
via bulk Cu L-edge resonant X-ray scattering. We indeed observe CDW
correlations in the absence of a magnetic field, although the correlations and
competition with superconductivity are weaker than in YBCO. Interestingly, at
the measured hole-doping level, both the short-range CDW and Fermi-liquid
transport appear below the same temperature of about 200 K. Our result points
to a unifying picture in which the CDW formation is preceded at the higher
pseudogap temperature by = 0 magnetic order [11,12] and the build-up of
significant dynamic antiferromagnetic correlations [13]. Furthermore, the
smaller CDW modulation wave vector observed for Hg1201 is consistent with the
larger electron pocket implied by both QO [4] and Hall-effect [14]
measurements, which suggests that CDW correlations are indeed responsible for
the low-temperature QO phenomenon
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