Scattering-Independent Anomalous Nernst Effect in Ferromagnets

Using the full-potential linearized augmented plane-wave method within the density functional theory, we compute all contributions to the scattering independent part of the thermoelectric conductivity tensor, namely the intrinsic contribution and the side-jump contribution. For the ferromagnetic materials bcc Fe, hcp Co, fcc Ni and L1_0 ordered alloys FePd and FePt, our investigations of the energy and temperature dependence of the intrinsic and side-jump contributions show that they are both of equal importance. Overall, our calculations are able to correctly reproduce the order of magnitude and sign of the experimentally measured signal, suggesting that the scattering independent part plays an important role in the anomalous Nernst effect of ferromagnets.Comment: 5 pages, 2 figures plus supplement, accepted for publication as a Rapid Communication in Physical Review

Anomalous Hall effect in ferromagnets with Gaussian disorder

Using the Kubo formalism we derived expressions and implemented the method for calculating the anomalous Hall conductivity (AHC) in ferromagnets with short-range Gaussian disorder directly from first-principles electronic structure of the perfect crystal. We used this method to calculate the AHC in bcc Fe, fcc Co, L1o-FePd, L1o-FePt as well as thin bcc Fe(001) films. Within our approach we can transparently decompose the conductivity into intrinsic (IC), side jump (SJ) and intrinsic skew-scattering (ISK) contributions. The existence of ISK, which originates from asymmetric Mott scattering but is clearly distinguishable from conventional skew-scattering in that it converges to a finite value in clean limit, was pointed out by Sinitsyn et al. [Phys. Rev. B 75, 045315 (2007)]. Here, we collect all contributions to the AHC in ferromagnets which result in "scattering-independent" AHE in clean limit, and analyze their relative magnitude from first principles calculations. By comparing our results to existing experiments we show that the Gaussian disorder is well suited to model various types of disorder present in real materials, to some extent including the effect of temperature. In particular, we show that in addition to intrinsic and side-jump AHE, the intrinsic skew-scattering can be a major player in determining the magnitude of the AHE in ferromagnets.Comment: 10 pages, 3 figure

Ab Initio Theory of Scattering-Independent Anomalous Hall Effect

We report on first-principles calculations of the side-jump contribution to the anomalous Hall conductivity (AHC) directly from the electronic structure of a perfect crystal. We implemented our approach for a short-range scattering disorder model within the density functional theory and computed the full scattering-independent AHC in elemental bcc Fe, hcp Co, fcc Ni, and L1o FePd and FePt alloys. The full AHC thus calculated agrees systematically with experiment to a degree unattainable so far, correctly capturing the previously missing elements of side-jump contributions, hence paving the way to a truly predictive theory of the anomalous Hall effect and turning it from a characterization tool to a probing tool of multi-band complex electronic band structures.Comment: PRL in pres

Anisotropy of spin relaxation and transverse transport in metals

Using first principles methods we explore the anisotropy of the spin relaxation and transverse transport properties in bulk metals with respect to the direction of the spin quantization axis in paramagnets or of the spontaneous magnetization in ferromagnets. Owing to the presence of the spin-orbit interaction the orbital and spin character of the Bloch states depends sensitively on the orientation of the spins relative to the crystal axes. This leads to drastic changes in quantities which rely on interband mixing induced by the spin-orbit interaction. The anisotropy is particularly striking for quantities which exhibit spiky and irregular distribution in the Brillouin zone, such as the spin-mixing parameter or the Berry curvature of the electronic states. We demonstrate this for three cases: (i) the Elliott-Yafet spin-relaxation mechanism in paramagnets with structural inversion symmetry; (ii) the intrinsic anomalous Hall effect in ferromagnets; and (iii) the spin Hall effect in paramagnets. We discuss the consequences of the pronounced anisotropic behavior displayed by these properties for spin-polarized transport applications.Comment: Psi-k Highlight 111 (2012