Probing internucleus potential with large-angle quasi-elastic scattering

FUSION06 : reaction mechanisms and nuclear structure at the Coulomb barrier : San Servolo, Venezia, Italy 19-23 March 2006 / editors, Lorenzo Corradi ... [et al.

Probing surface diffuseness of nucleus-nucleus potential with quasielastic scattering at deep sub-barrier energies

We perform a systematic study on the surface property of nucleus-nucleus potential in heavy-ion reactions using large-angle quasielastic scattering at energies well below the Coulomb barrier. At these energies, the quasielastic scattering can be well described by a single-channel potential model. Exploiting this fact, we point out that systems which involve spherical nuclei require the diffuseness parameter of around 0.60 fm in order to fit the experimental data, while systems with a deformed target between 0.8 fm and 1.1 fm.Comment: 6 pages, 6 figure

Extraction of nucleus-nucleus potential and energy dissipation from dynamical mean-field theory

Nucleus-nucleus interaction potentials in heavy-ion fusion reactions are extracted from the microscopic time-dependent Hartree-Fock theory. When the center-of-mass energy is much higher than the Coulomb barrier energy, extracted potentials identify with the frozen density approximation. As the center-of-mass energy decreases to the Coulomb barrier energy, potentials become energy dependent. This dependence indicates dynamical reorganization of internal degrees of freedom and leads to a reduction of the "apparent" barrier. Including this effect leads to the Coulomb barrier energy very close to experimental one. Aspects of one-body energy dissipation extracted from the mean-field theory are discussed.Comment: 6 pages, 5 figures. Uses aipxfm.sty. A talk given at the FUSION08: New Aspects of Heavy Ion Collisions Near the Coulomb Barrier, September 22-26, 2008, Chicago, US

Quantum effects in the diffusion process to form a heavy nucleus in heavy-ion fusion reactions

We discuss quantum effects in the diffusion process which is used to describe the shape evolution from the touching configuration of fusing two nuclei to a compound nucleus. Applying the theory with quantum effects to the case where the potential field, the mass and friction parameters are adapted to realistic values of heavy-ion collisions, we show that the quantum effects play significant roles at low temperatures which are relevant to the synthesis of superheavy elements

On nucleon exchange mechanism in heavy-ion collisions at near-barrier energies

Nucleon drift and diffusion mechanisms in central collisions of asymmetric heavy-ions at near-barrier energies are investigated in the framework of a stochastic mean-field approach. Expressions for diffusion and drift coefficients for nucleon transfer deduced from the stochastic mean-field approach in the semiclassical approximation have similar forms familiar from the phenomenological nucleon exchange model. The variance of fragment mass distribution agrees with the empirical formula $\sigma^2_{AA}(t)= N_{\rm exc}(t)$. The comparison with the time-dependent Hartree-Fock calculations shows that, below barrier energies, the drift coefficient in the semiclassical approximation underestimates the mean number of nucleon transfer obtained in the quantal framework. Motion of the window in the dinuclear system has a significant effect on the nucleon transfer in asymmetric collisions.Comment: 10 pages, 10 figures, submitted for publicatio

Fluctuation and dissipation dynamics in fusion reactions from stochastic mean-field approach

By projecting the stochastic mean-field dynamics on a suitable collective path during the entrance channel of heavy-ion collisions, expressions for transport coefficients associated with relative distance are extracted. These transport coefficients, which have similar forms to those familiar from nucleon exchange model, are evaluated by carrying out TDHF simulations. The calculations provide an accurate description of the magnitude and form factor of transport coefficients associated with one-body dissipation and fluctuation mechanism.Comment: 9 pages, 5 figure

Molecular weight effects on chain pull-out fracture of reinforced polymeric interfaces

Using Brownian dynamics, we simulate the fracture of polymer interfaces reinforced by diblock connector chains. We find that for short chains the interface fracture toughness depends linearly on the degree of polymerization $N$ of the connector chains, while for longer chains the dependence becomes $N^{3/2}$. Based on the geometry of initial chain configuration, we propose a scaling argument that accounts for both short and long chain limits and crossover between them.Comment: 5 pages, 3 figure

Mass dispersion in transfer reactions with a stochastic mean-field theory

Nucleon transfer in symmetric heavy-ion reactions at energies below the Coulomb barrier is investigated in the framework of a microscopic stochastic mean-field theory. While mean-field alone is known to significantly underpredict the dispersion of the fragment mass distribution, a considerable enhancement of the dispersion is obtained in the stochastic mean-field theory. The variance of the fragment mass distribution deduced from the stochastic theory scales with the number of exchanged nucleon. Therefore, the new approach provides the first fully microscopic theory consistent with the phenomenological analysis of the experimental data.Comment: 4 pages, 2 figures, 1 tabl

Extraction of astatine isotopes for development of radiopharmaceuticals using a 211Rn–211At generator

In order to utilize a 211At isotope, a promising α-emitter for radionuclide therapy, the chemical properties of astatine isotopes are studied. We have examined wet chemistry methods through the distribution ratios of astatine in liquid–liquid extraction. The astatine isotopes have been found to be well extracted into DIPE and MIBK. We observed that the distribution ratio of astatine isotopes increases with concentrations of HCl greater than 3 M, while it decreases with the HCl concentration less than 2 M. The results will be useful for development of the 211Rn–211At generator