309 research outputs found
Shock enhancement and control of hypersonic mixing and combustion
The possibility that shock enhanced mixing can
substantially increase the rate of mixing between
coflowing streams of hydrogen and air has been
studied in experimental and computational investigations.
Early numerical computations indicated that
the steady interaction between a weak shock in air
with a coflowing hydrogen jet can be well approximated
by the two-dimensional time-dependent interaction
between a weak shock and an initially circular
region filled with hydrogen imbedded in air. An experimental
investigation of the latter process has been
carned out in the Caltech 17 Inch Shock Tube in experiments
in which the laser induced fluorescence of
byacetyl dye is used as a tracer for the motion of the
helium gas after shock waves have passed across the
helium cylinder. The flow field has also been studied
using an Euler code computation of the flow field.
Both investigations show that the shock impinging
process causes the light gas cylinder to split into two
parts. One of these mixes rapidly with air and the
other forms a stably stratified vortex pair which mixes
more slowly; about 60% of the light gas mixes rapidly
with the ambient fluid. The geometry of the flow field
and the mixing process and scaling parameters are
discussed here. The success of this program encouraged
the exploration of a low drag injection system in
which the basic concept of shock generated streamwise
vorticity could be incorporated in an injector for
a Scramjet combustor at Mach numbers between 5
and 8. The results of a substantial computational
program and a description of the wind tunnel model and preliminary experimental results obtained in the
High Reynolds Number Mach 6 Tunnel at NASA Langley
Research Center are given here
Interatomic-Coulombic-decay-induced recapture of photoelectrons in helium dimers
We investigate the onset of photoionization shakeup induced interatomic
Coulombic decay (ICD) in He2 at the He+*(n = 2) threshold by detecting two He+
ions in coincidence. We find this threshold to be shifted towards higher
energies compared to the same threshold in the monomer. The shifted onset of
ion pairs created by ICD is attributed to a recapture of the threshold
photoelectron after the emission of the faster ICD electron.Comment: 5 Pages, 2 Figure
Vibrationally Resolved Decay Width of Interatomic Coulombic Decay in HeNe
We investigate the ionization of HeNe from below the He 1s3p excitation to
the He ionization threshold. We observe HeNe ions with an enhancement by
more than a factor of 60 when the He side couples resonantly to the radiation
field. These ions are an experimental proof of a two-center resonant
photoionization mechanism predicted by Najjari et al. [Phys. Rev. Lett. 105,
153002 (2010)]. Furthermore, our data provide electronic and vibrational state
resolved decay widths of interatomic Coulombic decay (ICD) in HeNe dimers. We
find that the ICD lifetime strongly increases with increasing vibrational
state.Comment: 7 pages, 5 figure
A measurement of the evolution of Interatomic Coulombic Decay in the time domain
During the last 15 years a novel decay mechanism of excited atoms has been
discovered and investigated. This so called ''Interatomic Coulombic Decay''
(ICD) involves the chemical environment of the electronically excited atom: the
excitation energy is transferred (in many cases over long distances) to a
neighbor of the initially excited particle usually ionizing that neighbor. It
turned out that ICD is a very common decay route in nature as it occurs across
van-der-Waals and hydrogen bonds. The time evolution of ICD is predicted to be
highly complex, as its efficiency strongly depends on the distance of the atoms
involved and this distance typically changes during the decay. Here we present
the first direct measurement of the temporal evolution of ICD using a novel
experimental approach.Comment: 6 pages, 4 figures, submitted to PR
Sub-harmonic resonant excitation of confined acoustic modes at GHz frequencies with a high-repetition-rate femtosecond laser
We propose sub-harmonic resonant optical excitation with femtosecond lasers
as a new method for the characterization of phononic and nanomechanical systems
in the gigahertz to terahertz frequency range. This method is applied for the
investigation of confined acoustic modes in a free-standing semiconductor
membrane. By tuning the repetition rate of a femtosecond laser through a
sub-harmonic of a mechanical resonance we amplify the mechanical amplitude,
directly measure the linewidth with megahertz resolution, infer the lifetime of
the coherently excited vibrational states, accurately determine the system's
quality factor, and determine the amplitude of the mechanical motion with
femtometer resolution
Ion and Electron Momentum Distributions from Single and Double Ionization of Helium Induced by Compton Scattering
We present the momentum distributions of the nucleus and of the electrons from double ionization of the helium atom by Compton scattering of photons with hÎœ=40ââkeV. We find that the doubly charged ion momentum distribution is very close to the Compton profile of the nucleus in the ground state of the helium atom, and the momentum distribution of the singly charged ion to give a precise image of the electron Compton profile. To reproduce these results, nonrelativistic calculations require the use of highly correlated initial- and final-state wave functions
Aristotleâs assertoric syllogistic and modern relevance logic
This paper sets out to evaluate the claim that Aristotleâs Assertoric Syllogistic is a relevance logic or shows significant similarities with it. I prepare the grounds for a meaningful comparison by extracting the notion of relevance employed in the most influential work on modern relevance logic, Anderson and Belnapâs Entailment. This notion is characterized by two conditions imposed on the concept of validity: first, that some meaning content is shared between the premises and the conclusion, and second, that the premises of a proof are actually used to derive the conclusion. Turning to Aristotleâs Prior Analytics, I argue that there is evidence that Aristotleâs Assertoric Syllogistic satisfies both conditions. Moreover, Aristotle at one point explicitly addresses the potential harmfulness of syllogisms with unused premises. Here, I argue that Aristotleâs analysis allows for a rejection of such syllogisms on formal grounds established in the foregoing parts of the Prior Analytics. In a final section I consider the view that Aristotle distinguished between validity on the one hand and syllogistic validity on the other. Following this line of reasoning, Aristotleâs logic might not be a relevance logic, since relevance is part of syllogistic validity and not, as modern relevance logic demands, of general validity. I argue that the reasons to reject this view are more compelling than the reasons to accept it and that we can, cautiously, uphold the result that Aristotleâs logic is a relevance logic
Photoelectron circular dichroism of O 1-photoelectrons of uniaxially oriented trifluoromethyloxirane: Energy dependence and sensitivity to molecular configuration
The photoelectron circular dichroism (PECD) of the O 1s-photoelectrons of
trifluoromethyloxirane(TFMOx) is studied experimentally and theoretically for
different photoelectron kinetic energies. The experiments were performed
employing circularly polarized synchrotron radiation and coincidentelectron and
fragment ion detection using Cold Target Recoil Ion Momentum Spectroscopy. The
corresponding calculations were performed by means of the Single Center method
within the relaxed-core Hartree-Fock approximation. We concentrate on the
energy dependence of the differential PECD of uniaxially oriented TFMOx
molecules, which is accessible through the employed coincident detection. We
also compare results for differential PECD of TFMOx to those obtained for the
equivalent fragmentation channel and similar photoelectron kinetic energy of
methyloxirane (MOx), studied in our previous work. Thereby, we investigate the
influence of the substitution of the methyl-group by the trifluoromethyl-group
at the chiral center on the molecular chiral response. Finally, the presently
obtained angular distribution parameters are compared to those available in
literature.Comment: 6 fig
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