730 research outputs found
Enhancing the Catalytic Activity of Palladium Nanoparticles via Sandwich-Like Confinement by Thin Titanate Nanosheets
As atomically thin oxide layers deposited on flat (noble) metal surfaces have been proven to have a significant influence on the electronic structure and thus the catalytic activity of the metal, we sought to mimic this architecture at the bulk scale. This could be achieved by intercalating small positively charged Pd nanoparticles of size 3.8 nm into a nematic liquid crystalline phase of lepidocrocite-type layered titanate. Upon intercalation the galleries collapsed and Pd nanoparticles were captured in a sandwichlike mesoporous architecture showing good accessibility to Pd nanoparticles. On the basis of X-ray photoelectron spectroscopy (XPS) and CO diffuse reflectance Fourier transform infrared spectroscopy (DRIFTS) Pd was found to be in a partially oxidized state, while a reduced Ti species indicated an electronic interaction between nanoparticles and nanosheets. The close contact of titanate sandwiching Pd nanoparticles, moreover, allows for the donation of a lattice oxygen to the noble metal (inverse spillover). Due to the metal–support interactions of this peculiar support, the catalyst exhibited the oxidation of CO with a turnover frequency as high as 0.17 s–1 at a temperature of 100 °C
A Measurement of the Coulomb Dissociation of 8B at 254 MeV/nucleon and the 8B Solar Neutrino Flux
We have measured the Coulomb dissociation of 8B into 7Be and proton at 254
MeV/nucleon using a large-acceptance focusing spectrometer. The astrophysical
S17 factor for the 7Be(p,gamma)8B reaction at E{c.m.} = 0.25-2.78 MeV is
deduced yielding S17(0)=20.6 \pm 1.2 (exp.) \pm 1.0 (theo.) eV-b.
This result agrees with the presently adopted zero-energy S17 factor obtained
in direct-reaction measurements and with the results of other
Coulomb-dissociation studies performed at 46.5 and 51.2 MeV/nucleon.Comment: paper to be published in Phys. Rev. Lett. 3 figures. New Version
fixes formatting problems with the figures only. There are no other change
Patterned growth of InGaN/GaN quantum wells on freestanding GaN grating by molecular beam epitaxy
We report here the epitaxial growth of InGaN/GaN quantum wells on freestanding GaN gratings by molecular beam epitaxy (MBE). Various GaN gratings are defined by electron beam lithography and realized on GaN-on-silicon substrate by fast atom beam etching. Silicon substrate beneath GaN grating region is removed from the backside to form freestanding GaN gratings, and the patterned growth is subsequently performed on the prepared GaN template by MBE. The selective growth takes place with the assistance of nanoscale GaN gratings and depends on the grating period P and the grating width W. Importantly, coalescences between two side facets are realized to generate epitaxial gratings with triangular section. Thin epitaxial gratings produce the promising photoluminescence performance. This work provides a feasible way for further GaN-based integrated optics devices by a combination of GaN micromachining and epitaxial growth on a GaN-on-silicon substrate
Observation of Hadronic W Decays in t-tbar Events with the Collider Detector at Fermilab
We observe hadronic W decays in t-tbar -> W (-> l nu) + >= 4 jet events using
a 109 pb-1 data sample of p-pbar collisions at sqrt{s} = 1.8 TeV collected with
the Collider Detector at Fermilab (CDF). A peak in the dijet invariant mass
distribution is obtained that is consistent with W decay and inconsistent with
the background prediction by 3.3 standard deviations. From this peak we measure
the W mass to be 77.2 +- 4.6 (stat+syst) GeV/c^2. This result demonstrates the
presence of two W bosons in t-tbar candidates in the W (-> l nu) + >= 4 jet
channel.Comment: 20 pages, 4 figures, submitted to PR
Measurement of the lepton charge asymmetry in W-boson decays produced in p-pbar collisions
We describe a measurement of the charge asymmetry of leptons from W boson
decays in the rapidity range 0 enu, munu events from
110+/-7 pb^{-1}of data collected by the CDF detector during 1992-95. The
asymmetry data constrain the ratio of d and u quark momentum distributions in
the proton over the x range of 0.006 to 0.34 at Q2 \approx M_W^2. The asymmetry
predictions that use parton distribution functions obtained from previously
published CDF data in the central rapidity region (0.0<|y_l|<1.1) do not agree
with the new data in the large rapidity region (|y_l|>1.1).Comment: 13 pages, 3 tables, 1 figur
Search for Narrow Diphoton Resonances and for gamma-gamma+W/Z Signatures in p\bar p Collisions at sqrt(s)=1.8 TeV
We present results of searches for diphoton resonances produced both
inclusively and also in association with a vector boson (W or Z) using 100
pb^{-1} of p\bar p collisions using the CDF detector. We set upper limits on
the product of cross section times branching ratio for both p\bar
p\to\gamma\gamma + X and p\bar p\to\gamma\gamma + W/Z. Comparing the inclusive
production to the expectations from heavy sgoldstinos we derive limits on the
supersymmetry-breaking scale sqrt{F} in the TeV range, depending on the
sgoldstino mass and the choice of other parameters. Also, using a NLO
prediction for the associated production of a Higgs boson with a W or Z boson,
we set an upper limit on the branching ratio for H\to\gamma\gamma. Finally, we
set a lower limit on the mass of a `bosophilic' Higgs boson (e.g. one which
couples only to \gamma, W, and Z$ bosons with standard model couplings) of 82
GeV/c^2 at 95% confidence level.Comment: 30 pages, 11 figure
Measurement of the Associated Production Cross Section in Collisions at TeV
We present the first measurement of associated direct photon + muon
production in hadronic collisions, from a sample of 1.8 TeV
collisions recorded with the Collider Detector at Fermilab. Quantum
chromodynamics (QCD) predicts that these events are primarily from the Compton
scattering process , with the final state charm quark producing
a muon. Hence this measurement is sensitive to the charm quark content of the
proton. The measured cross section of is compared to a
leading-order QCD parton shower model as well as a next-to-leading-order QCD
calculation.Comment: 12 pages, 4 figures Added more detailed description of muon
background estimat
Measurement of the top quark mass and top-antitop production cross section from dilepton events at the Collider Detector at Fermilab
We present an analysis of dilepton events originating from top-antitop
production in proton-antiproton collisions at sqrt{s}=1.8 TeV at the Fermilab
Tevatron Collider. The sample corresponds to an integrated luminosity of 109+-7
pb^{-1}. We observe 9 candidate events, with an estimated background of
2.4+-0.5 events. We determine the mass of the top quark to be M_top =
161+-17(stat.)+-10(syst.) GeV/c^2. In addition we measure a top-antitop
production cross section of 8.2+4.4-3.4 pb (where M_top = 175 GeV/c^2 has been
assumed for the acceptance estimate).Comment: 6 pages of text, 3 figure
Search for a Technicolor omega_T Particle in Events with a Photon and a b-quark Jet at CDF
If the Technicolor omega_T particle exists, a likely decay mode is omega_T ->
gamma pi_T, followed by pi_T -> bb-bar, yielding the signature gamma bb-bar. We
have searched 85 pb^-1 of data collected by the CDF experiment at the Fermilab
Tevatron for events with a photon and two jets, where one of the jets must
contain a secondary vertex implying the presence of a b quark. We find no
excess of events above standard model expectations. We express the result of an
exclusion region in the M_omega_T - M_pi_T mass plane.Comment: 14 pages, 2 figures. Available from the CDF server (PS with figs):
http://www-cdf.fnal.gov/physics/pub98/cdf4674_omega_t_prl_4.ps
FERMILAB-PUB-98/321-
Search for the Supersymmetric Partner of the Top-Quark in Collisions at
We report on a search for the supersymmetric partner of the top quark (stop)
produced in events using of
collisions at recorded with the Collider Detector at
Fermilab. In the case of a light stop squark, the decay of the top quark into
stop plus the lightest supersymmetric particle (LSP) could have a significant
branching ratio. The observed events are consistent with Standard Model production and decay. Hence, we set limits on the branching ratio of
the top quark decaying into stop plus LSP, excluding branching ratios above 45%
for a LSP mass up to 40 {\rm GeV/c}.Comment: 11 pages, 4 figure
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