70 research outputs found
On-chain electrodynamics of metallic (TMTSF)_2 X salts: Observation of Tomonaga-Luttinger liquid response
We have measured the electrodynamic response in the metallic state of three
highly anisotropic conductors, (TMTSF)_2 X, where X=PF_6, AsF_6, or ClO_4, and
TMTSF is the organic molecule tetramethyltetraselenofulvalene. In all three
cases we find dramatic deviations from a simple Drude response. The optical
conductivity has two features: a narrow mode at zero frequency, with a small
spectral weight, and a mode centered around 200 cm^{-1}, with nearly all of the
spectral weight expected for the relevant number of carriers and single
particle bandmass. We argue that these features are characteristic of a nearly
one-dimensional half- or quarter-filled band with Coulomb correlations, and
evaluate the finite energy mode in terms of a one-dimensional Mott insulator.
At high frequencies (\hbar\omega > t_\perp, the transfer integral perpendicular
to the chains), the frequency dependence of the optical conductivity
\sigma_1(\omega) is in agreement with calculations based on an interacting
Tomonaga-Luttinger liquid, and is different from what is expected for an
uncorrelated one-dimensional semiconductor. The zero frequency mode shows
deviations from a simple Drude response, and can be adequately described with a
frequency dependent mass and relaxation rate.Comment: 12 pages, 7 figures, RevTeX; minor corrections to text and
references; To be published in Phys. Rev. B, 15 July 199
Thermal Imaging of Nanostructures by Quantitative Optical Phase Analysis
International audienceWe introduce an optical microscopy technique aimed at characterizing the heat generation arising from nanostructures, in a comprehensive and quantitative manner. Namely, the technique permits (i) mapping the temperature distribution around the source of heat, (ii) mapping the heat power density delivered by the source, and (iii) retrieving the absolute absorption cross section of light-absorbing structures. The technique is based on the measure of the thermal-induced refractive index variation of the medium surrounding the source of heat. The measurement is achieved using an association of a regular CCD camera along with a modified Hartmann diffraction grating. Such a simple association makes this technique straightforward to implement on any conventional microscope with its native broadband illumination conditions. We illustrate this technique on gold nanoparticles illuminated at their plasmonic resonance. The spatial resolution of this technique is diffraction limited, and temperature variations weaker than 1 K can be detected
Maskless Plasmonic Lithography at 22 nm Resolution
Optical imaging and photolithography promise broad applications in nano-electronics, metrologies, and single-molecule biology. Light diffraction however sets a fundamental limit on optical resolution, and it poses a critical challenge to the down-scaling of nano-scale manufacturing. Surface plasmons have been used to circumvent the diffraction limit as they have shorter wavelengths. However, this approach has a trade-off between resolution and energy efficiency that arises from the substantial momentum mismatch. Here we report a novel multi-stage scheme that is capable of efficiently compressing the optical energy at deep sub-wavelength scales through the progressive coupling of propagating surface plasmons (PSPs) and localized surface plasmons (LSPs). Combining this with airbearing surface technology, we demonstrate a plasmonic lithography with 22 nm half-pitch resolution at scanning speeds up to 10 m/s. This low-cost scheme has the potential of higher throughput than current photolithography, and it opens a new approach towards the next generation semiconductor manufacturing
Optical and infrared properties of tetramethyltetraselenafulvalene [(TMTSF)2X] and tetramethyltetrathiafulvalene [(TMTTF)2X] compounds
A polarizing situation: Taking an in-plane perspective for next-generation near-field studies
Near-Field Radiation from a Ridge Waveguide Transducer in the Vicinity of a Solid Immersion Lens
Heat-assisted magnetic recording by a near-field transducer with efficient optical energy transfer
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