159 research outputs found
Shallow seismic sounding based on ellipticity analysis of microtremor
A brief review is carried out of the previous study about the spectral ratios of horizontal and vertical components of microseismic oscillations displacement. The basic principles of resonant boundaries allocation and the construction of deep sections based on the H/V relations (ellipticity) are considered. A description of the equipment used, the method of recording and processing microseismic noise are presented. The main goal of the research work is to clarify the nature of the connection between the ellipticity of microseisms with geological features and the correctness of constructing deep sections based on them. The initial data are the amplitude spectra of the components of microseismic signal, obtained using the fast Fourier transformation. In the course of experimental work it was found that the spectral relations retain their characteristic features regardless of the azimuth of observations. A number of practical examples compare microseismic sections with results from other geophysical methods and drilling information. The results obtained indicate the complex nature of the ellipticity of microseismic noise under different conditions, however, they make it possible to determine the main interfaces between the upper part of the geological section. Resonant boundaries emitted by microtremor are often located near refractive seismic boundaries. This is consistent with the theory that resonance effects occur at the interface between two media with a high contrast of acoustic impedance
Compacton-like solutions of the hydrodynamic system describing relaxing media
We show the existence of a compacton-like solutions within the relaxing
hydrodynamic-type model and perform numerical study of attracting features of
these solutions
Nanosized carbon forms in the processes of pressure–temperature-induced transformations of hydrocarbons
The products of thermal conversions of naphthalene, anthracene, pentacene, perylene, and coronene at 8 GPa in the temperature range up to 1300 C have been studied by scanning electron and high-resolution transmission electron microscopies. As a result, it has been established that various nanometer-sized carbon species (spherical and coalesced two-core onion-like carbon particles, faceted polyhedral particles, graphitic ribbons, graphitic folds, and nanocrystalline diamonds) are present in the conversion products together with micron-sized crystallites of graphite and diamond. 2006 Elsevier Ltd. All rights reserved
Exciton Dephasing and Thermal Line Broadening in Molecular Aggregates
Using a model of Frenkel excitons coupled to a bath of acoustic phonons in
the host medium, we study the temperature dependence of the dephasing rates and
homogeneous line width in linear molecular aggregates. The model includes
localization by disorder and predicts a power-law thermal scaling of the
effective homogeneous line width. The theory gives excellent agreement with
temperature dependent absorption and hole-burning experiments on aggregates of
the dye pseudoisocyanine.Comment: 11 pages, 3 PostScript figure
Ultrabright single-photon emission from germanium-vacancy zero-phonon lines: deterministic emitter-waveguide interfacing at plasmonic hot spots
Striving for nanometer-sized solid-state single-photon sources, we investigate atom-like quantum emitters based on single germanium-vacancy (GeV) centers isolated in crystalline nanodiamonds (NDs). Cryogenic characterization indicated symmetry-protected and bright (>106 counts/s with off-resonance excitation) zero-phonon optical transitions with up to 6-fold enhancement in energy splitting of their ground states as compared to that found for GeV centers in bulk diamonds (i.e. up to 870 GHz in highly strained NDs vs. 150 GHz in bulk). Utilizing lithographic alignment techniques, we demonstrate an integrated nanophotonic platform for deterministic interfacing plasmonic waveguides with isolated GeV centers in NDs, which enables 10-fold enhancement of single-photon decay rates along with the emission direction control by judiciously designing and positioning a Bragg reflector. This approach allows one to realize the unidirectional emission from single-photon dipolar sources, thereby opening new perspectives for the realization of quantum optical integrated circuits
Low-temperature quenching of one-dimensional localised Frenkel excitons
We present a theoretical analysis of low-temperature quenching of
one-dimensional Frenkel excitons that are localised by moderate on-site
(diagonal) uncorrelated disorder. Exciton diffusion is considered as an
incoherent hopping over localization segments and is probed by the exciton
fluorescence quenching at point traps. The rate equation is used to calculate
the temperature dependence of the exciton quenching. The activation temperature
of the diffusion is found to be of the order of the width of the exciton
absorption band. We demonstrate that the intra-segment scattering is extremely
important for the exciton diffusion. We discuss also experimental data on the
fast exciton-exciton annihilation in linear molecular aggregates at low
temperatures.Comment: 7 pages, 3 figures, accepted to Chem. Phys. Let
Far-infrared vibrational properties of high-pressure-high-temperature C60 polymers and the C60 dimer
We report high-resolution far-infrared transmission measurements of the 2 + 2 cycloaddition C-60 dimer and two-dimensional rhombohedral and one-dimensional orthorhombic high-pressure high-temperature C60 polymers. In the spectral region investigated(20-650 cm(-1)), we see no low-energy interball modes, but symmetry breaking of the linked C-60 balls is evident in the complex spectrum of intramolecular modes. Experimental features suggest large splittings or frequency shifts of some IhC60-derived modes that are activated by symmetry reduction, implying that the balls are strongly distorted in these structures. We have calculated the vibrations of all three systems by first-principles quantum molecular dynamics and use them to assign the predominant IhC60 symmetries of observed modes. Pur calculations show unprecedentedly large downshifts of T-1u(2)-derived modes and extremely large splittings of other modes, both of which are consistent with the experimental spectra. For the rhombohedral and orthorhombic polymers, the T-1u(2)-derived mode that is polarized along the bonding direction is calculated to downshift below any T-1u(1)-derived modes. We also identify a previously unassigned feature near 610 cm(-1) in all three systems as a widely split or shifted mode derived from various silent IhC60 vibrations, confirming a strong perturbation model for these linked fullerene structures
Linear optical properties of one-dimensional Frenkel exciton systems with intersite energy correlations
We analyze the effects of intersite energy correlations on the linear optical
properties of one-dimensional disordered Frenkel exciton systems. The
absorption line width and the factor of radiative rate enhancement are studied
as a function of the correlation length of the disorder. The absorption line
width monotonously approaches the seeding degree of disorder on increasing the
correlation length. On the contrary, the factor of radiative rate enhancement
shows a non-monotonous trend, indicating a complicated scenario of the exciton
localization in correlated systems. The concept of coherently bound molecules
is exploited to explain the numerical results, showing good agreement with
theory. Some recent experiments are discussed in the light of the present
theory.Comment: 18 pages, 3 figues, REVTeX, to appear in Physical Review
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