4,735 research outputs found
Momentum space tomographic imaging of photoelectrons
We apply tomography, a general method for reconstructing 3-D distributions
from multiple projections, to reconstruct the momentum distribution of
electrons produced via strong field photoionization. The projections are
obtained by rotating the electron distribution via the polarization of the
ionizing laser beam and recording a momentum spectrum at each angle with a 2-D
velocity map imaging spectrometer. For linearly polarized light the tomographic
reconstruction agrees with the distribution obtained using an Abel inversion.
Electron tomography, which can be applied to any polarization, will simplify
the technology of electron imaging. The method can be directly generalized to
other charged particles.Comment: Accepted by J. Phys.
A two-dimensional, two-electron model atom in a laser pulse: exact treatment, single active electron-analysis, time-dependent density functional theory, classical calculations, and non-sequential ionization
Owing to its numerical simplicity, a two-dimensional two-electron model atom,
with each electron moving in one direction, is an ideal system to study
non-perturbatively a fully correlated atom exposed to a laser field. Frequently
made assumptions, such as the ``single active electron''- approach and
calculational approximations, e.g. time dependent density functional theory or
(semi-) classical techniques, can be tested. In this paper we examine the
multiphoton short pulse-regime. We observe ``non-sequential'' ionization, i.e.\
double ionization at lower field strengths as expected from a sequential,
single active electron-point of view. Since we find non-sequential ionization
also in purely classical simulations, we are able to clarify the mechanism
behind this effect in terms of single particle trajectories. PACS Number(s):
32.80.RmComment: 10 pages, 16 figures (gzipped postscript), see also
http://www.physik.tu-darmstadt.de/tqe
Websites recommended to patients with adolescent idiopathic scoliosis at first point of diagnosis: a content analysis
Anisotropic splitting of intersubband spin plasmons in quantum wells with bulk and structural inversion asymmetry
In semiconductor heterostructures, bulk and structural inversion asymmetry
and spin-orbit coupling induce a k-dependent spin splitting of valence and
conduction subbands, which can be viewed as being caused by momentum-dependent
crystal magnetic fields. This paper studies the influence of these effective
magnetic fields on the intersubband spin dynamics in an asymmetric n-type
GaAs/AlGaAs quantum well. We calculate the dispersions of intersubband spin
plasmons using linear response theory. The so-called D'yakonov-Perel'
decoherence mechanism is inactive for collective intersubband excitations,
i.e., crystal magnetic fields do not lead to decoherence of spin plasmons.
Instead, we predict that the main signature of bulk and structural inversion
asymmetry in intersubband spin dynamics is a three-fold, anisotropic splitting
of the spin plasmon dispersion. The importance of many-body effects is pointed
out, and conditions for experimental observation with inelastic light
scattering are discussed.Comment: 8 pages, 6 figure
EUV ionization of pure He nanodroplets: Mass-correlated photoelectron imaging, Penning ionization and electron energy-loss spectra
The ionization dynamics of pure He nanodroplets irradiated by EUV radiation
is studied using Velocity-Map Imaging PhotoElectron-PhotoIon COincidence
(VMI-PEPICO) spectroscopy. We present photoelectron energy spectra and angular
distributions measured in coincidence with the most abundant ions He+, He2+,
and He3+. Surprisingly, below the autoionization threshold of He droplets we
find indications for multiple excitation and subsequent ionization of the
droplets by a Penning-like process. At high photon energies we evidence
inelastic collisions of photoelectrons with the surrounding He atoms in the
droplets
C in intense femtosecond laser pulses: nonlinear dipole response and ionization
We study the interaction of strong femtosecond laser pulses with the C
molecule employing time-dependent density functional theory with the ionic
background treated in a jellium approximation. The laser intensities considered
are below the threshold of strong fragmentation but too high for perturbative
treatments such as linear response. The nonlinear response of the model to
excitations by short pulses of frequencies up to 45eV is presented and analyzed
with the help of Kohn-Sham orbital resolved dipole spectra. In femtosecond
laser pulses of 800nm wavelength ionization is found to occur multiphoton-like
rather than via excitation of a ``giant'' resonance.Comment: 14 pages, including 1 table, 5 figure
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Photoluminescence lineshape of ZnO
The merger of the absorption coefficient dispersion, retrieved from transmission by the modified Urbach rule introduced by Ullrich and Bouchenaki [Jpn. J. Appl. Phys. 30, L1285, 1991], with the extended Roosbroeck-Shockley relation reveals that the optical absorption in ZnO distinctively determines the photoluminescence lineshape. Additionally, the ab initio principles employed enable the accurate determination of the carrier lifetime without further specific probing techniques
Thermal expansion in small metal clusters and its impact on the electric polarizability
The thermal expansion coefficients of clusters with and , and
are obtained from {\it ab initio} Born-Oppenheimer LDA molecular dynamics.
Thermal expansion of small metal clusters is considerably larger than that in
the bulk and size-dependent. We demonstrate that the average static electric
dipole polarizability of Na clusters depends linearly on the mean interatomic
distance and only to a minor extent on the detailed ionic configuration when
the overall shape of the electron density is enforced by electronic shell
effects. The polarizability is thus a sensitive indicator for thermal
expansion. We show that taking this effect into account brings theoretical and
experimental polarizabilities into quantitative agreement.Comment: 4 pages, 2 figures, one table. Accepted for publication in Physical
Review Letters. References 10 and 23 update
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