Quantum optical signatures in strong-field laser physics: Infrared photon counting in high-order-harmonic generation

We analytically describe the strong-field light-electron interaction using a quantized coherent laser state with arbitrary photon number. We obtain a light-electron wave function which is a closed-form solution of the time-dependent Schrodinger equation (TDSE). This wave function provides information about the quantum optical features of the interaction not accessible by semi-classical theories. With this approach we can reveal the quantum optical properties of high harmonic generation (HHG) process in gases by measuring the photon statistics of the transmitted infrared (IR) laser radiation. This work can lead to novel experiments in high-resolution spectroscopy in extreme-ultraviolet (XUV) and attosecond science without the need to measure the XUV light, while it can pave the way for the development of intense non-classical light sources.Comment: 9 pages, 4 figure

High-order harmonics measured by the photon statistics of the infrared driving-field exiting the atomic medium

High-order harmonics in the extreme-ultraviolet spectral range, resulting from the strong-field laser-atom interaction, have been used in a broad range of fascinating applications in all states of matter. In the majority of these studies the harmonic generation process is described using semi-classical theories which treat the electromagnetic field of the driving laser pulse classically without taking into account its quantum nature. In addition, for the measurement of the generated harmonics, all the experiments require diagnostics in the extreme-ultraviolet spectral region. Here by treating the driving laser field quantum mechanically we reveal the quantum-optical nature of the high-order harmonic generation process by measuring the photon number distribution of the infrared light exiting the harmonic generation medium. It is found that the high-order harmonics are imprinted in the photon number distribution of the infrared light and can be recorded without the need of a spectrometer in the extreme-ultraviolet

Time gated ion microscopy of light-atom interactions

The development of ultra-short intense laser sources in the visible and extreme ultraviolet (XUV) spectral range has led to fascinating studies in laser-matter interactions and attosecond science. In the majority of these studies, the system under investigation interacts with a focused light beam, which ionizes the system. The ionization products are usually measured by devices, which spatiotemporally integrate the ionization signal originating from the entire focal area, discarding in this way valuable information about the ionization dynamics that take place in the interaction volume. Here, we review a recently developed approach in measuring the spatially resolved photoionization yields resulting from the interaction of infrared (IR)/XUV ultra-short light pulses in gas phase media. We show how this approach enables (a) the in situ focus diagnostic, (b) quantitative studies of linear and non-linear ionization processes in the IR/XUV regime, (c) single-shot XUV-pump-XUV-probe studies and (d) single-shot 2nd-order XUV autocorrelation measurements

Quantum optical signatures in a strong laser pulse after interaction with semiconductors

Electrodynamical processes induced in complex systems like semiconductors by strong electromagnetic fields have traditionally been described using semiclassical approaches. Although these approaches allowed the investigation of ultrafast dynamics in solids culminating in multipetahertz electronics, they do not provide any access to the quantum-optical nature of the interaction, as they treat the driving field classically and unaffected by the interaction. Here, using a full quantum-optical approach, we demonstrate that the subcycle electronic response in a strongly driven semiconductor crystal is imprinted in the quantum state of the driving field resulting in nonclassical light states carrying the information of the interaction. This vital step towards strong-field ultrafast quantum electrodynamics unravels information inaccessible by conventional approaches and leads to the development of a new class of nonclassical light sources

The ion microscope as a tool for quantitative measurements in the extreme ultraviolet

We demonstrate a tool for quantitative measurements in the extreme ultraviolet (EUV) spectral region measuring spatially resolved atomic ionization products at the focus of an EUV beam. The ionizing radiation is a comb of the 11th-15th harmonics of a Ti:Sapphire femtosecond laser beam produced in a Xenon gas jet. The spatial ion distribution at the focus of the harmonics is recorded using an ion microscope. Spatially resolved single-and two-photon ionization products of Argon and Helium are observed. From such ion distributions single-and two-photon generalized cross sections can be extracted by a self-calibrating method. The observation of spatially resolved two-EUV-photon ionization constitutes an initial step towards future single-shot temporal characterization of attosecond pulses